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Hollow Nanostructures for Photocatalysis: Advantages and Challenges

文献类型:期刊论文

作者Xiao, Mu2,3; Wang, Zhiliang2,3; Lyu, Miaoqiang2,3; Luo, Bin2,3; Wang, Songcan2,3; Liu, Gang1,4; Cheng, Hui-Ming1; Wang, Lianzhou2,3
刊名ADVANCED MATERIALS
出版日期2019-09-01
卷号31期号:38页码:23
关键词charge separation hollow nanostructures light harvesting photocatalysis surface reactions
ISSN号0935-9648
DOI10.1002/adma.201801369
通讯作者Liu, Gang(gangliu@imr.ac.cn) ; Wang, Lianzhou(l.wang@uq.edu.au)
英文摘要Photocatalysis for solar-driven reactions promises a bright future in addressing energy and environmental challenges. The performance of photocatalysis is highly dependent on the design of photocatalysts, which can be rationally tailored to achieve efficient light harvesting, promoted charge separation and transport, and accelerated surface reactions. Due to its unique feature, semiconductors with hollow structure offer many advantages in photo-catalyst design including improved light scattering and harvesting, reduced distance for charge migration and directed charge separation, and abundant surface reactive sites of the shells. Herein, the relationship between hollow nanostructures and their photocatalytic performance are discussed. The advantages of hollow nanostructures are summarized as: 1) enhancement in the light harvesting through light scattering and slow photon effects; 2) suppression of charge recombination by reducing charge transfer distance and directing separation of charge carriers; and 3) acceleration of the surface reactions by increasing accessible surface areas for separating the redox reactions spatially. Toward the end of the review, some insights into the key challenges and perspectives of hollow structured photocatalysts are also discussed, with a good hope to shed light on further promoting the rapid progress of this dynamic research field.
资助项目Australian Research Council ; National Natural Science Foundation of China[51629201] ; Australian Government
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
语种英语
WOS记录号WOS:000486253200018
出版者WILEY-V C H VERLAG GMBH
资助机构Australian Research Council ; National Natural Science Foundation of China ; Australian Government
源URL[http://ir.imr.ac.cn/handle/321006/135493]  
专题金属研究所_中国科学院金属研究所
通讯作者Liu, Gang; Wang, Lianzhou
作者单位1.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, 72 Wenhua Rd, Shenyang 110016, Liaoning, Peoples R China
2.Univ Queensland, Sch Chem Engn, Nanomat Ctr, St Lucia, Qld 4072, Australia
3.Univ Queensland, Australian Inst Bioengn & Nanotechnol, St Lucia, Qld 4072, Australia
4.Univ Sci & Technol China, Sch Mat Sci & Engn, 72 Wenhua Rd, Shenyang 110016, Liaoning, Peoples R China
推荐引用方式
GB/T 7714
Xiao, Mu,Wang, Zhiliang,Lyu, Miaoqiang,et al. Hollow Nanostructures for Photocatalysis: Advantages and Challenges[J]. ADVANCED MATERIALS,2019,31(38):23.
APA Xiao, Mu.,Wang, Zhiliang.,Lyu, Miaoqiang.,Luo, Bin.,Wang, Songcan.,...&Wang, Lianzhou.(2019).Hollow Nanostructures for Photocatalysis: Advantages and Challenges.ADVANCED MATERIALS,31(38),23.
MLA Xiao, Mu,et al."Hollow Nanostructures for Photocatalysis: Advantages and Challenges".ADVANCED MATERIALS 31.38(2019):23.

入库方式: OAI收割

来源:金属研究所

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