Engineering a chemoenzymatic cascade for sustainable photobiological hydrogen production with green algae
文献类型:期刊论文
作者 | Chen, J; Li, J; Li, Q; Wang, S; Wang, LH; Liu, HJ; Fan, CH |
刊名 | ENERGY & ENVIRONMENTAL SCIENCE |
出版日期 | 2020 |
卷号 | 13期号:7页码:2064-2068 |
ISSN号 | 1754-5692 |
关键词 | CHLAMYDOMONAS-REINHARDTII CHLOROPHYLL CONTENT H-2 PHOTOPRODUCTION EVOLUTION |
DOI | 10.1039/d0ee00993h |
文献子类 | 期刊论文 |
英文摘要 | Photobiological hydrogen generation is among the most promising routes for the mass production of hydrogen energy. However, the cost and sustainability of photobiological methods largely hamper their large-scale commercial production. Here, we design an anaerobic environment with a constant near-neutral pH for the sustainable induction of green algae flocculation by engineering a robust chemoenzymatic cascade system consisting of glucose, glucose oxidase, catalase, and magnesium hydroxide. We found thatChlamydomonas reinhardtiicould stably produce hydrogen in this engineered photobiological system for nearly a month, with an average rate of 0.44 mu mol H(2)h(-1)(mg chlorophyll)(-1). This study thus opens a new avenue to photobiological hydrogen production at industrial scales for promising "liquid sunshine" applications. |
语种 | 英语 |
源URL | [http://ir.sinap.ac.cn/handle/331007/32851] |
专题 | 上海应用物理研究所_中科院上海应用物理研究所2011-2017年 |
作者单位 | 1.Shanghai Jiao Tong Univ, Sch Chem & Chem Engn, Shanghai 200240, Peoples R China 2.Chinese Acad Sci, Div Phys Biol, CAS Key Lab Interfacial Phys & Technol, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China 3.Chinese Acad Sci, Shanghai Synchrotron Radiat Facil, Zhangjiang Lab, Shanghai Adv Res Inst, Shanghai, Peoples R China 4.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 5.Tongji Univ, Shanghai Res Inst Intelligent Autonomous Syst, Key Lab Adv Civil Engn Mat, Sch Chem Sci & Engn,Minist Educ, Shanghai 200092, Peoples R China |
推荐引用方式 GB/T 7714 | Chen, J,Li, J,Li, Q,et al. Engineering a chemoenzymatic cascade for sustainable photobiological hydrogen production with green algae[J]. ENERGY & ENVIRONMENTAL SCIENCE,2020,13(7):2064-2068. |
APA | Chen, J.,Li, J.,Li, Q.,Wang, S.,Wang, LH.,...&Fan, CH.(2020).Engineering a chemoenzymatic cascade for sustainable photobiological hydrogen production with green algae.ENERGY & ENVIRONMENTAL SCIENCE,13(7),2064-2068. |
MLA | Chen, J,et al."Engineering a chemoenzymatic cascade for sustainable photobiological hydrogen production with green algae".ENERGY & ENVIRONMENTAL SCIENCE 13.7(2020):2064-2068. |
入库方式: OAI收割
来源:上海应用物理研究所
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