A Durable and Efficient Electrocatalyst for Saline Water Splitting with Current Density Exceeding 2000 mA cm(-2)
文献类型：期刊论文
| 作者 | Yang, Fengning1,2; Luo, Yuting1,2; Yu, Qiangmin1,2; Zhang, Zhiyuan1,2; Zhang, Shuo3; Liu, Zhibo4; Ren, Wencai4; Cheng, Hui-Ming1,2,4; Li, Jiong3; Liu, Bilu1,2 |
| 刊名 | ADVANCED FUNCTIONAL MATERIALS
 |
| 出版日期 | 2021-03-12 |
| 页码 | 10 |
| ISSN号 | 1616-301X |
| 关键词 | high current density hydrogen evolution reaction low Pt catalyst saline water water splitting |
| DOI | 10.1002/adfm.202010367 |
| 通讯作者 | Li, Jiong(lijiong@sinap.ac.cn) ; Liu, Bilu(bilu.liu@sz.tsinghua.edu.cn) |
| 英文摘要 | Water electrolysis is promising for industrial hydrogen production to achieve a sustainable and green hydrogen economy, but the high cost of the technology limits its market share. Developing efficient yet economic electrocatalysts is crucial to decrease the cost of electricity and electrolytic cell. Meanwhile, electrolysis in seawater electrolyte can further reduce feedstock cost. Here, a type of electrocatalyst is synthesized, where trace precious metals are strongly anchored on a corrosion-resistive matrix. As an example, the produced Pt/Ni-Mo electrocatalyst only needs an overpotential of 113 mV to reach an ultrahigh current density of 2000 mA cm(-2) in the saline-alkaline electrolyte, demonstrating the best performance reported thus far. It shows high activity and long durability in various electrolytes and under harsh conditions, including strong alkaline and simulated seawater electrolytes, and under elevated temperatures up to 80 degrees C. This electrocatalyst is produced on a large scale at a low cost and shows good performance in a commercial membrane electrode assembly stack, demonstrating its feasibility for practical water electrolysis. |
| 资助项目 | National Natural Science Foundation of China[51722206] ; Guangdong Innovative and Entrepreneurial Research Team Program[2017ZT07C341] ; Bureau of Industry and Information Technology of Shenzhen[201901171523] ; Youth 1000-Talent Program of China |
| WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
| 语种 | 英语 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| WOS记录号 | WOS:000627911100001 |
| 资助机构 | National Natural Science Foundation of China ; Guangdong Innovative and Entrepreneurial Research Team Program ; Bureau of Industry and Information Technology of Shenzhen ; Youth 1000-Talent Program of China |
| 源URL | [http://ir.imr.ac.cn/handle/321006/161751]  |
| 专题 | 金属研究所_中国科学院金属研究所 |
| 通讯作者 | Li, Jiong; Liu, Bilu |
| 作者单位 | 1.Tsinghua Univ, Tsinghua Berkeley Shenzhen Inst, Shenzhen Geim Graphene Ctr, Shenzhen 518055, Peoples R China 2.Tsinghua Univ, Tsinghua Shenzhen Int Grad Sch, Shenzhen 518055, Peoples R China 3.Chinese Acad Sci, Shanghai Adv Res Inst, Shanghai Synchrotron Radiat Facil, Shanghai 201210, Peoples R China 4.Chinese Acad Sci, Inst Met Res, Shenyang Natl Lab Mat Sci, Shenyang 110016, Liaoning, Peoples R China |
| 推荐引用方式 GB/T 7714 | Yang, Fengning,Luo, Yuting,Yu, Qiangmin,et al. A Durable and Efficient Electrocatalyst for Saline Water Splitting with Current Density Exceeding 2000 mA cm(-2)[J]. ADVANCED FUNCTIONAL MATERIALS,2021:10. |
| APA | Yang, Fengning.,Luo, Yuting.,Yu, Qiangmin.,Zhang, Zhiyuan.,Zhang, Shuo.,...&Liu, Bilu.(2021).A Durable and Efficient Electrocatalyst for Saline Water Splitting with Current Density Exceeding 2000 mA cm(-2).ADVANCED FUNCTIONAL MATERIALS,10. |
| MLA | Yang, Fengning,et al."A Durable and Efficient Electrocatalyst for Saline Water Splitting with Current Density Exceeding 2000 mA cm(-2)".ADVANCED FUNCTIONAL MATERIALS (2021):10. |
入库方式： OAI收割
来源：金属研究所
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