中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Imaging the formation and surface phase separation of the CE phase

文献类型:期刊论文

作者Zhou, Haibiao3,4,5,6; Feng, Qiyuan4,5,6; Hou, Yubin4; Nakamura, Masao2; Tokura, Yoshinori1,2,7; Kawasaki, Masashi1,2,7; Sheng, Zhigao4,5,6,8; Lu, Qingyou4,5,6,8
刊名NPJ QUANTUM MATERIALS
出版日期2021-06-03
卷号6
DOI10.1038/s41535-021-00353-2
通讯作者Zhou, Haibiao(haibiaozhou24@gmail.com) ; Sheng, Zhigao(zhigaosheng@hmfl.ac.cn) ; Lu, Qingyou(qxl@ustc.edu.cn)
英文摘要The CE phase is an extraordinary phase exhibiting the simultaneous spin, charge, and orbital ordering due to strong electron correlation. It is an ideal platform to investigate the role of the multiple orderings in the phase transitions and discover emergent properties. Here, we use a cryogenic high-field magnetic force microscope to image the phase transitions and properties of the CE phase in a Pr0.5Ca0.5MnO3 thin film. In a high magnetic field, we observed a clear suppression of magnetic susceptibility at the charge-ordering insulator transition temperature (T-COI), whereas, at the Neel temperature (T-N), no significant change is observed. This observation favors the scenario of strong antiferromagnetic correlation developed below T-COI but raises questions about the Zener polaron paramagnetic phase picture. Besides, we discoverd a phase-separated surface state in the CE phase regime. Ferromagnetic phase domains residing at the surface already exist in zero magnetic field and show ultra-high magnetic anisotropy. Our results provide microscopic insights into the unconventional spin- and charge-ordering transitions and revealed essential attributes of the CE phase, highlighting unusual behaviors when multiple electronic orderings are involved.
WOS关键词MAGNETIC-FIELD ; CHARGE ; TRANSITION ; MECHANISMS ; ORDER
资助项目National Key Research and Development Program of China[2017YFA0402903] ; National Key Research and Development Program of China[2017YFA0303603] ; National Key Research and Development Program of China[2016YFA0401003] ; National Key Research and Development Program of China[2016YFA0401803] ; National Natural Science Foundation of China (NSFC)[U1932216] ; National Natural Science Foundation of China (NSFC)[51627901] ; National Natural Science Foundation of China (NSFC)[U2032218] ; National Natural Science Foundation of China (NSFC)[11574316] ; National Natural Science Foundation of China (NSFC)[21505139] ; National Natural Science Foundation of China (NSFC)[11474263] ; National Natural Science Foundation of China (NSFC)[U1432251] ; National Natural Science Foundation of China (NSFC)[11374278] ; National Natural Science Foundation of China (NSFC)[U1632160] ; National Natural Science Foundation of China (NSFC)[11704384] ; Maintenance and Renovation Project for CAS[DSS-WXGZ-2019-0011] ; Key Research Program of Frontier Sciences, CAS[QYZDB-SSW-SLH011] ; Instrument Developing Project of the Chinese Academy of Sciences[YZ201423] ; Hefei Science Center CAS[2020HSC-UE014] ; High Magnetic Field Laboratory of Anhui Province ; Chinese Academy of Science Scientific Research Equipment[YZ201628] ; One Thousand Youth Talents Program of China ; Japan Science and Technology (JST), PRESTO[JPMJPR16R5] ; Anhui Lab of Adv. Photon Sci. and Tech.
WOS研究方向Materials Science ; Physics
语种英语
WOS记录号WOS:000657744800001
出版者NATURE RESEARCH
资助机构National Key Research and Development Program of China ; National Natural Science Foundation of China (NSFC) ; Maintenance and Renovation Project for CAS ; Key Research Program of Frontier Sciences, CAS ; Instrument Developing Project of the Chinese Academy of Sciences ; Hefei Science Center CAS ; High Magnetic Field Laboratory of Anhui Province ; Chinese Academy of Science Scientific Research Equipment ; One Thousand Youth Talents Program of China ; Japan Science and Technology (JST), PRESTO ; Anhui Lab of Adv. Photon Sci. and Tech.
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/123694]  
专题中国科学院合肥物质科学研究院
通讯作者Zhou, Haibiao; Sheng, Zhigao; Lu, Qingyou
作者单位1.Univ Tokyo, Dept Appl Phys, Tokyo, Japan
2.RIKEN Ctr Emergent Matter Sci CEMS, Wako, Saitama, Japan
3.Weizmann Inst Sci, Dept Condensed Matter Phys, Rehovot, Israel
4.Chinese Acad Sci, High Field Magnet Lab, Anhui Key Lab Condensed Matter Phys Extreme Condi, High Field Magnet Lab, Hefei, Peoples R China
5.Univ Sci & Technol China, Hefei Natl Lab Phys Sci Microscale, Hefei, Peoples R China
6.Univ Sci & Technol China, Anhui Lab Adv Photon Sci & Technol, Hefei, Peoples R China
7.Univ Tokyo, Quantum Phase Elect Res Ctr QPEC, Tokyo, Japan
8.Nanjing Univ, Collaborat Innovat Ctr Adv Microstruct, Nanjing, Peoples R China
推荐引用方式
GB/T 7714
Zhou, Haibiao,Feng, Qiyuan,Hou, Yubin,et al. Imaging the formation and surface phase separation of the CE phase[J]. NPJ QUANTUM MATERIALS,2021,6.
APA Zhou, Haibiao.,Feng, Qiyuan.,Hou, Yubin.,Nakamura, Masao.,Tokura, Yoshinori.,...&Lu, Qingyou.(2021).Imaging the formation and surface phase separation of the CE phase.NPJ QUANTUM MATERIALS,6.
MLA Zhou, Haibiao,et al."Imaging the formation and surface phase separation of the CE phase".NPJ QUANTUM MATERIALS 6(2021).

入库方式: OAI收割

来源:合肥物质科学研究院

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