Effect of Ru addition to CO/SiO2/HZSM-5 catalysts on Fischer-Tropsch synthesis of gasoline-range hydrocarbons
文献类型：期刊论文
| 作者 | Li, Yu-Ping1 ; Wang, Tie-Jun1; Wu, Chuang-Zhi1; Qin, Xin-Xin1; Tsubaki, Noritatsu2
|
| 刊名 | catalysis communications
 |
| 出版日期 | 2009-08-25 |
| 卷号 | 10期号:14页码:1868-1874 |
| 关键词 | Fischer-Tropsch synthesis Gasoline-range hydrocarbons Ru adding Ru-Co/SiO2/HZSM-5 catalyst |
| ISSN号 | 1566-7367 |
| 通讯作者 | liyp@ms.giec.ac.cn ; wangtj@ms.giec.ac.cn |
| 中文摘要 | microporous hzsm-5 zeolite and mesoporous sio2 supported ru-co catalysts of various ru adding amounts were prepared and evaluated for fischer-tropsch synthesis (fts) of gasoline-range hydrocarbons (c-5-c-12). the tailor-made ru-co/sio2/hzsm-5 catalysts possessed both micro- and mesopores, which accelerated hydrocracking/hydroisomerization of long-chain products and provided quick mass transfer channels respectively during fts. in the same time. ru increased cor reduction degree by hydrogen spillover, thus co conversion of 62.8% and gasoline-range hydrocarbon selectivity of 47%, including more than 14% isoparaffins, were achieved simultaneously when ru content was optimized at 1 wt% in ru-co/sio2/hzsm-5 catalyst. |
| 英文摘要 | microporous hzsm-5 zeolite and mesoporous sio2 supported ru-co catalysts of various ru adding amounts were prepared and evaluated for fischer-tropsch synthesis (fts) of gasoline-range hydrocarbons (c-5-c-12). the tailor-made ru-co/sio2/hzsm-5 catalysts possessed both micro- and mesopores, which accelerated hydrocracking/hydroisomerization of long-chain products and provided quick mass transfer channels respectively during fts. in the same time. ru increased cor reduction degree by hydrogen spillover, thus co conversion of 62.8% and gasoline-range hydrocarbon selectivity of 47%, including more than 14% isoparaffins, were achieved simultaneously when ru content was optimized at 1 wt% in ru-co/sio2/hzsm-5 catalyst. (c) 2009 elsevier b.v. all rights reserved. |
| WOS标题词 | science & technology ; physical sciences |
| 类目[WOS] | chemistry, physical |
| 研究领域[WOS] | chemistry |
| 关键词[WOS] | ru/sio2 catalysts ; co hydrogenation ; iso-paraffins ; syngas ; deactivation ; performance ; conversion ; ru/al2o3 ; mn |
| 收录类别 | SCI |
| 资助信息 | national key basic research program 973 project founded by most of china [2007cb210207]; national 863 plan [2007aa05z416] |
| 原文出处 | http://www.sciencedirect.com/science/journal/15667367 |
| 语种 | 英语 |
| WOS记录号 | WOS:000269664200019 |
| 公开日期 | 2010-09-16 |
| 源URL | [http://ir.giec.ac.cn/handle/344007/3304]  |
| 专题 | 中国科学院广州能源研究所 |
| 作者单位 | 1.Chinese Acad Sci, Key Lab Renewable Energy & Gas Hydrate, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China 2.Toyama Univ, Dept Appl Chem, Sch Engn, Toyama 9308555, Japan |
| 推荐引用方式 GB/T 7714 | Li, Yu-Ping,Wang, Tie-Jun,Wu, Chuang-Zhi,et al. Effect of Ru addition to CO/SiO2/HZSM-5 catalysts on Fischer-Tropsch synthesis of gasoline-range hydrocarbons[J]. catalysis communications,2009,10(14):1868-1874. |
| APA | Li, Yu-Ping,Wang, Tie-Jun,Wu, Chuang-Zhi,Qin, Xin-Xin,&Tsubaki, Noritatsu.(2009).Effect of Ru addition to CO/SiO2/HZSM-5 catalysts on Fischer-Tropsch synthesis of gasoline-range hydrocarbons.catalysis communications,10(14),1868-1874. |
| MLA | Li, Yu-Ping,et al."Effect of Ru addition to CO/SiO2/HZSM-5 catalysts on Fischer-Tropsch synthesis of gasoline-range hydrocarbons".catalysis communications 10.14(2009):1868-1874. |
入库方式： OAI收割
来源：广州能源研究所
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