Bioinspired Dual-Responsive Nanofluidic Diodes by Poly-L-lysine Modification
文献类型：期刊论文
| 作者 | Li, Jun3; An, Pengrong3; Qin, Chuanguang3; Sun, Chun-Lin1; Sun, Miao3; Ji, Zhenming3; Wang, Chending3; Du, Guanghua2 ; Liu, Jie2; Xie, Yanbo3
|
| 刊名 | ACS OMEGA
 |
| 出版日期 | 2020-03-10 |
| 卷号 | 5期号:9页码:4501-4506 |
| ISSN号 | 2470-1343 |
| DOI | 10.1021/acsomega.9b03850 |
| 通讯作者 | Li, Jun(lij06lzu@nwpu.edu.cn) ; Qin, Chuanguang(qinchg@nwpu.edu.cn) ; Xie, Yanbo(ybxie@nwpu.edu.cn) |
| 英文摘要 | A smart nanofluidic device attracts attention as it enables to control the physicochemical properties and transportation phenomena, by using stimuli-responsive materials. This work reports a bioinspired modification of a conical ion track-etched polyethylene terephthalate nanopore surface by coating a layer of poly-L-lysine (PLL), which is a commonly used coating in biotechnology to achieve a dual-responsive nanofluidic channel by pH or temperature. The rectification of ionic transportation can be reversed by assembling PLL because of the change of surface bonds from the carboxyl to amine group. The PLL-modified nanopore becomes nonconductive as an "OFF" state at pH 11.5 and at a temperature of 70 degrees C in solution. The ionic transport in nanopores can be switched to the "ON" (conductive) state, by either decreasing pH or temperature. The transitions between "ON" and "OFF" states present excellent reversibility, which make the PLL-modified nanopores a promising smart nanofluidic device that can be used for drug delivery or biomimic ion/mass transport in future, besides the good biocompatibility and ease of use of PLL modification. |
| WOS关键词 | SOLID-STATE NANOPORES ; CURRENT RECTIFICATION ; SURFACE-CHEMISTRY ; PH ; NANOCHANNELS ; ADSORPTION ; TRANSPORT ; DRIVEN |
| 资助项目 | National Natural Science Foundation of China[NSFC 21602176] ; National Natural Science Foundation of China[21702085] ; National Natural Science Foundation of China[U1730133] ; National Natural Science Foundation of China[U1732143] ; National Natural Science Foundation of China[21572180] ; Natural Science Basic Research Plan in Shaanxi Province of China[2017JQ2039] ; Key Laboratory of Special Function Materials and Structure Design, Ministry of Education, Lanzhou University[lzujbky-2018-kb06] ; Fundamental Research Funds for the Central Universities[3102017jc01001] ; Fundamental Research Funds for the Central Universities[3102019ghxm020] ; Fundamental Research Funds for the Central Universities[3102019PB006] ; Analytics and Testing center in NPU |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000519806000015 |
| 出版者 | AMER CHEMICAL SOC |
| 资助机构 | National Natural Science Foundation of China ; Natural Science Basic Research Plan in Shaanxi Province of China ; Key Laboratory of Special Function Materials and Structure Design, Ministry of Education, Lanzhou University ; Fundamental Research Funds for the Central Universities ; Analytics and Testing center in NPU |
| 源URL | [http://119.78.100.186/handle/113462/140593]  |
| 专题 | 中国科学院近代物理研究所 |
| 通讯作者 | Li, Jun; Qin, Chuanguang; Xie, Yanbo |
| 作者单位 | 1.Lanzhou Univ, Coll Chem & Chem Engn, SKLAOC, Lanzhou 730000, Gansu, Peoples R China 2.Chinese Acad Sci, Inst Modern Phys, Lanzhou 730000, Gansu, Peoples R China 3.Northwestern Polytech Univ, Sch Nat & Appl Sci, Joint Lab Nanofluid & Inteifaces LONI, MOE Key Lab Mat Phys & Chem Extraordinary Condit, Xian 710072, Shaanxi, Peoples R China |
| 推荐引用方式 GB/T 7714 | Li, Jun,An, Pengrong,Qin, Chuanguang,et al. Bioinspired Dual-Responsive Nanofluidic Diodes by Poly-L-lysine Modification[J]. ACS OMEGA,2020,5(9):4501-4506. |
| APA | Li, Jun.,An, Pengrong.,Qin, Chuanguang.,Sun, Chun-Lin.,Sun, Miao.,...&Xie, Yanbo.(2020).Bioinspired Dual-Responsive Nanofluidic Diodes by Poly-L-lysine Modification.ACS OMEGA,5(9),4501-4506. |
| MLA | Li, Jun,et al."Bioinspired Dual-Responsive Nanofluidic Diodes by Poly-L-lysine Modification".ACS OMEGA 5.9(2020):4501-4506. |
入库方式： OAI收割
来源：近代物理研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。