Experimental Investigation of the Hydrate-Based Gas Separation of Synthetic Flue Gas with 5A Zeolite
文献类型：期刊论文
| 作者 | Zang, Xiaoya1,2,3,4 ; Zhang, Na1; Zhou, Xuebing1,2,3,4; Wan, Lihua1,2,3,4; Liang, Deqing1,2,3,4
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| 刊名 | ENERGIES
 |
| 出版日期 | 2020-09-01 |
| 卷号 | 13期号:17页码:12 |
| 关键词 | hydrate 5A zeolite flue gas CO2 separation |
| DOI | 10.3390/en13174556 |
| 通讯作者 | Liang, Deqing(liangdq@ms.giec.ac.cn) |
| 英文摘要 | Coal combustion flue gas contains CO2, a greenhouse gas and driver of climate change. Therefore, CO2 separation and removal is necessary. Fortunately, 5A zeolites are highly porous and can be used as a CO2 adsorbent. In addition, they act as nuclei for hydrate formation. In this work, a composite technology, based on the physical adsorption of CO2 by 5A zeolite and hydrate-based gas separation, was used to separate CO2/N-2 gas mixtures. The influence of water content, temperature, pressure, and particle size on gas adsorption and CO2 separation was studied, revealing that the CO2 separation ability of zeolite particles sized 150-180 mu m was better than that of those sized 380-830 mu m at 271.2 K and 273.2 K. When the zeolite particles were 150-180 mu m (type-B zeolite) with a water content of 35.3%, the gas consumption per mole of water (n(gas)/n(H2O)) reached the maximum, 0.048, and the CO2 separation ratio reached 14.30%. The CO2 molar concentration in the remaining gas phase (x(CO2)(gas)) was lowest at 271.2 K in the type-B zeolite system with a water content of 47.62%. Raman analysis revealed that CO2 preferentially occupied the small hydrate cages and there was a competitive relationship between N-2 and CO2. |
| WOS关键词 | CARBON-DIOXIDE CAPTURE ; CO2 CAPTURE ; ADSORPTION ; N-2 ; CH4 |
| 资助项目 | National key research and development plan of China[2017YFC0307305] ; National Natural Science Foundation of China[51676197] ; Guangzhou Science and Technology Project[201804010411] ; Youth Innovation Promotion Association CAS |
| WOS研究方向 | Energy & Fuels |
| 语种 | 英语 |
| WOS记录号 | WOS:000569626900001 |
| 出版者 | MDPI |
| 资助机构 | National key research and development plan of China ; National Natural Science Foundation of China ; Guangzhou Science and Technology Project ; Youth Innovation Promotion Association CAS |
| 源URL | [http://ir.giec.ac.cn/handle/344007/32027]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Liang, Deqing |
| 作者单位 | 1.Chinese Acad Sci, Guangzhou Ctr Gas Hydrate Res, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China 2.CAS Key Lab Gas Hydrate, Guangzhou 510640, Peoples R China 3.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China 4.State Key Lab Nat Gas Hydrate, Beijing 100028, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zang, Xiaoya,Zhang, Na,Zhou, Xuebing,et al. Experimental Investigation of the Hydrate-Based Gas Separation of Synthetic Flue Gas with 5A Zeolite[J]. ENERGIES,2020,13(17):12. |
| APA | Zang, Xiaoya,Zhang, Na,Zhou, Xuebing,Wan, Lihua,&Liang, Deqing.(2020).Experimental Investigation of the Hydrate-Based Gas Separation of Synthetic Flue Gas with 5A Zeolite.ENERGIES,13(17),12. |
| MLA | Zang, Xiaoya,et al."Experimental Investigation of the Hydrate-Based Gas Separation of Synthetic Flue Gas with 5A Zeolite".ENERGIES 13.17(2020):12. |
入库方式： OAI收割
来源：广州能源研究所
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