Ion-Exchange Resins for Efficient Removal of Colorants in Bis(hydroxyethyl) Terephthalate
文献类型：期刊论文
| 作者 | Huang, Rong2,3; Zhang, Qi2,3; Yao, Haoyu2,3; Lu, Xingmei1,2,3,4; Zhou, Qing1,2,3; Yan, Dongxia2 |
| 刊名 | ACS OMEGA
 |
| 出版日期 | 2021-05-11 |
| 卷号 | 6期号:18页码:12351-12360 |
| ISSN号 | 2470-1343 |
| DOI | 10.1021/acsomega.1c01477 |
| 英文摘要 | Bis(hydroxyethyl) terephthalate (BHET) obtained from waste poly(ethylene terephthalate) (PET) glycolysis often have undesirable colors, leading to an increased cost in the decoloration of the product and limiting the industrialization of chemical recycling. In this work, eight types of ion-exchange resins were used for BHET decoloration, and resin D201 showed an outstanding performance not only in the decoloration efficiency but also in the retention rate of the product. Under the optimal conditions, the removal rate of the colorant and the retention efficiency of BHET were over 99% and 95%, respectively. D201 showed outstanding reusability with five successive cycles, and the decolored BHET and its r-PET showed good chromaticity. Furthermore, the investigations of adsorption isotherms, kinetics, and thermodynamics have been conducted, which indicated that the decoloration process was a natural endothermic reaction. Adsorption interactions between the colorant and resin were extensively examined by various characterizations, revealing that electrostatic force, pi-pi interactions, and hydrogen bonding were the dominant adsorption mechanisms. |
| WOS关键词 | ADSORPTION ; PET ; DYES ; PURIFICATION ; DECOLORATION ; DEGRADATION ; ORANGE ; WASTE |
| 资助项目 | National Key Research and Development Program of China[2019YFC1908204] ; National Natural Scientific Fund of China[21776289] ; National Natural Scientific Fund of China[21978291] ; National Natural Scientific Fund of China[21878292] ; National Natural Scientific Fund of China[21908232] ; Innovation Academy for Green Manufacture, Chinese Academy of Sciences[IAGM2020C21] ; Innovation Academy for Green Manufacture, Chinese Academy of Sciences[IAGM2020C12] ; K. C. Wong Education Foundation[GJTD-2018-04] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| 出版者 | AMER CHEMICAL SOC |
| WOS记录号 | WOS:000651520800056 |
| 资助机构 | National Key Research and Development Program of China ; National Natural Scientific Fund of China ; Innovation Academy for Green Manufacture, Chinese Academy of Sciences ; K. C. Wong Education Foundation |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/48995]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Lu, Xingmei; Zhou, Qing |
| 作者单位 | 1.Chinese Acad Sci, Innovat Acad Green Manufacture, Beijing 100190, Peoples R China 2.Chinese Acad Sci, Inst Proc Engn,State Key Lab Multiphase Complex S, Beijing Key Lab Ion Liquids Clean Proc, CAS Key Lab Green Proc & Engn, Beijing 100190, Peoples R China 3.Univ Chinese Acad Sci, Sch Chem & Engn, Beijing 100049, Peoples R China 4.Univ Chinese Acad Sci, Sino Danish Coll, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Huang, Rong,Zhang, Qi,Yao, Haoyu,et al. Ion-Exchange Resins for Efficient Removal of Colorants in Bis(hydroxyethyl) Terephthalate[J]. ACS OMEGA,2021,6(18):12351-12360. |
| APA | Huang, Rong,Zhang, Qi,Yao, Haoyu,Lu, Xingmei,Zhou, Qing,&Yan, Dongxia.(2021).Ion-Exchange Resins for Efficient Removal of Colorants in Bis(hydroxyethyl) Terephthalate.ACS OMEGA,6(18),12351-12360. |
| MLA | Huang, Rong,et al."Ion-Exchange Resins for Efficient Removal of Colorants in Bis(hydroxyethyl) Terephthalate".ACS OMEGA 6.18(2021):12351-12360. |
入库方式： OAI收割
来源：过程工程研究所
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