中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Two-center interference and stereo Wigner time delay in photoionization of asymmetric molecules

文献类型:期刊论文

作者Liao, Yijie5,6; Zhou, Yueming5,6; Pi, Liang-Wen3,4; Ke, Qinghua5,6; Liang, Jintai5,6; Zhao, Yong5,6; Li, Min5,6; Lu, Peixiang1,2,5,6
刊名PHYSICAL REVIEW A
出版日期2021-07-20
卷号104期号:1
ISSN号2469-9926;2469-9934
DOI10.1103/PhysRevA.104.013110
产权排序3
英文摘要

We present numerical simulations of the time delay in photoemission of asymmetric diatomic molecules using the technique of reconstruction of attosecond beating by interference of two-photon transitions (RABITT) by solving the time-dependent Schrodinger equation. Our results show an obvious time delay between photoelectrons emitted to the left and right and this relative time delay oscillates as the photoelectron energy changes. More interestingly, the amplitude of this oscillation increases when the asymmetry degree of diatomic molecules decreases. With the method of the selected continuum wave functions, we calculate the Wigner time delay in photoionization. The obtained stereo Wigner time delay also oscillates with photoelectron energy. This oscillation is traced back to two-center interferences and it could explain the relative time delay in the RABITT measurement. Furthermore, our results indicate that the continuum-continuum time delay in photoemission of heteronuclear molecules is asymmetric.

语种英语
出版者AMER PHYSICAL SOC
WOS记录号WOS:000675550300005
源URL[http://ir.opt.ac.cn/handle/181661/94979]  
专题西安光学精密机械研究所_瞬态光学技术国家重点实验室
通讯作者Zhou, Yueming
作者单位1.CAS Ctr Excellence Ultraintense Laser Sci, Shanghai 201800, Peoples R China
2.Wuhan Inst Technol, Hubei Key Lab Opt Informat & Pattern Recognit, Wuhan 430205, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
4.Chinese Acad Sci, State Key Lab Transient Opt & Photon, Xian Inst Opt & Precis Mech, Xian 710119, Peoples R China
5.Huazhong Univ Sci & Technol, Wuhan Natl Lab Optoelect, Wuhan 430074, Peoples R China
6.Huazhong Univ Sci & Technol, Sch Phys, Wuhan 430074, Peoples R China
推荐引用方式
GB/T 7714
Liao, Yijie,Zhou, Yueming,Pi, Liang-Wen,et al. Two-center interference and stereo Wigner time delay in photoionization of asymmetric molecules[J]. PHYSICAL REVIEW A,2021,104(1).
APA Liao, Yijie.,Zhou, Yueming.,Pi, Liang-Wen.,Ke, Qinghua.,Liang, Jintai.,...&Lu, Peixiang.(2021).Two-center interference and stereo Wigner time delay in photoionization of asymmetric molecules.PHYSICAL REVIEW A,104(1).
MLA Liao, Yijie,et al."Two-center interference and stereo Wigner time delay in photoionization of asymmetric molecules".PHYSICAL REVIEW A 104.1(2021).

入库方式: OAI收割

来源:西安光学精密机械研究所

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