Comprehensive characterization of hygroscopic properties of methanesulfonates
文献类型:期刊论文
作者 | Guo, Liya; Peng, Chao; Zong, Taomou; Gu, Wenjun; Ma, Qingxin; Wu, Zhijun; Wang, Zhe; Ding, Xiang; Hu, Min; Wang, Xinming |
刊名 | ATMOSPHERIC ENVIRONMENT |
出版日期 | 2020-03-01 |
卷号 | 224页码:1-8 |
ISSN号 | 1352-2310 |
关键词 | Hygroscopic properties Methanesulfonate Aerosol-water interaction Dimethyl sulfide Marine aerosol |
英文摘要 | Methanesulfonate, formed in atmospheric oxidation of dimethyl sulfide, is abundant in marine aerosols; however, its hygroscopic properties have not been well understood. In this work, two complementary techniques (a vapor sorption analyzer and a humidity tandem differential mobility analyzer) were employed to investigate hygroscopic properties of CH3SO3Na, CH3SO3K and (CH3SO3)(2)Ca at different relative humidities (RH). The deliquescence relative humidities were measured to be 70-71% for CH3SO3Na at 15-35 degrees C, displaying no dependence on temperature. The mass changes at 90% RH, relative to that at <1% RH, were measured to be 4.002 +/- 0.053 for CH3SO3Na, 3.479 +/- 0.031 for CH3SO3K, and 3.663 +/- 0.019 for (CH3SO3)(2)Ca at 25 degrees C. CH3SO3Na and CH3SO3K aerosols started to grow at >70% RH, while continuous growth since very low RH (<40%) was observed for (CH3SO3)(2)Ca aerosols. At room temperature, hygroscopic growth factors at 90% RH were measured to be 1.48 +/- 0.02, 1.53 +/- 0.04 and 1.65 +/- 0.02 for CH3SO3Na, CH3SO3K and (CH3SO3)(2)Ca aerosols, respectively. |
源URL | [http://ir.rcees.ac.cn/handle/311016/45024] |
专题 | 生态环境研究中心_水污染控制实验室 |
推荐引用方式 GB/T 7714 | Guo, Liya,Peng, Chao,Zong, Taomou,et al. Comprehensive characterization of hygroscopic properties of methanesulfonates[J]. ATMOSPHERIC ENVIRONMENT,2020,224:1-8. |
APA | Guo, Liya.,Peng, Chao.,Zong, Taomou.,Gu, Wenjun.,Ma, Qingxin.,...&Tang, Mingjin.(2020).Comprehensive characterization of hygroscopic properties of methanesulfonates.ATMOSPHERIC ENVIRONMENT,224,1-8. |
MLA | Guo, Liya,et al."Comprehensive characterization of hygroscopic properties of methanesulfonates".ATMOSPHERIC ENVIRONMENT 224(2020):1-8. |
入库方式: OAI收割
来源:生态环境研究中心
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