中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Temperature Induced Dimensional Tuning and Anomalous Deformation of Micro/Nanopores

文献类型:期刊论文

作者Zhang, Shusong1; Ji, Zhenming1; Du, Guanghua2; Liu, Jie2; Zhou, Xi1; Xie, Yanbo1
刊名NANO LETTERS
出版日期2021-04-14
卷号21期号:7页码:2766-2772
ISSN号1530-6984
关键词Micro/nanopore thermal shrinkage ion track etching transportation phenomena nanofluidics
DOI10.1021/acs.nanolett.0c04708
通讯作者Zhou, Xi(zhouxi@nwpu.edu.cn) ; Xie, Yanbo(ybxie@nwpu.edu.cn)
英文摘要Artificial nanopores have become a common toolbox in nanotechnologies, with dimension and geometry as predominant factors. Most fabrication technologies determine the pore size beforehand, but few exist that enable size-tuning post-manufacturing. In this work, we reported a type of ion track etched micro/nanopores on uniaxially drawn PET foils that enable irreversible thermal shrinkage, thus tuning the pore dimensions by increasing ambient temperatures. Importantly, we found a complex pore deformation process, which for a specific range of pore sizes and temperatures resulted in a peculiar "eye"-shaped appearance of the pore openings. We analyzed the mechanical stresses and theoretically illustrated the complex deformation process by a phase diagram. Temperature-induced dimensional tuning nanopores reduced maximally over 98% of ionic conduction in a single nanopore and 99% of pressure-driven flow in a pore-array membrane within few seconds at 90 degrees C, which is useful for temperature-modulated mass transport in nanotechnology and energy applications.
WOS关键词GLASS-TRANSITION TEMPERATURE ; ATOMIC LAYER DEPOSITION ; SURFACE-PROPERTIES ; NANOPORES ; FILMS ; MEMBRANES ; DYNAMICS
资助项目National Natural Science Foundation of China[12075191]
WOS研究方向Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics
语种英语
出版者AMER CHEMICAL SOC
WOS记录号WOS:000641160500009
资助机构National Natural Science Foundation of China
源URL[http://119.78.100.186/handle/113462/137571]  
专题中国科学院近代物理研究所
通讯作者Zhou, Xi; Xie, Yanbo
作者单位1.Northwestern Polytech Univ, MOE Key Lab Mat Phys & Chem Extraordinary Condit, Xian 710072, Peoples R China
2.Chinese Acad Sci, Inst Modern Phys, Lanzhou 730000, Peoples R China
推荐引用方式
GB/T 7714
Zhang, Shusong,Ji, Zhenming,Du, Guanghua,et al. Temperature Induced Dimensional Tuning and Anomalous Deformation of Micro/Nanopores[J]. NANO LETTERS,2021,21(7):2766-2772.
APA Zhang, Shusong,Ji, Zhenming,Du, Guanghua,Liu, Jie,Zhou, Xi,&Xie, Yanbo.(2021).Temperature Induced Dimensional Tuning and Anomalous Deformation of Micro/Nanopores.NANO LETTERS,21(7),2766-2772.
MLA Zhang, Shusong,et al."Temperature Induced Dimensional Tuning and Anomalous Deformation of Micro/Nanopores".NANO LETTERS 21.7(2021):2766-2772.

入库方式: OAI收割

来源:近代物理研究所

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