Highly efficient and stable CuZr-based metallic glassy catalysts for azo dye degradation
文献类型：期刊论文
| 作者 | Zhao, Bowen1,2; Zhu, Zhengwang2; Qin, Xin Dong3; Li, Zhengkun2; Zhang, Haifeng2 |
| 刊名 | JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY
 |
| 出版日期 | 2020-06-01 |
| 卷号 | 46页码:88-97 |
| 关键词 | Metallic glasses Catalytic performance Degradation Azo dyes |
| ISSN号 | 1005-0302 |
| DOI | 10.1016/j.jmst.2019.12.012 |
| 通讯作者 | Zhu, Zhengwang(zwzhu@imr.ac.cn) |
| 英文摘要 | Metallic glasses with the unique disordered atomic structure and metastable nature have been recently applied to degrade the azo dyes and other organic pollutants based on their superior catalytic performance. In this work, the functional properties of six CuZr-based metallic glassy ribbons with the different nominal components in degrading Acid Orange II (AO II) azo dyes were investigated. The Cu47.5Zr46Al6.5 metallic glassy ribbons could exhibit the more advanced catalytic performance for degradation process, which could completely degrade azo dye aqueous solution within 30 min. Additionally, the Cu47.5Zr46Al6.5 metallic glassy ribbons also showed the excellent cyclic stability along with approximately 97.68% degradation efficiency after 10 cycles. These excellent catalytic performance and stability are closely related to the synergistic effect of exposed copper nanoparticles and produced copper oxides in the reaction, which contributes to accelerate the generation of more hydroxyl radicals (OH) to react with dye molecules. Our findings can be able to develop a novel potential metallic glassy material for the functional application of wastewater treatment. (C) 2020 Published by Elsevier Ltd on behalf of The editorial office of Journal of Materials Science & Technology. |
| 资助项目 | National Natural Science Foundation of China[51801209] ; National Natural Science Foundation of China[51790484] ; National Natural Science Foundation of China[U1738101] ; LiaoNing Revitalization Talents Program[XLYC1802078] ; LiaoNing Revitalization Talents Program[XLYC1807062] ; Shenyang National Laboratory for Materials Science ; Dong Guan Innovative Research Team Program[2014607134] ; Shenyang Amorphous Metal Manufacturing Co., Ltd., Shenyang, China |
| WOS研究方向 | Materials Science ; Metallurgy & Metallurgical Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:000525326000009 |
| 出版者 | JOURNAL MATER SCI TECHNOL |
| 资助机构 | National Natural Science Foundation of China ; LiaoNing Revitalization Talents Program ; Shenyang National Laboratory for Materials Science ; Dong Guan Innovative Research Team Program ; Shenyang Amorphous Metal Manufacturing Co., Ltd., Shenyang, China |
| 源URL | [http://ir.imr.ac.cn/handle/321006/138309]  |
| 专题 | 金属研究所_中国科学院金属研究所 |
| 通讯作者 | Zhu, Zhengwang |
| 作者单位 | 1.Univ Sci & Technol China, Sch Mat Sci & Engn, Shenyang 110016, Peoples R China 2.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Peoples R China 3.Liaoning Univ, Coll Chem, Inst Rare & Scattered Elements, Shenyang 110036, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhao, Bowen,Zhu, Zhengwang,Qin, Xin Dong,et al. Highly efficient and stable CuZr-based metallic glassy catalysts for azo dye degradation[J]. JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY,2020,46:88-97. |
| APA | Zhao, Bowen,Zhu, Zhengwang,Qin, Xin Dong,Li, Zhengkun,&Zhang, Haifeng.(2020).Highly efficient and stable CuZr-based metallic glassy catalysts for azo dye degradation.JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY,46,88-97. |
| MLA | Zhao, Bowen,et al."Highly efficient and stable CuZr-based metallic glassy catalysts for azo dye degradation".JOURNAL OF MATERIALS SCIENCE & TECHNOLOGY 46(2020):88-97. |
入库方式： OAI收割
来源：金属研究所
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