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New equation to predict size-resolved gas-particle partitioning quotients for polybrominated diphenyl ethers

文献类型：期刊论文

作者Hu, Peng-Tuan2,3,4; Su, Peng-Hao5; Ma, Wan-Li2,3,4; Zhang, Zi-Feng2,3,4; Liu, Li-Yan2,3,4; Song, Wei-Wei2,3,4; Qiao, Li-Na2,3,4; Tian, Chong-Guo6; Macdonald, Robie W.1; Nikolaev, Anatoly7
刊名JOURNAL OF HAZARDOUS MATERIALS
出版日期2020-12-05
卷号400页码:10
关键词Size-segregated Gas/particle partition Polybrominated diphenyl ethers Healthy exposure
ISSN号0304-3894
DOI10.1016/j.jhazmat.2020.123245
通讯作者Li, Yi-Fan(ijrc_pts_paper@yahoo.com)
英文摘要Gas/particle (G/P) partition quotients of semi-volatile organic compounds (SVOCs) for bulk air have been widely discussed in experimental and theoretical contexts, but research on size-resolved G/P partition quotients (K-Pi) are scarce and limited in scope. To investigate G/P partition behavior of polybrominated diphenyl ethers (PBDEs) for size-segregated particles in the atmosphere, 396 individual size-segregated particulate samples (36 batches x 11 size-ranges), and 108 pairs of concurrent gaseous and bulk particulate samples were collected in Harbin, China. A steady-state equation based on bulk particles is derived to determine G/P partition quotients of PBDEs for size-segregated particles, which depends on the organic matter contents of size-segregated particles (f(OMi)). This equation can well predict K-Pi with knowledge of bulk partition quotient (K-PS), ambient temperature, and f(OMi), the results of which match well with monitoring data in Harbin and other published data collected in Shanghai and Guangzhou of China and Thessaloniki of Greece, and remedies a defect of over-estimate K-Pi for high-brominated PBDEs by the previous equation. In particular, the new equation contributes to obtaining the PBDEs concentrations in all atmospheric phase from partial phase, then provides a credible path to evaluate healthy exposure dose from the airborne PBDEs, by co-utilization with exposure models.
WOS关键词POLYCYCLIC AROMATIC-HYDROCARBONS ; HALOGENATED FLAME RETARDANTS ; LONG-RANGE TRANSPORT ; SEMIVOLATILE ORGANIC-CHEMICALS ; DRY DEPOSITION ; AEROSOL-SIZE ; ATMOSPHERIC PARTICLES ; MODEL DEVELOPMENT ; URBAN ATMOSPHERE ; HUMAN EXPOSURE
资助项目National Natural Science Foundation of China[21577030] ; Polar Academy, Harbin Institute of Technology[PA-HIT-201901] ; State Key Laboratory of Urban Water Resource and Environment (Harbin Institute of Technology)[2019DX04]
WOS研究方向Engineering ; Environmental Sciences & Ecology
语种英语
WOS记录号WOS:000572999700005
资助机构National Natural Science Foundation of China ; Polar Academy, Harbin Institute of Technology ; State Key Laboratory of Urban Water Resource and Environment (Harbin Institute of Technology)
源URL[http://ir.yic.ac.cn/handle/133337/28471]  
专题烟台海岸带研究所_近岸生态与环境实验室
烟台海岸带研究所_中科院海岸带环境过程与生态修复重点实验室
通讯作者Li, Yi-Fan
作者单位1.Inst Ocean Sci, Dept Fisheries & Oceans, POB 6000, Sidney, BC V8L 4B2, Canada
2.Harbin Inst Technol HIT, State Key Lab Urban Water Resource & Environm, Int Joint Res Ctr Persistent Tox Subst IJRC PTS, Harbin 150090, Peoples R China
3.HIT PA HIT, Polar Acad, Int Joint Res Ctr Arctic Environm & Ecosyst IJRC, Harbin 150090, Peoples R China
4.HIT, Sch Environm, Heilongjiang Prov Key Lab Polar Environm & Ecosys, Harbin 150090, Peoples R China
5.Shanghai Maritime Univ, Dept Environm Engn, Shanghai 201306, Peoples R China
6.Chinese Acad Sci, Yantai Inst Coastal Zone Res, Yantai, Shandong, Peoples R China
7.North Eastern Fed Univ, Inst Nat Sci, Yakutsk, Russia
8.Henan Normal Univ, Sch Environm, Key Lab Yellow River & Huai River Water Environm, Minist Educ, Xinxiang 453007, Henan, Peoples R China
9.IJRC PTS NA, Toronto, ON M2N 6X9, Canada
推荐引用方式
GB/T 7714		 Hu, Peng-Tuan,Su, Peng-Hao,Ma, Wan-Li,et al. New equation to predict size-resolved gas-particle partitioning quotients for polybrominated diphenyl ethers[J]. JOURNAL OF HAZARDOUS MATERIALS,2020,400:10.
APA Hu, Peng-Tuan.,Su, Peng-Hao.,Ma, Wan-Li.,Zhang, Zi-Feng.,Liu, Li-Yan.,...&Li, Yi-Fan.(2020).New equation to predict size-resolved gas-particle partitioning quotients for polybrominated diphenyl ethers.JOURNAL OF HAZARDOUS MATERIALS,400,10.
MLA Hu, Peng-Tuan,et al."New equation to predict size-resolved gas-particle partitioning quotients for polybrominated diphenyl ethers".JOURNAL OF HAZARDOUS MATERIALS 400(2020):10.

入库方式： OAI收割

来源：烟台海岸带研究所

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