中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Oil shale pyrolysis in a moving bed with internals enhanced by rapid preheating in a heated drop tube

文献类型:期刊论文

作者Chen, Zhaohui2,4; Tian, Yong4; Lai, Dengguo3; Zhan, Jin-hui4; Han, Zhennan1; Xu, Guangwen1,4; Gao, Shiqiu4
刊名ENERGY CONVERSION AND MANAGEMENT
出版日期2020-11-15
卷号224页码:10
ISSN号0196-8904
关键词Oil shale pyrolysis Moving bed with internals Rapid preheating Drop tube Volatiles reaction Shale oil
DOI10.1016/j.enconman.2020.113358
英文摘要The enhanced oil shale pyrolysis in a moving bed with internals (MBI) by rapid preheating in a drop tube was developed to improve the quality of shale oil through reaction regulation in stages. Initially rapid preheating of oil shale in the upper drop tube endowed the generation of massive free radical fragments and volatile precursors, which would simultaneously restrict the remarkable release of volatiles from particles to minimize the gas-phase secondary reactions. The preheated oil shale subsequently fell into the lower MBI to shape a granular bed with the cocurrent flow of heat and volatiles. In the MBI, the oil shale pyrolysis and volatiles reactions were directed and regulated by matching the flow and temperature fields to realize the selective cracking of heavy fraction in shale oil. The granular bed also served as a filter for the in-situ removal of dust entrained by the volatiles. The shale oil yield reached 83.0% of Fischer Assay oil yield, its light fraction was as high as 89.2 wt% and dust content was as low as 0.6 wt%. The advantages of pyrolysis in the MBI enhanced by rapid preheating were further justified by comparison with other pyrolysis processes.
WOS关键词HIGH-QUALITY TAR ; INTEGRATED FLUIDIZED-BED ; FIXED-BED ; COAL PYROLYSIS ; PRODUCT DISTRIBUTION ; SECONDARY REACTIONS ; SYNGAS PRODUCTION ; CARRIER ; GASIFICATION ; COMBUSTION
资助项目National Natural Science Foundation of China[U1908201]
WOS研究方向Thermodynamics ; Energy & Fuels ; Mechanics
语种英语
出版者PERGAMON-ELSEVIER SCIENCE LTD
WOS记录号WOS:000603322000010
资助机构National Natural Science Foundation of China
源URL[http://ir.ipe.ac.cn/handle/122111/43158]  
专题中国科学院过程工程研究所
通讯作者Lai, Dengguo; Xu, Guangwen
作者单位1.Shenyang Univ Chem Technol, Inst Ind Chem & Energy Technol, Shenyang 110142, Peoples R China
2.Polytech Montreal, Proc Engn Adv Res Lab PEARL, Chem Engn Dept, Montreal, PQ H3T 1J4, Canada
3.Chinese Acad Sci, Inst Urban Environm, CAS Key Lab Urban Pollutant Convers, Xiamen 361021, Peoples R China
4.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China
推荐引用方式
GB/T 7714
Chen, Zhaohui,Tian, Yong,Lai, Dengguo,et al. Oil shale pyrolysis in a moving bed with internals enhanced by rapid preheating in a heated drop tube[J]. ENERGY CONVERSION AND MANAGEMENT,2020,224:10.
APA Chen, Zhaohui.,Tian, Yong.,Lai, Dengguo.,Zhan, Jin-hui.,Han, Zhennan.,...&Gao, Shiqiu.(2020).Oil shale pyrolysis in a moving bed with internals enhanced by rapid preheating in a heated drop tube.ENERGY CONVERSION AND MANAGEMENT,224,10.
MLA Chen, Zhaohui,et al."Oil shale pyrolysis in a moving bed with internals enhanced by rapid preheating in a heated drop tube".ENERGY CONVERSION AND MANAGEMENT 224(2020):10.

入库方式: OAI收割

来源:过程工程研究所

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