Simultaneous removal of NO(x)and SO(2)using two-stage O(3)oxidation combined with Ca(OH)(2)absorption
文献类型:期刊论文
作者 | Zou, Yang1,2; Wang, Yan2; Liu, Xiaolong2; Zhu, Tingyu2,3; Tian, Mengkui1; Cai, Maoyu1,2 |
刊名 | KOREAN JOURNAL OF CHEMICAL ENGINEERING
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出版日期 | 2020-10-17 |
页码 | 8 |
关键词 | Iron Ore Sintering Flue Gas SO2 NOx Ozone Two-stage Oxidation |
ISSN号 | 0256-1115 |
DOI | 10.1007/s11814-020-0597-z |
英文摘要 | This paper proposes two-stage O(3)oxidation combined with Ca(OH)(2)for simultaneous removal of NO(x)and SO2(NOx: Nitrogen oxides including NO, NO(2)and N2O5). In two-stage oxidation, NO was first oxidized to NO(2)in an oxidation tube, and NO(2)was further oxidized into N(2)O(5)in the spray tower. NO(x)and SO(2)were simultaneously removed in the spray tower. This method can effectively reduce the extra waste of O(3)caused by the decomposition of N2O5, especially at high temperature. Effects of various factors on denitrification efficiency were investigated. The results showed that the NO(x)removal efficiency decreased and O(3)extra consumption ratio increased with the increase of oxidation temperature or oxidation reaction time. When the O-3/NO molar ratio was 1.8, one-stage O(3)oxidation at 150(o)C extra wasted 33.3% of O-3. With the increase of O(3)concentration at site 2, the NO(x)removal efficiency first increased and then stabilized. Compared with the one-stage O(3)oxidation-absorption, the two-stage oxidation-absorption improved NO(x)removal efficiency from 62.5% to 89%. In addition, the increase of CaSO(3)slurry concentration had little effect on the denitrification efficiency. |
WOS关键词 | NITRIC-OXIDE REMOVAL ; FLUE-GAS ; SIMULTANEOUS ABSORPTION ; COMBINED PERSULFATE ; OXIDATION-REMOVAL ; OZONE OXIDATION ; NO OXIDATION ; SO2 ; TEMPERATURE ; POLLUTION |
资助项目 | National key research and development program of China[2017YFC0210600] ; National Natural Science Foundation of China[51978644] |
WOS研究方向 | Chemistry ; Engineering |
语种 | 英语 |
WOS记录号 | WOS:000578940600001 |
出版者 | KOREAN INSTITUTE CHEMICAL ENGINEERS |
资助机构 | National key research and development program of China ; National Natural Science Foundation of China |
源URL | [http://ir.ipe.ac.cn/handle/122111/42473] ![]() |
专题 | 中国科学院过程工程研究所 |
通讯作者 | Liu, Xiaolong; Zhu, Tingyu |
作者单位 | 1.Guizhou Univ, Sch Chem & Chem Engn, Guiyang 550025, Guizhou, Peoples R China 2.Chinese Acad Sci, Beijing Engn Res Ctr Proc Pollut Control, Natl Engn Lab Hydrometallurg Cleaner Prod Technol, Inst Proc Engn, Beijing 100190, Peoples R China 3.Chinese Acad Sci, Inst Urban Environm, Ctr Excellence Reg Atmospher Environm, Xiamen 361021, Peoples R China |
推荐引用方式 GB/T 7714 | Zou, Yang,Wang, Yan,Liu, Xiaolong,et al. Simultaneous removal of NO(x)and SO(2)using two-stage O(3)oxidation combined with Ca(OH)(2)absorption[J]. KOREAN JOURNAL OF CHEMICAL ENGINEERING,2020:8. |
APA | Zou, Yang,Wang, Yan,Liu, Xiaolong,Zhu, Tingyu,Tian, Mengkui,&Cai, Maoyu.(2020).Simultaneous removal of NO(x)and SO(2)using two-stage O(3)oxidation combined with Ca(OH)(2)absorption.KOREAN JOURNAL OF CHEMICAL ENGINEERING,8. |
MLA | Zou, Yang,et al."Simultaneous removal of NO(x)and SO(2)using two-stage O(3)oxidation combined with Ca(OH)(2)absorption".KOREAN JOURNAL OF CHEMICAL ENGINEERING (2020):8. |
入库方式: OAI收割
来源:过程工程研究所
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