Temperature Induced Dimensional Tuning and Anomalous Deformation of Micro/Nanopores
文献类型:期刊论文
作者 | Zhang, Shusong1; Ji, Zhenming1; Du, Guanghua2; Liu, Jie2; Zhou, Xi1; Xie, Yanbo1 |
刊名 | NANO LETTERS |
出版日期 | 2021-04-14 |
卷号 | 21期号:7页码:2766-2772 |
ISSN号 | 1530-6984 |
关键词 | Micro/nanopore thermal shrinkage ion track etching transportation phenomena nanofluidics |
DOI | 10.1021/acs.nanolett.0c04708 |
通讯作者 | Zhou, Xi(zhouxi@nwpu.edu.cn) ; Xie, Yanbo(ybxie@nwpu.edu.cn) |
英文摘要 | Artificial nanopores have become a common toolbox in nanotechnologies, with dimension and geometry as predominant factors. Most fabrication technologies determine the pore size beforehand, but few exist that enable size-tuning post-manufacturing. In this work, we reported a type of ion track etched micro/nanopores on uniaxially drawn PET foils that enable irreversible thermal shrinkage, thus tuning the pore dimensions by increasing ambient temperatures. Importantly, we found a complex pore deformation process, which for a specific range of pore sizes and temperatures resulted in a peculiar "eye"-shaped appearance of the pore openings. We analyzed the mechanical stresses and theoretically illustrated the complex deformation process by a phase diagram. Temperature-induced dimensional tuning nanopores reduced maximally over 98% of ionic conduction in a single nanopore and 99% of pressure-driven flow in a pore-array membrane within few seconds at 90 degrees C, which is useful for temperature-modulated mass transport in nanotechnology and energy applications. |
WOS关键词 | GLASS-TRANSITION TEMPERATURE ; ATOMIC LAYER DEPOSITION ; SURFACE-PROPERTIES ; NANOPORES ; FILMS ; MEMBRANES ; DYNAMICS |
资助项目 | National Natural Science Foundation of China[12075191] |
WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
语种 | 英语 |
出版者 | AMER CHEMICAL SOC |
WOS记录号 | WOS:000641160500009 |
资助机构 | National Natural Science Foundation of China |
源URL | [http://119.78.100.186/handle/113462/137571] |
专题 | 中国科学院近代物理研究所 |
通讯作者 | Zhou, Xi; Xie, Yanbo |
作者单位 | 1.Northwestern Polytech Univ, MOE Key Lab Mat Phys & Chem Extraordinary Condit, Xian 710072, Peoples R China 2.Chinese Acad Sci, Inst Modern Phys, Lanzhou 730000, Peoples R China |
推荐引用方式 GB/T 7714 | Zhang, Shusong,Ji, Zhenming,Du, Guanghua,et al. Temperature Induced Dimensional Tuning and Anomalous Deformation of Micro/Nanopores[J]. NANO LETTERS,2021,21(7):2766-2772. |
APA | Zhang, Shusong,Ji, Zhenming,Du, Guanghua,Liu, Jie,Zhou, Xi,&Xie, Yanbo.(2021).Temperature Induced Dimensional Tuning and Anomalous Deformation of Micro/Nanopores.NANO LETTERS,21(7),2766-2772. |
MLA | Zhang, Shusong,et al."Temperature Induced Dimensional Tuning and Anomalous Deformation of Micro/Nanopores".NANO LETTERS 21.7(2021):2766-2772. |
入库方式: OAI收割
来源:近代物理研究所
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