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CFD Simulation of a Fluid-Solid Non-Catalytic Reaction Based on a Structure-Based Mass Transfer Model: Shrinking Spherical Reaction

文献类型：期刊论文

作者Zou, Zheng1,3; Zhu, Jingyi1,3; Jia, Jibin1,3; Du, Zhan3; Wang, Qiao2; Zhu, Qingshan1,3; Li, Hongzhong1,3
刊名INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
出版日期2020-11-11
卷号59期号:45页码:19989-19998
ISSN号0888-5885
DOI10.1021/acs.iecr.0c04409
英文摘要To forecast the mass transfer behavior in consideration of noncatalytic solid reaction characteristics with the shrinking spherical model (SPM), a structure-based mass transfer model taking account of the gas-solid mass exchange within both the emulsion and bubble/interphase phases is built and coupled with computational fluid dynamics (CFD) to predict the carbochlorination of TiO2 with a binary gas-solid phase system. Based on the validation through comparing with the experimental data, the simulation gives a comprehensive understanding and deep analysis of the gas-solid reaction that is helpful for the design and optimization of a non-catalytic fluidized reactor. It is concluded that the fluidized mass transfer process with a heterogeneous flow structure is not only affected by the chemical reaction rate but also dependent on local flow parameters.
资助项目National Natural Science Foundation of China[21878304] ; National Natural Science Foundation of China[21736010] ; National Natural Science Foundation of China[21908227] ; Science Fund for Creative Research Groups of the National Natural Science Foundation of China[21921005] ; State Key Laboratory of Multiphase Complex Systems[MPCS-2019-A-07]
WOS研究方向Engineering
语种英语
WOS记录号WOS:000592479200016
出版者AMER CHEMICAL SOC
资助机构National Natural Science Foundation of China ; Science Fund for Creative Research Groups of the National Natural Science Foundation of China ; State Key Laboratory of Multiphase Complex Systems
源URL[http://ir.ipe.ac.cn/handle/122111/43167]  
专题中国科学院过程工程研究所
通讯作者Zou, Zheng; Zhu, Qingshan
作者单位1.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
2.Chinese Acad Sci, Comp Network Informat Ctr, Beijing 100190, Peoples R China
3.Chinese Acad Sci, Inst Proc Engn, State Key Lab Multi Phase Complex Syst, Beijing 100190, Peoples R China
推荐引用方式
GB/T 7714		 Zou, Zheng,Zhu, Jingyi,Jia, Jibin,et al. CFD Simulation of a Fluid-Solid Non-Catalytic Reaction Based on a Structure-Based Mass Transfer Model: Shrinking Spherical Reaction[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2020,59(45):19989-19998.
APA Zou, Zheng.,Zhu, Jingyi.,Jia, Jibin.,Du, Zhan.,Wang, Qiao.,...&Li, Hongzhong.(2020).CFD Simulation of a Fluid-Solid Non-Catalytic Reaction Based on a Structure-Based Mass Transfer Model: Shrinking Spherical Reaction.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,59(45),19989-19998.
MLA Zou, Zheng,et al."CFD Simulation of a Fluid-Solid Non-Catalytic Reaction Based on a Structure-Based Mass Transfer Model: Shrinking Spherical Reaction".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 59.45(2020):19989-19998.

入库方式： OAI收割

来源：过程工程研究所

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