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ZSM-5-Supported Graphene-Encapsulated Nickel Nanoparticles: Formation, Properties, and Exceptional Performance in Lipid Hydrogenation

文献类型：期刊论文

作者Li, Ming3,4,5; Fu, Junying3,4,5; Lv, Pengmei1,3,4,5; Zhang, Xufeng3,4,5; Liu, Xiaochun2,3,4,5; Zeng, Qiongyao2,3,4,5; Yang, Lingmei3,4,5; Wang, Zhongming3,4,5; Yuan, Zhenhong3,4,5
刊名ACS SUSTAINABLE CHEMISTRY & ENGINEERING
出版日期2020-10-19
卷号8期号:41页码:15484-15495
关键词graphene hydrogenation jet fuel nickel loss nickel agglomeration
ISSN号2168-0485
DOI10.1021/acssuschemeng.0c03559
通讯作者Fu, Junying(fujy@ms.giec.ac.cn) ; Lv, Pengmei(lvpm@ms.giec.ac.cn)
英文摘要Graphene-encapsulated nickel nanoparticles (Ni@C) were loaded on Zeolite Socony Mobil (ZSM)-5 for lipid hydrogenation to produce biojet fuel. Ni@C and ZSM-5 exhibit an efficient and synergistic catalytic activity, and the strong chemical interaction between graphene and nickel significantly improves the hydrogenation capacity of the catalyst. The graphene layers strengthened the dispersion of nickel, reduced the size of Ni@C to similar to 3.6 nm, and kept the valence state of nickel at 0. According to the hydrogenation tests, the conversion of oleic acid to jet fuel could reach 98.59% with only 3 wt % nickel loading amount. Furthermore, Ni@C/ZSM-5 shows excellent resistance to nickel agglomeration and loss.
WOS关键词BIO-JET FUEL ; CARBON NANOTUBES ; FATTY-ACIDS ; OLEIC-ACID ; RANGE HYDROCARBONS ; VEGETABLE-OILS ; NONEDIBLE OIL ; FOSSIL-FUELS ; METAL ; CATALYSTS
资助项目Guangdong Special Support Program[2017TX04Z109] ; National Key RD Program[2019YFB1504003] ; Natural Science Foundation of Guangdong Province[2016A030308004] ; Natural Science Foundation of Guangdong Province[2018A030310078] ; National Natural Science Foundation of China[51861145103] ; National Natural Science Foundation of China Youth[51903236]
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Engineering
语种英语
WOS记录号WOS:000584349900008
出版者AMER CHEMICAL SOC
资助机构Guangdong Special Support Program ; National Key RD Program ; Natural Science Foundation of Guangdong Province ; National Natural Science Foundation of China ; National Natural Science Foundation of China Youth
源URL[http://ir.giec.ac.cn/handle/344007/34856]  
专题中国科学院广州能源研究所
通讯作者Fu, Junying; Lv, Pengmei
作者单位1.Collaborat Innovat Ctr Biomass Energy, Zhengzhou 450002, Henan, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Guangdong Prov Key Lab New & Renewable Energy Res, Guangzhou 510640, Peoples R China
4.CAS Key Lab Renewable Energy, Guangzhou 510640, Peoples R China
5.Chinese Acad Sci, Guangzhou Inst Energy Convers, Guangzhou 510640, Peoples R China
推荐引用方式
GB/T 7714		 Li, Ming,Fu, Junying,Lv, Pengmei,et al. ZSM-5-Supported Graphene-Encapsulated Nickel Nanoparticles: Formation, Properties, and Exceptional Performance in Lipid Hydrogenation[J]. ACS SUSTAINABLE CHEMISTRY & ENGINEERING,2020,8(41):15484-15495.
APA Li, Ming.,Fu, Junying.,Lv, Pengmei.,Zhang, Xufeng.,Liu, Xiaochun.,...&Yuan, Zhenhong.(2020).ZSM-5-Supported Graphene-Encapsulated Nickel Nanoparticles: Formation, Properties, and Exceptional Performance in Lipid Hydrogenation.ACS SUSTAINABLE CHEMISTRY & ENGINEERING,8(41),15484-15495.
MLA Li, Ming,et al."ZSM-5-Supported Graphene-Encapsulated Nickel Nanoparticles: Formation, Properties, and Exceptional Performance in Lipid Hydrogenation".ACS SUSTAINABLE CHEMISTRY & ENGINEERING 8.41(2020):15484-15495.

入库方式： OAI收割

来源：广州能源研究所

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