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Metal-organic frameworks containing solid-state electrolytes for lithium metal batteries and beyond

文献类型：期刊论文

作者Chen, Tianhua1; Chen, Shimou2,3; Chen, Yong4; Zhao, Ming3; Losic, Dusan1; Zhang, Suojiang2
刊名MATERIALS CHEMISTRY FRONTIERS
出版日期2021-02-21
卷号5期号:4页码:1771-1794
DOI10.1039/d0qm00856g
英文摘要For solid-state Li and other metal batteries, solid-state electrolytes (SSEs) are a bridge between electrodes, and are significant in determining the behavior of batteries. Thus, constructing stable and excellent SSEs is vital for the feasible application of metal batteries. Because of their unique and multifunctional properties, namely unsaturated metal sites, tunable structure, and high specific surface area, porous metal-organic frameworks (MOFs) have been applied to SSEs to enhance the performance of metal batteries. In this review, the mechanisms of MOFs within polymer electrolytes on improving the Li-ion movement, stabilizing the solid/solid interfacial contact, and prohibiting the Li dendrite are briefly summarized. The multiple factors of MOF-based SSEs, including MOF structures, unsaturated metal sites, incorporation with ionic liquids, different organic ligands, pore size and nano/micro hierarchical structure that affect the battery performance are comprehensively discussed. Moreover, the mechanism and advancement of MOF-based SSEs for other metal batteries, including Na, Zn, and Mg batteries, are also illustrated. Eventually, new insights and future prospects in terms of MOF-based SSEs are proposed to stimulate more innovative approaches for the commercial applications of Li and other metal batteries.
资助项目National Natural Science Foundation of China[51922099] ; Innovation Academy for Light-duty Gas Turbine, Chinese Academy of Sciences[CXYJJ20-MS-05] ; Natural Science Foundation of Hebei Province for Distinguished Young Scholars[E2020103052]
WOS研究方向Chemistry ; Materials Science
语种英语
WOS记录号WOS:000621097700012
出版者ROYAL SOC CHEMISTRY
资助机构National Natural Science Foundation of China ; Innovation Academy for Light-duty Gas Turbine, Chinese Academy of Sciences ; Natural Science Foundation of Hebei Province for Distinguished Young Scholars
源URL[http://ir.ipe.ac.cn/handle/122111/47882]  
专题中国科学院过程工程研究所
通讯作者Chen, Shimou; Losic, Dusan; Zhang, Suojiang
作者单位1.Univ Adelaide, Sch Chem Engn & Adv Mat, Adelaide, SA 5005, Australia
2.Chinese Acad Sci, Inst Proc Engn, Beijing 100190, Peoples R China
3.Beijing Univ Chem Technol, State Key Lab Organ Inorgan Composites, Beijing 100029, Peoples R China
4.China Univ Min & Technol, Sch Chem & Environm Engn, Beijing 100083, Peoples R China
推荐引用方式
GB/T 7714		 Chen, Tianhua,Chen, Shimou,Chen, Yong,et al. Metal-organic frameworks containing solid-state electrolytes for lithium metal batteries and beyond[J]. MATERIALS CHEMISTRY FRONTIERS,2021,5(4):1771-1794.
APA Chen, Tianhua,Chen, Shimou,Chen, Yong,Zhao, Ming,Losic, Dusan,&Zhang, Suojiang.(2021).Metal-organic frameworks containing solid-state electrolytes for lithium metal batteries and beyond.MATERIALS CHEMISTRY FRONTIERS,5(4),1771-1794.
MLA Chen, Tianhua,et al."Metal-organic frameworks containing solid-state electrolytes for lithium metal batteries and beyond".MATERIALS CHEMISTRY FRONTIERS 5.4(2021):1771-1794.

入库方式： OAI收割

来源：过程工程研究所

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