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Single-atom catalysts for metal-sulfur batteries: Current progress and future perspectives

文献类型：期刊论文

作者Xiao, Ru3,4; Chen, Ke1,3; Zhang, Xiaoyin3,4; Yang, Zhenzhen2,3; Hu, Guangjian3,4; Sun, Zhenhua3,4; Cheng, Hui-Ming3,4,5; Li, Feng3,4
刊名JOURNAL OF ENERGY CHEMISTRY
出版日期2021-03-01
卷号54页码:452-466
关键词Single-atom catalysts Metal-sulfur batteries Redox kinetics Synthesis Characterization Electrochemical performance
ISSN号2095-4956
DOI10.1016/j.jechem.2020.06.018
通讯作者Sun, Zhenhua(zhsun@imr.ac.cn) ; Li, Feng(fli@imr.ac.cn)
英文摘要Metal-sulfur batteries are recognized as a promising candidate for next generation electrochemical energy storage systems owing to their high theoretical energy density, low cost and environmental friendliness. However, sluggish redox kinetics of sulfur species and the shuttle effect lead to large polarization and severe capacity decay. Numerous approaches from physical barrier, chemical adsorption strategies to electrocatalysts have been tried to solve these issues and pushed the rate and cycle performance of sulfur electrodes to higher levels. Most recently, single-atom catalysts (SACs) with high catalytic efficiency have been introduced into metal-sulfur systems to achieve fast redox kinetics of sulfur conversion. In this review, we systematically summarize the current progress on SACs for sulfur electrodes from aspects of synthesis, characterization and electrochemical performance. Challenges and potential solutions for designing SACs for high-performance sulfur electrodes are discussed. (C) 2020 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. All rights reserved.
资助项目National Natural Science Foundation of China[51972313] ; National Natural Science Foundation of China[51525206] ; National Natural Science Foundation of China[51927803] ; Ministry of Science and Technology of China[2016YFA0200100] ; Ministry of Science and Technology of China[2016YFB0100100] ; Strategic Priority Research Program of Chinese Academy of Science[XDA22010602] ; Youth Innovation Promotion Association of the Chinese Academy of Sciences[Y201942] ; Key Research Program of Chinese Academy of Sciences[KGZD-EW-T06] ; Special Projects of the Central Government in Guidance of Local Science and Technology Development[2020JH6/10500024] ; Program for Guangdong Introducing Innovative and Entrepreneurial Teams ; Development and Reform Commission of Shenzhen Municipality ; China Petrochemical Cooperation[218025] ; Economic, The Bureau of Industry and Information Technology of Shenzhen for the 2017 Graphene Manufacturing Innovation Center Project[201901171523]
WOS研究方向Chemistry ; Energy & Fuels ; Engineering
语种英语
WOS记录号WOS:000605249800011
出版者ELSEVIER
资助机构National Natural Science Foundation of China ; Ministry of Science and Technology of China ; Strategic Priority Research Program of Chinese Academy of Science ; Youth Innovation Promotion Association of the Chinese Academy of Sciences ; Key Research Program of Chinese Academy of Sciences ; Special Projects of the Central Government in Guidance of Local Science and Technology Development ; Program for Guangdong Introducing Innovative and Entrepreneurial Teams ; Development and Reform Commission of Shenzhen Municipality ; China Petrochemical Cooperation ; Economic, The Bureau of Industry and Information Technology of Shenzhen for the 2017 Graphene Manufacturing Innovation Center Project
源URL[http://ir.imr.ac.cn/handle/321006/158957]  
专题金属研究所_中国科学院金属研究所
通讯作者Sun, Zhenhua; Li, Feng
作者单位1.ShanghaiTech Univ, Sch Phys Sci & Technol, Shanghai 201210, Peoples R China
2.Jilin Univ, Coll Phys, Key Lab Phys & Technol Adv Batteries, Minist Educ, Changchun 130012, Jilin, Peoples R China
3.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Liaoning, Peoples R China
4.Univ Sci & Technol China, Sch Mat Sci & Engn, Hefei 230026, Anhui, Peoples R China
5.Tsinghua Univ, Shenzhen Geim Graphene Ctr, Tsinghua Berkeley Shenzhen Inst, Shenzhen 518055, Guangdong, Peoples R China
推荐引用方式
GB/T 7714		 Xiao, Ru,Chen, Ke,Zhang, Xiaoyin,et al. Single-atom catalysts for metal-sulfur batteries: Current progress and future perspectives[J]. JOURNAL OF ENERGY CHEMISTRY,2021,54:452-466.
APA Xiao, Ru.,Chen, Ke.,Zhang, Xiaoyin.,Yang, Zhenzhen.,Hu, Guangjian.,...&Li, Feng.(2021).Single-atom catalysts for metal-sulfur batteries: Current progress and future perspectives.JOURNAL OF ENERGY CHEMISTRY,54,452-466.
MLA Xiao, Ru,et al."Single-atom catalysts for metal-sulfur batteries: Current progress and future perspectives".JOURNAL OF ENERGY CHEMISTRY 54(2021):452-466.

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来源：金属研究所

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