Scale study of direct synthesis of dimethyl ether from biomass synthesis gas
文献类型：期刊论文
| 作者 | Lv, Yongxing; Wang, Tiejun; Wu, Chuangzhi; Ma, Longlong; Zhou, Yi |
| 刊名 | biotechnology advances
 |
| 出版日期 | 2009-09-01 |
| 卷号 | 27期号:5页码:551-554 |
| ISSN号 | 0734-9750 |
| 关键词 | 100 ton/year scale Biomass Synthesis gas DME |
| 通讯作者 | wucz@ms.giec.ac.cn |
| 中文摘要 | we investigated the synthesis of dimethyl ether (dme) from biomass synthesis gas using a kind of hybrid catalyst consisting of methanol and hzsm-5 zeolite in a fixed-bed reactor in a 100 ton/year pilot plant. the biomass synthesis gas was produced by oxygen-rich gasification of corn core in a two-stage fixed bed. the results showed that co conversions reached 82.00% and 73.55%, the selectivities for dme were 73.95% and 69.73%, and the space-time yields were 124.28 kg m- 3 h- 1 and 203.80 kg m- 3 h- 1 when gas hourly space velocities were 650 h- 1 and 1200 h- 1, respectively. deoxidation and tar removal from biomass synthesis gas was critical to the stable operation of the dme synthesis system. using single-pass synthesis, the h2/co ratio improved from 0.98-1.17 to 2.12-2.22. the yield of dme would be increased greatly if the exhaust was reused after removal of the co2. |
| 英文摘要 | we investigated the synthesis of dimethyl ether (dme) from biomass synthesis gas using a kind of hybrid catalyst consisting of methanol and hzsm-5 zeolite in a fixed-bed reactor in a 100 ton/year pilot plant. the biomass synthesis gas was produced by oxygen-rich gasification of corn core in a two-stage fixed bed. the results showed that co conversions reached 82.00% and 73.55%, the selectivities for dme were 73.95% and 69.73%, and the space-time yields were 124.28 kg m(-3) h(-1) and 203.80 kg m(-3) h(-1) when gas hourly space velocities were 650 h(-1) and 1200 h(-1), respectively. deoxidation and tar removal from biomass synthesis gas was critical to the stable operation of the dme synthesis system. using single-pass synthesis, the h(2)/co ratio improved from 0.98-1.17 to 2.12-2.22. the yield of dme would be increased greatly if the exhaust was reused after removal of the co(2). (c) 2009 elsevier inc. all rights reserved. |
| WOS标题词 | science & technology ; life sciences & biomedicine |
| 类目[WOS] | biotechnology & applied microbiology |
| 研究领域[WOS] | biotechnology & applied microbiology |
| 关键词[WOS] | alternative fuel ; dme ; catalysts |
| 收录类别 | SCI ; ISTP |
| 原文出处 | http://www.sciencedirect.com/science/journal/07349750 |
| 语种 | 英语 |
| WOS记录号 | WOS:000267741300003 |
| 公开日期 | 2010-09-16 |
| 源URL | [http://ir.giec.ac.cn/handle/344007/3322]  |
| 专题 | 中国科学院广州能源研究所 |
| 作者单位 | Chinese Acad Sci, Guangzhou Inst Energy Convers, Key Lab Renewable Energy & Gas Hydrate, Guangzhou 510640, Guangdong, Peoples R China |
| 推荐引用方式 GB/T 7714 | Lv, Yongxing,Wang, Tiejun,Wu, Chuangzhi,et al. Scale study of direct synthesis of dimethyl ether from biomass synthesis gas[J]. biotechnology advances,2009,27(5):551-554. |
| APA | Lv, Yongxing,Wang, Tiejun,Wu, Chuangzhi,Ma, Longlong,&Zhou, Yi.(2009).Scale study of direct synthesis of dimethyl ether from biomass synthesis gas.biotechnology advances,27(5),551-554. |
| MLA | Lv, Yongxing,et al."Scale study of direct synthesis of dimethyl ether from biomass synthesis gas".biotechnology advances 27.5(2009):551-554. |
入库方式： OAI收割
来源：广州能源研究所
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