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Coupling mechanisms of S-Fe-P in surface sediments under the stresses of high salinity and heavy metals in coastal rivers

文献类型：期刊论文

作者Jiang, Ming1,2; Sheng, Yanqing1; Zhao, Guoqiang1,2; Wang, Wenjing1
刊名JOURNAL OF SOILS AND SEDIMENTS
出版日期2021-04-15
页码12
关键词Inorganic sulfur Phosphorus Reactive iron Coastal sediments
ISSN号1439-0108
DOI10.1007/s11368-021-02948-5
通讯作者Sheng, Yanqing(yqsheng@yic.ac.cn)
英文摘要Purpose The aim of the study was to (1) investigate the distributions of sulfur (S), iron (Fe), and phosphorus (P) in coastal surface sediments under the stresses of high salinity and heavy metals; (2) identify potential sources and the environmental geochemical process of S-Fe mineral accumulation; and (3) elucidate the coupling mechanisms of S-Fe-P in coastal sediments under environmental stresses. Materials and methods The distributions of reduced inorganic sulfur (RIS), inorganic P, and reactive Fe (RFe) in surface sediments in two coastal rivers with heavy metals and high salinity (similar to 50 psu, brine drainage) and in offshore areas in the Bohai Sea were investigated. Results and discussion Pyrite sulfur (CRS) was the predominant fraction of RIS in two rivers (Jiaolai River (JL), 56%; Jiehe River (JH), 72%), whereas acid volatile sulfur (AVS) dominated RIS in their offshore sediments (L, 66%; J, 45%). RFe(II) dominated RFe in JH (70%) and JL (66%), while RFe(III) dominated the fractions in their offshore areas (53%). Coastal surface sediments under the stresses of high salinity and heavy metals were dominated by HCl-P (Ca-bound P) and NaOH-P (Fe- and Al-bound P), respectively. Conclusions Accumulated Fe sulfide was limited by elemental sulfur (ES) availability under high salinity, while it was limited by total organic carbon (TOC) availability when the river was heavily polluted. High salinity produced sulfide-dominated environments, which could reduce the NaOH-P and facilitate HCl-P immobilization. However, the presence of heavy metals resulted in Fe-dominated environments, which could promote metal sulfides formation and increase the NaOH-P fixation.
资助项目Strategic Priority Research Program of the Chinese Academy of Sciences[XDA23050203] ; Key Project of Shandong Provincial Natural Science Foundation[ZR2020KE048] ; Key Project of Research and Development Plan of Yantai[2018ZHGY083] ; Key Research and Development Program of Shandong Province[2019GSF109002]
WOS研究方向Environmental Sciences & Ecology ; Agriculture
语种英语
WOS记录号WOS:000640482300001
资助机构Strategic Priority Research Program of the Chinese Academy of Sciences ; Key Project of Shandong Provincial Natural Science Foundation ; Key Project of Research and Development Plan of Yantai ; Key Research and Development Program of Shandong Province
源URL[http://ir.yic.ac.cn/handle/133337/27293]  
专题烟台海岸带研究所_山东省海岸带环境工程技术研究中心
烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
通讯作者Sheng, Yanqing
作者单位1.Chinese Acad Sci, Res Ctr Coastal Environm Engn Technol Shandong Pr, Yantai Inst Coastal Zone Res, Yantai, Peoples R China
2.Univ Chinese Acad Sci, Beijing, Peoples R China
推荐引用方式
GB/T 7714		 Jiang, Ming,Sheng, Yanqing,Zhao, Guoqiang,et al. Coupling mechanisms of S-Fe-P in surface sediments under the stresses of high salinity and heavy metals in coastal rivers[J]. JOURNAL OF SOILS AND SEDIMENTS,2021:12.
APA Jiang, Ming,Sheng, Yanqing,Zhao, Guoqiang,&Wang, Wenjing.(2021).Coupling mechanisms of S-Fe-P in surface sediments under the stresses of high salinity and heavy metals in coastal rivers.JOURNAL OF SOILS AND SEDIMENTS,12.
MLA Jiang, Ming,et al."Coupling mechanisms of S-Fe-P in surface sediments under the stresses of high salinity and heavy metals in coastal rivers".JOURNAL OF SOILS AND SEDIMENTS (2021):12.

入库方式： OAI收割

来源：烟台海岸带研究所

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