Fabrication of Ag3PO4/TiO2@molecular sieve (MS) ternary composites with remarkably enhanced visible light-responded photocatalytic activity and mechanism insight
文献类型：期刊论文
| 作者 | Bian, Zhenzhong1; Feng, Yali1; Li, Haoran2; Zhan, Jing1 |
| 刊名 | ENVIRONMENTAL RESEARCH
 |
| 出版日期 | 2020-11-01 |
| 卷号 | 190页码:12 |
| ISSN号 | 0013-9351 |
| 关键词 | Ag3PO4-TiO2 Molecular sieve Photocatalysis Formaldehyde Sodium isobutyl xanthate |
| DOI | 10.1016/j.envres.2020.109984 |
| 英文摘要 | In this study, Ag3PO4/TiO2@molecular sieve (MS) ternary composites were fabricated via in-situ deposition and hydrothermal growth method for photocatalytic degradation of formaldehyde and sodium isobutyl xanthate (SIBX) under visible light irradiation. XRD, PL, UV-vis, UPS, SEM-EDS and XPS techniques were adopted to characterize the composite. The results show that the MS material was indexed as zeolite P and Ag3PO4/TiO2 hybrid structure could improve the absorption of visible light and greatly inhibit the recombination of photogenerated charge carriers by introducing 3 times TiO2. After evaluating the photocatalytic activity and kinetics model, it is found that photocatalytic activity is consistent with the apparent first-order kinetic model. The Ag3PO4/TiO2-3@MS ternary composite under visible light irradiation appears the highest removal rate with 97.9% of formaldehyde and 96.7% of SIBX, respectively. Furthermore, the reusability of the photocatalyst was investigated by successive reuse. After five reuses, the removal rates reached 97.3% and 94.6% within 105 min for formaldehyde and SIBX, respectively. At last, the proposed mechanism of the photocatalytic reaction and the degradation mutes of formaldehyde and SIBX were systematically discussed. |
| WOS关键词 | GRAPHENE OXIDE ; EFFICIENT PHOTODEGRADATION ; AQUEOUS-SOLUTION ; METHYL-ORANGE ; COAL GANGUE ; AZO DYES ; DEGRADATION ; AG3PO4 ; TIO2 ; DECOMPOSITION |
| 资助项目 | China Ocean Mineral Resources RD Association[DY135-B2-15] ; Major Science and Technology Program for Water Pollution Control and Treatment[2015ZX07205-003] ; National Natural Science Foundation of China[21176242] ; National Natural Science Foundation of China[21176026] |
| WOS研究方向 | Environmental Sciences & Ecology ; Public, Environmental & Occupational Health |
| 语种 | 英语 |
| 出版者 | ACADEMIC PRESS INC ELSEVIER SCIENCE |
| WOS记录号 | WOS:000656320000003 |
| 资助机构 | China Ocean Mineral Resources RD Association ; Major Science and Technology Program for Water Pollution Control and Treatment ; National Natural Science Foundation of China |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/49145]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Feng, Yali |
| 作者单位 | 1.Univ Sci & Technol Beijing, Sch Civil & Resource Engn, Beijing 100083, Peoples R China 2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Bian, Zhenzhong,Feng, Yali,Li, Haoran,et al. Fabrication of Ag3PO4/TiO2@molecular sieve (MS) ternary composites with remarkably enhanced visible light-responded photocatalytic activity and mechanism insight[J]. ENVIRONMENTAL RESEARCH,2020,190:12. |
| APA | Bian, Zhenzhong,Feng, Yali,Li, Haoran,&Zhan, Jing.(2020).Fabrication of Ag3PO4/TiO2@molecular sieve (MS) ternary composites with remarkably enhanced visible light-responded photocatalytic activity and mechanism insight.ENVIRONMENTAL RESEARCH,190,12. |
| MLA | Bian, Zhenzhong,et al."Fabrication of Ag3PO4/TiO2@molecular sieve (MS) ternary composites with remarkably enhanced visible light-responded photocatalytic activity and mechanism insight".ENVIRONMENTAL RESEARCH 190(2020):12. |
入库方式： OAI收割
来源：过程工程研究所
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