A bio-inspired nanocomposite membrane with improved light-trapping and salt-rejecting performance for solar-driven interfacial evaporation applications
文献类型:期刊论文
作者 | Ying, Peijin3; Ai, Bin1; Hu, Wei2; Geng, Yang3; Li, Ling4; Sun, Kuan3; Tan, Swee Ching5; Zhang, Wei6; Li, Meng3 |
刊名 | NANO ENERGY |
出版日期 | 2021-11-01 |
卷号 | 89页码:10 |
ISSN号 | 2211-2855 |
关键词 | Solar-driven interfacial evaporation Surface engineering Bio-inspired materials Light-trapping nanostructure Salt-rejecting nanostructure |
DOI | 10.1016/j.nanoen.2021.106443 |
通讯作者 | Li, Meng(limeng@cqu.edu.cn) |
英文摘要 | Solar-driven interfacial water evaporation is a rapid emerging technology to address the global water crisis. Efficient solar absorption as well as robust salt-rejecting performance are among the critical requirements of this technology. Here, we report a novel double-layered nanocomposite membrane with improved solar absorption capability while simultaneously achieving enhanced salt-rejecting performance for solar-driven interfacial evaporation applications, such as seawater purification. Two bio-inspired material engineering strategies are utilized: first, inspired by black butterfly wings, a top sublayer based on MXene nanostructures is utilized to reduce light reflection and thereby improve its photo-thermal efficiency. Secondly, inspired by the selective mass transport capability of plant root cells, a bottom sublayer based on reduced graphene oxide (rGO) nanosheets with similar characteristics is designed and fabricated. The narrowed interlayer spacing between adjacent rGO nanosheets is demonstrated to effectively transport water molecules while rejecting salt ions. Finally, the nanocomposite MXene@rGO membrane achieves an evaporation rate of 1.33 kg m- 2 h-1 and efficiency of 85.2% at 1 Sun. And the efficiency maintains 81.4% after 40 cycles of testing in seawater. In addition, simulations are performed to understand the light-trapping phenomenon for the MXene nanostructured surface. This bio-inspired work provides valuable insights for designing next-generation solar absorbers. |
资助项目 | Natural Science Foundation of China[52173235] ; Graduate Research and Innovation Foundation of Chongqing, China[CYS20012] ; Fundamental Research Funds for the Central Universities[2018CDQYDL0051] ; Fundamental Research Funds for the Central Universities[2019CDXYDL0007] ; Key Innovation Project for Clinical Technology of the Second Affiliated Hospital of Army Medical University[2018JSLC0025] |
WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
语种 | 英语 |
出版者 | ELSEVIER |
WOS记录号 | WOS:000703207800001 |
源URL | [http://119.78.100.138/handle/2HOD01W0/14155] |
专题 | 中国科学院重庆绿色智能技术研究院 |
通讯作者 | Li, Meng |
作者单位 | 1.Chongqing Univ, Sch Microelect & Commun Engn, Chongqing Key Lab Biopercept & Intelligent Inform, Chongqing 400044, Peoples R China 2.Chongqing Univ, Key Lab Optoelect Technol & Syst, Coll Optoelect Engn, Educ Minist China, Chongqing 400044, Peoples R China 3.Chongqing Univ, MOE Key Lab Low Grade Energy Utilizat Technol & S, CQU NUS Renewable Energy Mat & Devices Joint Lab, Sch Energy & Power Engn, Chongqing 400044, Peoples R China 4.Virginia Tech, Dept Mech Engn, Blacksburg, VA 24061 USA 5.Natl Univ Singapore, Dept Mat Sci & Engn, CQU NUS Renewable Energy Mat & Devices Joint Lab, Singapore 117573, Singapore 6.Chinese Acad Sci, Chongqing Inst Green & Intelligent Technol, Chongqing 400714, Peoples R China |
推荐引用方式 GB/T 7714 | Ying, Peijin,Ai, Bin,Hu, Wei,et al. A bio-inspired nanocomposite membrane with improved light-trapping and salt-rejecting performance for solar-driven interfacial evaporation applications[J]. NANO ENERGY,2021,89:10. |
APA | Ying, Peijin.,Ai, Bin.,Hu, Wei.,Geng, Yang.,Li, Ling.,...&Li, Meng.(2021).A bio-inspired nanocomposite membrane with improved light-trapping and salt-rejecting performance for solar-driven interfacial evaporation applications.NANO ENERGY,89,10. |
MLA | Ying, Peijin,et al."A bio-inspired nanocomposite membrane with improved light-trapping and salt-rejecting performance for solar-driven interfacial evaporation applications".NANO ENERGY 89(2021):10. |
入库方式: OAI收割
来源:重庆绿色智能技术研究院
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