Enhanced Performance in Uranium Extraction by Quaternary Ammonium-Functionalized Amidoxime-Based Fibers
文献类型：期刊论文
| 作者 | Ao, JX; Han, JG; Xu, X; Qi, SM; Ma, L; Wang, ZQ; Zhang, L; Li, QN; Xu, L; Ma, HJ |
| 刊名 | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
 |
| 出版日期 | 2020 |
| 卷号 | 59期号:13页码:5828-5837 |
| 关键词 | MAGNETIC NANOPARTICLES ADSORPTION PERFORMANCE EFFICIENT EXTRACTION CHEMICAL SPECIATION MESOPOROUS SILICA AQUEOUS-SOLUTIONS SEAWATER ADSORBENT RECOVERY OPTIMIZATION |
| ISSN号 | 0888-5885 |
| DOI | 10.1021/acs.iecr.9b06829 |
| 文献子类 | 期刊论文 |
| 英文摘要 | Acrylonitrile and 2-(dimethylamino)ethyl methacrylate were grafted onto ultrahigh molecular weight polyethylene fibers, and a series of quaternary ammonium (Q)-functionalized amidoxime (AO)-based fibers including QAO fibers and AO-Q fibers were synthesized. The optimal preparation process was determined. The results show that the QAO fibers with quaternary ammonium grafting chains in the inner layer and the amidoxime groups in the outer layer exhibited the best adsorption performance. Enhanced adsorption kinetics and adsorption capacities of the Q-AO fibers were obtained in simulated seawater. In comparison with the AO-Q fibers, the Q-AO fibers showed a higher adsorption capacity of 29.73 mg/g, which was 54.7% higher than that of the AO-Qfiber and 108.6% higher than that of the traditional amidoximebased adsorbent (AO fiber). These implied the obvious effect on the distinction of the preparation processes. Compared with AO fibers, the adsorption capacity for uranium by the Q-AO fibers in natural seawater increased nearly seven-fold to 0.210 mg/g, while the capacity for other metal ions decreased. This study concluded that synergistic groups with positive charges could result in enhanced adsorption performance for uranyl tricarbonate from natural seawater, and the distribution distinction of the AO group and synergistic group deeply affect the adsorption performance. |
| 语种 | 英语 |
| 源URL | [http://ir.sinap.ac.cn/handle/331007/32856]  |
| 专题 | 上海应用物理研究所_中科院上海应用物理研究所2011-2017年 |
| 作者单位 | 1.Guilin Univ Elect Technol, Guangxi Key Lab Optoeletron Informat Proc, Guilin 541004, Peoples R China 2.Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China 3.Univ Chinese Acad Sci, Shanghai 201800, Peoples R China 4.Jining Univ, Qufu 273155, Shandong, Peoples R China |
| 推荐引用方式 GB/T 7714 | Ao, JX,Han, JG,Xu, X,et al. Enhanced Performance in Uranium Extraction by Quaternary Ammonium-Functionalized Amidoxime-Based Fibers[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2020,59(13):5828-5837. |
| APA | Ao, JX.,Han, JG.,Xu, X.,Qi, SM.,Ma, L.,...&Ma, HJ.(2020).Enhanced Performance in Uranium Extraction by Quaternary Ammonium-Functionalized Amidoxime-Based Fibers.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,59(13),5828-5837. |
| MLA | Ao, JX,et al."Enhanced Performance in Uranium Extraction by Quaternary Ammonium-Functionalized Amidoxime-Based Fibers".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 59.13(2020):5828-5837. |
入库方式： OAI收割
来源：上海应用物理研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。