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Occurrence and spatial distribution of organophosphorus flame retardants and plasticizers in the Bohai, Yellow and East China seas

文献类型：期刊论文

作者Zhong, Mingyu4; Tang, Jianhui1,5; Guo, Xinyu2; Guo, Chao1,3; Li, Fei1; Wu, Huifeng1
刊名SCIENCE OF THE TOTAL ENVIRONMENT
出版日期2020-11-01
卷号741页码:9
关键词Organophosphate esters Concentrations and distributions Seasonal variation Chinese marginal sea
ISSN号0048-9697
DOI10.1016/j.scitotenv.2020.140434
通讯作者Tang, Jianhui(jhtang@yic.ac.cn)
英文摘要Organophosphate esters (OPEs) are man-made organic pollutants that are used in flame retardants (FRs), plasticizers, antifoaming and hydraulic agents, and extractants. The demand for FRs in China has increased, thereby rapidly increasing the use of OPEs and hence resulted in its high levels in the environment. In this study, we measured the concentrations of seven OPE congeners in the seawaters of the Bohai Sea (BS), the Yellow Sea (YS), and the East China Sea (ECS). The horizontal and vertical spatial distributions were then analyzed to assess the OPE pollution. The total concentrations of the seven OPE congeners (COPEs) in the three seas ranged from 7.31 to 100 ng L-1. The main OPE compounds were tris-(1-chloro-2-propyl) phosphate (TCPP, 3.97-35.6 ng L-1), tris(2-chloroethyl) phosphate (TCEP, 0.59-19.8 ng L-1), and triphenylphosphine oxide (TPPO, from below the detection limit to 43.5 ng L-1). The inventory of the COPEs in the BS, YS, and ECS was estimated as 54.2, 513, and 3950 tons, respectively. Horizontally, the COPE concentration was ranked as BS > YS > ECS. In the vertical direction, the OPE concentrations in the surface water were higher than those in the bottom water. Ocean currents and riverine inputs might be the main factors influencing the distributions of the OPEs in these seas. Moreover, a seasonal variation (summer 2015 versus winter 2016) in the OPEs was observed in the YS, which was probably due to anthropogenic influences and hydrological, meteorological, and biological factors. (c) 2020 Elsevier B.V. All rights reserved.
WOS关键词MASS-SPECTROMETRY ; ESTERS ; CHROMATOGRAPHY ; AIR ; EXTRACTION ; SEDIMENTS ; OCEAN ; WATER ; SEAWATER ; PACIFIC
资助项目National Natural Science Foundation of China[41773138] ; National Natural Science Foundation of China[U1806207] ; project of Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences[YIC Y855011024]
WOS研究方向Environmental Sciences & Ecology
语种英语
WOS记录号WOS:000568814100009
资助机构National Natural Science Foundation of China ; project of Yantai Institute of Coastal Zone Research, Chinese Academy of Sciences
源URL[http://ir.yic.ac.cn/handle/133337/28380]  
专题烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
烟台海岸带研究所_近岸生态与环境实验室
通讯作者Tang, Jianhui
作者单位1.Chinese Acad Sci, Yantai Inst Coastal Zone Res YIC, Key Lab Coastal Environm Proc & Ecol Remediat, Yantai 264003, Peoples R China
2.Ehime Univ, Ctr Marine Environm Studies, Matsuyama, Ehime 7908577, Japan
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
4.Yantai Univ, Ocean Sch, Yantai 264005, Peoples R China
5.Chinese Acad Sci, Ctr Ocean Mega Sci, Qingdao 266071, Peoples R China
推荐引用方式
GB/T 7714		 Zhong, Mingyu,Tang, Jianhui,Guo, Xinyu,et al. Occurrence and spatial distribution of organophosphorus flame retardants and plasticizers in the Bohai, Yellow and East China seas[J]. SCIENCE OF THE TOTAL ENVIRONMENT,2020,741:9.
APA Zhong, Mingyu,Tang, Jianhui,Guo, Xinyu,Guo, Chao,Li, Fei,&Wu, Huifeng.(2020).Occurrence and spatial distribution of organophosphorus flame retardants and plasticizers in the Bohai, Yellow and East China seas.SCIENCE OF THE TOTAL ENVIRONMENT,741,9.
MLA Zhong, Mingyu,et al."Occurrence and spatial distribution of organophosphorus flame retardants and plasticizers in the Bohai, Yellow and East China seas".SCIENCE OF THE TOTAL ENVIRONMENT 741(2020):9.

入库方式： OAI收割

来源：烟台海岸带研究所

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