Distribution, sources and transport of organophosphorus flame retardants in the water and sediment of Ny-Alesund, Svalbard, the Arctic
文献类型:期刊论文
作者 | Gao, Xiaozhong; Xu, Yiping; Ma, Mei; Huang, Qinghui; Gabrielsen, Geir Wing; Hallanger, Ingeborg; Rao, Kaifeng; Lu, Zhibo; Wang, Zijian |
刊名 | ENVIRONMENTAL POLLUTION |
出版日期 | 2020-09 |
卷号 | 264页码:1-8 |
ISSN号 | 0269-7491 |
关键词 | Organophosphorus flame retardants The Arctic Passive sampling Water Spatial distribution |
英文摘要 | Organophosphorus flame retardants (PFRs) are contaminants of emerging concern which have been detected globally. However, little information on PFRs in the Arctic freshwater environment is currently available. In this study, both hydrophilic and hydrophobic PFRs in the water and sediment of four areas (town, surroundings, coastal marine water, and glacier melt runoff) near Ny-Alesund Svalbard were investigated by time-integrated passive sampling (water) and grab sampling (sediment). Seven kinds of PFRs were found in the Arctic waters with individual freely dissolved concentrations from 0.007 ng L-1 to 355 ng L-1, and the concentrations of chlorinated PFRs were 3-4 orders of magnitude higher than those of non-chlorinated PFRs. The distribution of different PFRs in freshwater showed significant spatial differences among the different areas, and the town was found to have most kinds of PFRs and highest PFRs concentrations. The sources and transport of different kinds of PFRs were explored based on a spatial overlay analysis of the contaminant distributions, environmental conditions, and PFR applications. As a result, human settlements, industrial activities, atmospheric deposition, and transportation in Ny-Alesund were proposed to be related to the pollution of different PFRs at Ny-Alesund. The PFRs in the inshore marine water were found to be affected by both local ship contamination and ocean current transport. Furthermore, nine PFRs were detected in the sediments of Ny-Alesund. Accumulation of different PFRs in the Arctic sediment was found to be dominated by their physico-chemical properties (polarity). (C) 2020 Elsevier Ltd. All rights reserved. |
源URL | [http://ir.rcees.ac.cn/handle/311016/45269] |
专题 | 生态环境研究中心_中国科学院饮用水科学与技术重点实验室 |
推荐引用方式 GB/T 7714 | Gao, Xiaozhong,Xu, Yiping,Ma, Mei,et al. Distribution, sources and transport of organophosphorus flame retardants in the water and sediment of Ny-Alesund, Svalbard, the Arctic[J]. ENVIRONMENTAL POLLUTION,2020,264:1-8. |
APA | Gao, Xiaozhong.,Xu, Yiping.,Ma, Mei.,Huang, Qinghui.,Gabrielsen, Geir Wing.,...&Wang, Zijian.(2020).Distribution, sources and transport of organophosphorus flame retardants in the water and sediment of Ny-Alesund, Svalbard, the Arctic.ENVIRONMENTAL POLLUTION,264,1-8. |
MLA | Gao, Xiaozhong,et al."Distribution, sources and transport of organophosphorus flame retardants in the water and sediment of Ny-Alesund, Svalbard, the Arctic".ENVIRONMENTAL POLLUTION 264(2020):1-8. |
入库方式: OAI收割
来源:生态环境研究中心
浏览0
下载0
收藏0
其他版本
除非特别说明,本系统中所有内容都受版权保护,并保留所有权利。