Delicate Control on the Shell Structure of Hollow Spheres Enables Tunable Mass Transport in Water Splitting
文献类型：期刊论文
| 作者 | Hou, Ping1,2; Li, Dan1; Yang, Nailiang1,2; Wan, Jiawei1; Zhang, Chunhui3; Zhang, Xiqi3; Jiang, Hongyu4; Zhang, Qinghua4; Gu, Lin4; Wang, Dan1,2 |
| 刊名 | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
 |
| 出版日期 | 2021-02-18 |
| 页码 | 7 |
| 关键词 | duplicate shells hollow structures mass transport multi-shell structures water splitting |
| ISSN号 | 1433-7851 |
| DOI | 10.1002/anie.202016285 |
| 英文摘要 | In the study of structure-property relationships for rational materials design, hollow multishell structures (HoMSs) have attracted tremendous attention owing to the optimal balance between mass transfer and surface exposure. Considering the shell structure can significantly affect the properties of HoMSs, in this paper, we provide a novel one-step strategy to continually regulate the shell structures of HoMSs. Through a simple phosphorization process, we can effectively modify the shell from solid to bubble-like and even duplicate the shells with a narrow spacing. Benefitting from the structure merits, the fabricated CoP HoMSs with close duplicated shells can promote gas release owing to the unbalanced Laplace pressure, while accelerating liquid transfer for enhanced capillary force. It can provide effective channels for water and gas and thus exhibits a superior electrocatalytic performance in the hydrogen and oxygen evolution reaction. |
| 资助项目 | National Natural Science Foundation of China[21931012] ; National Natural Science Foundation of China[21821005] ; National Natural Science Foundation of China[21971244] ; National Natural Science Foundation of China[51932001] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000618975200001 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| 资助机构 | National Natural Science Foundation of China |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/43637]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Wang, Dan |
| 作者单位 | 1.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, 1 North 2nd St, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, 19A Yuquan Rd, Beijing 10049, Peoples R China 3.Chinese Acad Sci, Tech Inst Phys & Chem, Lab Bioinspired Mat & Interface Sci, Beijing 100190, Peoples R China 4.Chinese Acad Sci, Inst Phys, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Hou, Ping,Li, Dan,Yang, Nailiang,et al. Delicate Control on the Shell Structure of Hollow Spheres Enables Tunable Mass Transport in Water Splitting[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2021:7. |
| APA | Hou, Ping.,Li, Dan.,Yang, Nailiang.,Wan, Jiawei.,Zhang, Chunhui.,...&Wang, Dan.(2021).Delicate Control on the Shell Structure of Hollow Spheres Enables Tunable Mass Transport in Water Splitting.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,7. |
| MLA | Hou, Ping,et al."Delicate Control on the Shell Structure of Hollow Spheres Enables Tunable Mass Transport in Water Splitting".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021):7. |
入库方式： OAI收割
来源：过程工程研究所
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