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Ozone profile retrievals from TROPOMI: Implication for the variation of tropospheric ozone during the outbreak of COVID-19 in China

文献类型：期刊论文

作者Zhao, Fei1; Liu, Cheng1,2,3,7,8; Cai, Zhaonan4; Liu, Xiong5; Bak, Juseon5; Kim, Jae6; Hu, Qihou2; Xia, Congzi9; Zhang, Chengxin9; Sun, Youwen2
刊名SCIENCE OF THE TOTAL ENVIRONMENT
出版日期2021-04-10
卷号764
关键词COVID-19 Ozone profile retrievals TROPOMI Soft calibration Lockdown
ISSN号0048-9697
DOI10.1016/j.scitotenv.2020.142886
通讯作者Liu, Cheng(chliu81@ustc.edu.cn) ; Cai, Zhaonan(caizhaonan@mail.iap.ac.cn)
英文摘要During the outbreak of the coronavirus disease 2019 (COVID-19) in China in January and February 2020, production and living activities were drastically reduced to impede the spread of the virus, which also caused a strong reduction of the emission of primary pollutants. However, as a major species of secondary air pollutant, tropospheric ozone did not reduce synchronously, but instead rose in some region. Furthermore, higher concentrations of ozone may potentially promote the rates of COVID-19 infections, causing extra risk to human health. Thus, the variation of ozone should be evaluated widely. This paper presents ozone profiles and tropospheric ozone columns from ultraviolet radiances detected by TROPOospheric Monitoring Instrument (TROPOMI) onboard Sentinel 5 Precursor (S-5P) satellite based on the principle of optimal estimation method. We compare our TROPOMI retrievals with global ozonesonde observations, Fourier Transform Spectrometry (FTS) observation at Hefei (117.17 degrees E, 31.7 degrees N) and Global Positioning System (GPS) ozonesonde sensor (GPSO(3)) ozonesonde profiles at Beijing (116.46 degrees E, 39.80 degrees N). The integrated Tropospheric Ozone Column (TOC) and Stratospheric Ozone Column (SOC) show excellent agreement with validation data. We use the retrieved TOC combining with tropospheric vertical column density (TVCD) of NO2 and HCHO from TROPOMI to assess the changes of tropospheric during the outbreak of COVID-19 in China. Although NO2 TVCD decreased by 63%, the retrieved TOC over east China increase by 10% from the 20-day averaged before the lockdown on January 23, 2020 to 20-day averaged after it. Because the production of ozone in winter is controlled by volatile organic compounds (VOCs) indicated by monitored HCHO, which did not present evident change during the lockdown, the production of ozone did not decrease significantly. Besides, the decrease of NOx emission weakened the titration of ozone, causing an increase of ozone. (C) 2020 Elsevier B.V. All rights reserved.
资助项目National Key Research and Development Program of China[2018YFC0213104] ; National Key Research and Development Program of China[2016YFC0203302] ; National Key Research and Development Program of China[2017YFC0210002] ; National Natural Science Foundation of China[41722501] ; National Natural Science Foundation of China[41875043] ; National Natural Science Foundation of China[51778596] ; National Natural Science Foundation of China[41977184] ; Anhui Science and Technology Major Project[18030801111] ; Strategic Priority Research Program of the Chinese Academy of Sciences[XDA23020301] ; National Key Project for Causes and Control of Heavy Air Pollution[DQGG0102] ; National Key Project for Causes and Control of Heavy Air Pollution[DQGG0205] ; National High-Resolution Earth Observation Project of China[05-Y20A16-9001-15/17-2] ; National High-Resolution Earth Observation Project of China[05-Y30B01-9001-19/20-3] ; Civil Aerospace Technology Advance Research Project[Y7K00100KJ] ; Innovation Promotion Association, CAS
WOS研究方向Environmental Sciences & Ecology
语种英语
WOS记录号WOS:000614249600072
出版者ELSEVIER
资助机构National Key Research and Development Program of China ; National Natural Science Foundation of China ; Anhui Science and Technology Major Project ; Strategic Priority Research Program of the Chinese Academy of Sciences ; National Key Project for Causes and Control of Heavy Air Pollution ; National High-Resolution Earth Observation Project of China ; Civil Aerospace Technology Advance Research Project ; Innovation Promotion Association, CAS
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/120433]  
专题中国科学院合肥物质科学研究院
通讯作者Liu, Cheng; Cai, Zhaonan
作者单位1.Univ Sci & Technol China, Dept Precis Machinery & Precis Instrumentat, Hefei 230026, Peoples R China
2.Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Key Lab Environm Opt & Technol, Hefei 230031, Peoples R China
3.Chinese Acad Sci, Ctr Excellence Reg Atmospher Environm, Inst Urban Environm, Xiamen 361021, Peoples R China
4.Chinese Acad Sci, Inst Atmospher Phys, Key Lab Middle Atmosphere & Global Environm Obser, Beijing 100029, Peoples R China
5.Harvard Smithsonian Ctr Astrophys, 60 Garden St, Cambridge, MA 02138 USA
6.Pusan Natl Univ, Busan, South Korea
7.Univ Sci & Technol China, Key Lab Precis Sci Instrumentat, Anhui Higher Educ Inst, Hefei 230026, Peoples R China
8.Univ Sci & Technol China, Anhui Prov Key Lab Polar Environm & Global Change, Hefei 230026, Peoples R China
9.Univ Sci & Technol China, Sch Earth & Space Sci, Hefei 230026, Peoples R China
推荐引用方式
GB/T 7714		 Zhao, Fei,Liu, Cheng,Cai, Zhaonan,et al. Ozone profile retrievals from TROPOMI: Implication for the variation of tropospheric ozone during the outbreak of COVID-19 in China[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2021,764.
APA Zhao, Fei.,Liu, Cheng.,Cai, Zhaonan.,Liu, Xiong.,Bak, Juseon.,...&Liu, Jianguo.(2021).Ozone profile retrievals from TROPOMI: Implication for the variation of tropospheric ozone during the outbreak of COVID-19 in China.SCIENCE OF THE TOTAL ENVIRONMENT,764.
MLA Zhao, Fei,et al."Ozone profile retrievals from TROPOMI: Implication for the variation of tropospheric ozone during the outbreak of COVID-19 in China".SCIENCE OF THE TOTAL ENVIRONMENT 764(2021).

入库方式： OAI收割

来源：合肥物质科学研究院

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