中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
High performance organic solar cells enabled by an iodinated additive

文献类型:期刊论文

作者Yu, Qingqing2,3; Fu, Jiehao3; Chen, Haiyan3; Chen, Shanshan1; Hu, Dingqin3; Yang, Ke3; Kan, Zhipeng3; Sun, Kuan1; Lu, Shirong2,3; Xiao, Zeyun2,3
刊名ORGANIC ELECTRONICS
出版日期2021-06-01
卷号93页码:7
关键词Organic solar cells Additive engineering Morphology
ISSN号1566-1199
DOI10.1016/j.orgel.2021.106161
通讯作者Lu, Shirong(lushirong@cigit.ac.cn) ; Xiao, Zeyun(xiao.z@cigit.ac.cn)
英文摘要Additive engineering is a simple and effective strategy to enhance the efficiency of organic solar cells (OSCs). However, traditional additives such as 1,8-diiodooctane (DIO) or 1-chloronaphthalene (CN), suffer from inferior stability, concentration sensitivity, and need additional thermal treatments, which are not desirable for industrial application. Here we introduce a simple, effective and versatile solid additive 1,3-diiodobenzene (1,3-DIB) into the OSCs. In comparison to the control devices, the 1,3-DIB treated OSCs exhibit significantly improved performance with a power conversion efficiency (PCE) of 16.90% for polymer OSCs and a PCE of 14.35% for binary all-small-molecule OSCs. Mechanism studies reveal that 1,3-DIB can improve charge transport and extraction, decrease charge recombination, enhance crystallinity and improve the phase separation. Furthermore, no thermal annealing is needed in PM6:Y6 based OSCs and the 1,3-DIB treated devices show excellent stability and reproducibility in both polymer and small molecule OSCs. Our results demonstrated that additive engineering is a powerful method to enhance the OSC performance.
资助项目National Natural Science Foundation of China[22071238] ; National Natural Science Foundation of China[21801238] ; National Youth Thousand Program Project[R52A199Z11] ; CAS Pioneer Hundred Talents Program B[Y92A010Q10] ; Natural Science Foundation of Chongqing[cstc2018jcyjAX0556] ; Venture & Innovation Support Program for Chongqing Overseas Returnees[cx2019028] ; Chongqing Talents Top Youth Talent Program[CQYC201905057]
WOS研究方向Materials Science ; Physics
语种英语
WOS记录号WOS:000674507800007
出版者ELSEVIER
源URL[http://119.78.100.138/handle/2HOD01W0/13780]  
专题中国科学院重庆绿色智能技术研究院
通讯作者Lu, Shirong; Xiao, Zeyun
作者单位1.Chongqing Univ, Key Lab Low Grade Energy Utilizat Technol & Syst, Minist Educ, Sch Power Engn, Chongqing 400044, Peoples R China
2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
3.Chinese Acad Sci, Chongqing Inst Green & Intelligent Technol, Chongqing 400714, Peoples R China
推荐引用方式
GB/T 7714
Yu, Qingqing,Fu, Jiehao,Chen, Haiyan,et al. High performance organic solar cells enabled by an iodinated additive[J]. ORGANIC ELECTRONICS,2021,93:7.
APA Yu, Qingqing.,Fu, Jiehao.,Chen, Haiyan.,Chen, Shanshan.,Hu, Dingqin.,...&Xiao, Zeyun.(2021).High performance organic solar cells enabled by an iodinated additive.ORGANIC ELECTRONICS,93,7.
MLA Yu, Qingqing,et al."High performance organic solar cells enabled by an iodinated additive".ORGANIC ELECTRONICS 93(2021):7.

入库方式: OAI收割

来源:重庆绿色智能技术研究院

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