Steam reforming of toluene over nickel catalysts supported on coal gangue ash
文献类型：期刊论文
| 作者 | Lu, Min1,2,3; Xiong, Zuhong1,2,3 ; Fang, Kejing1,2,3; Li, Xi1,2,3; Li, Jiqing1,2,3; Li, Tao1,2,3
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| 刊名 | RENEWABLE ENERGY
 |
| 出版日期 | 2020-11-01 |
| 卷号 | 160页码:385-395 |
| 关键词 | Tar Coal gangue ash Catalyst Toluene Carbon deposition |
| ISSN号 | 0960-1481 |
| DOI | 10.1016/j.renene.2020.06.012 |
| 通讯作者 | Xiong, Zuhong(xiongzh@ms.giec.ac.cn) |
| 英文摘要 | The development of high performance and low-cost catalyst is very important to remove tar during biomass gasification. Solid waste coal gangue ash (CGA), which mainly contains SiO2, Al2O3, Fe2O3 and CaO, was selected as support for Ni-based catalyst. The prepared low-cost catalysts were characterized suitably by XRD, BET, TPR, SEM, TG and Raman techniques. Toluene was selected as typical biomass tar model compounds to test the catalyst performance and compared with traditional catalysts Ni/Al2O3 and Ni/SiO2. Ni/CGA-1d exhibited the highest catalytic performance with the toluene conversion and H-2 yield accounting for 91.5% and 58.2% respectively, at 800 degrees C. It was showed that the performance of Ni/CGA-1d was higher than traditional catalysts Ni/Al2O3 and Ni/SiO2, and comparable with other polymetallic reforming catalysts. Due to the good resistance of carbon deposition, the Ni/CGA-1d catalyst also per formed better catalytic activity stability. The ability should be attributing to the existence of some metal elements such as Fe, Mg, K, Ca et al. in coal gangue ash support. (C) 2020 Published by Elsevier Ltd. |
| WOS关键词 | OIL MODEL COMPOUNDS ; BIOMASS TAR ; HYDROGEN-PRODUCTION ; WASTE TIRES ; GASIFICATION ; DEACTIVATION ; COMPOUND ; ALUMINA ; SULFUR ; CARBON |
| 资助项目 | National Natural Science Foundation of China[21606228] |
| WOS研究方向 | Science & Technology - Other Topics ; Energy & Fuels |
| 语种 | 英语 |
| WOS记录号 | WOS:000572886800005 |
| 出版者 | PERGAMON-ELSEVIER SCIENCE LTD |
| 资助机构 | National Natural Science Foundation of China |
| 源URL | [http://ir.giec.ac.cn/handle/344007/32068]  |
| 专题 | 中国科学院广州能源研究所 |
| 通讯作者 | Xiong, Zuhong |
| 作者单位 | 1.CAS Key Lab Renewable Energy, Guangzhou 510640, Peoples R China 2.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China 3.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China |
| 推荐引用方式 GB/T 7714 | Lu, Min,Xiong, Zuhong,Fang, Kejing,et al. Steam reforming of toluene over nickel catalysts supported on coal gangue ash[J]. RENEWABLE ENERGY,2020,160:385-395. |
| APA | Lu, Min,Xiong, Zuhong,Fang, Kejing,Li, Xi,Li, Jiqing,&Li, Tao.(2020).Steam reforming of toluene over nickel catalysts supported on coal gangue ash.RENEWABLE ENERGY,160,385-395. |
| MLA | Lu, Min,et al."Steam reforming of toluene over nickel catalysts supported on coal gangue ash".RENEWABLE ENERGY 160(2020):385-395. |
入库方式： OAI收割
来源：广州能源研究所
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