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Development of Rapid Curing SiO2 Aerogel Composite-Based QuasiSolid-State Dye-Sensitized Solar Cells through Screen-Printing Technology

文献类型：期刊论文

作者Jiao, Shouzheng2; Sun, Zhicheng2; Wen, Jinyue2; Liu, Yuanyuan3; Li, Furong2; Miao, Qingqing1,4; Wu, Weixia2; Li, Luhai2; Zhou, Yang3
刊名ACS APPLIED MATERIALS & INTERFACES
出版日期2020-10-28
卷号12期号:43页码:48794-48803
关键词dye-sensitized solar cells SiO2 aerogel quasi-solid-state electrolyte rapid curing screen printing
ISSN号1944-8244
DOI10.1021/acsami.0c14551
英文摘要Gratzel's dye-sensitized solar cells (DSSCs) can readily convert sunlight into electricity, attracting considerable attention of global scientists. The fabrication efficiency of DSSCs was greatly limited by the slow fabrication (similar to 3.5-24 h) of quasi-solid (QS) electrolytes to date. In this study, novel composites of SiO2 aerogel with graphene (GR), multi-walled carbon nanotubes, or polyaniline were proposed in the fabrication of QS-state electrolytes. The morphology of these composites was characterized. The gels with SiO2 aerogels as QS electrolytes of DSSCs can be rapidly cured in similar to 3 s. Using the screen-printing technology, these QS electrolytes can be readily utilized to construct the QS-DSSC to provide high efficiency and great stability. The photovoltaic parameters and interfacial chargetransfer resistances of the QS-DSSC incorporated with our synthetic composites were investigated in detail. Specifically, the SiO2 aerogel composed of GR (SiO2@GR) as a gel can greatly improve the performance of QS-DSSCs up to 8.25%. It is likely that these SiO2 aerogel composite electrolytes could provide a rapid curing process in the preparation of QS-state DSSCs, which might be useful to promote the development of DSSCs for future industrialization.
WOS关键词GEL POLYMER ELECTROLYTES ; SILICA NANOPARTICLES ; IONIC LIQUID ; HIGH-EFFICIENCY ; PHOTOVOLTAIC PERFORMANCE ; REDOX ELECTROLYTE ; HOLE TRANSFER ; SURFACE-AREA ; LOW-COST ; HYBRID
资助项目National Natural Science Foundation of China[21776021] ; National Natural Science Foundation of China[21646013] ; National Natural Science Foundation of China[22007025] ; National Natural Science Foundation of China[21878309] ; National Natural Science Foundation of China[22078340] ; Key Scientific Research Project of Beijing Municipal commission of Education[KZ201910015016] ; BIGC Project[Ec202004] ; Youth Innovation Promotion Association, Chinese Academy of Sciences (CAS) ; Natural Science Foundation of Hebei Province[E2019103008] ; Hainan University[KYQD (ZR)20041] ; Hainan University[KYQD (ZR) 20040]
WOS研究方向Science & Technology - Other Topics ; Materials Science
语种英语
WOS记录号WOS:000586868400056
出版者AMER CHEMICAL SOC
资助机构National Natural Science Foundation of China ; Key Scientific Research Project of Beijing Municipal commission of Education ; BIGC Project ; Youth Innovation Promotion Association, Chinese Academy of Sciences (CAS) ; Natural Science Foundation of Hebei Province ; Hainan University
源URL[http://ir.ipe.ac.cn/handle/122111/42686]  
专题中国科学院过程工程研究所
通讯作者Sun, Zhicheng; Miao, Qingqing; Zhou, Yang
作者单位1.Chinese Acad Sci, Langfang Inst Proc Engn, Langfang 065001, Peoples R China
2.Beijing Inst Graph Commun, Beijing Engn Res Ctr Printed Elect, Beijing 102600, Peoples R China
3.Hainan Univ, Sch Chem Engn & Technol, Minist Educ, Key Lab Adv Mat Trop Isl Resources, Haikou 570228, Hainan, Peoples R China
4.Chinese Acad Sci, Inst Proc Engn, CAS Key Lab Green Proc & Engn, Beijing Key Lab Ion Liquids Clean Proc, Beijing 100190, Peoples R China
推荐引用方式
GB/T 7714		 Jiao, Shouzheng,Sun, Zhicheng,Wen, Jinyue,et al. Development of Rapid Curing SiO2 Aerogel Composite-Based QuasiSolid-State Dye-Sensitized Solar Cells through Screen-Printing Technology[J]. ACS APPLIED MATERIALS & INTERFACES,2020,12(43):48794-48803.
APA Jiao, Shouzheng.,Sun, Zhicheng.,Wen, Jinyue.,Liu, Yuanyuan.,Li, Furong.,...&Zhou, Yang.(2020).Development of Rapid Curing SiO2 Aerogel Composite-Based QuasiSolid-State Dye-Sensitized Solar Cells through Screen-Printing Technology.ACS APPLIED MATERIALS & INTERFACES,12(43),48794-48803.
MLA Jiao, Shouzheng,et al."Development of Rapid Curing SiO2 Aerogel Composite-Based QuasiSolid-State Dye-Sensitized Solar Cells through Screen-Printing Technology".ACS APPLIED MATERIALS & INTERFACES 12.43(2020):48794-48803.

入库方式： OAI收割

来源：过程工程研究所

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