Synchrotron x-ray spectroscopy investigation of the Ca(1-x)Ln(x)ZrTi(2-x)(Al, Fe)(x)O-7 zirconolite ceramics (Ln = La, Nd, Gd, Ho, Yb)
文献类型：期刊论文
| 作者 | Ji, Shiyin1,2,3; Su, Minhua4; Liao, Changzhong5,6; Ma, Shengshou6; Wang, Zhiguang2,3 ; Shih, Kaimin5; Chang, Chung-Kai7; Lee, Jyh-Fu7; Chan, Ting-Shan7; Li, Yuhong1
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| 刊名 | JOURNAL OF THE AMERICAN CERAMIC SOCIETY
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| 出版日期 | 2019-10-16 |
| 页码 | 13 |
| 关键词 | nuclear waste phase transformations x-ray methods zirconolite-2M |
| ISSN号 | 0002-7820 |
| DOI | 10.1111/jace.16832 |
| 通讯作者 | Liao, Changzhong(liaocz29@connect.hku.hk) ; Li, Yuhong(liyuhong@lzu.edu.cn) |
| 英文摘要 | When incorporating actinides into zirconolite for high-level radioactive waste immobilization, Al3+ and Fe3+ ions generally act as charge compensators. In this study, we rationally designed a series of Ca1-xLnxZrTi2-xmml:mfenced close=")" open="("separators=Al,FexO7 (Ln = La, Nd, Gd, Ho, Yb) to unravel the dopant solubility and evolutions of the crystalline phase and local environment of cations through synchrotron X-ray methods. It was found that single zirconolite phase is difficult to obtain and the fraction of perovskite have an increase with x from 0.1 to 0.9 in Ca1-xLaxZrTi2-x |
| WOS关键词 | HIGH-TEMPERATURE SYNTHESIS ; SELF-PROPAGATING SYNTHESIS ; LEVEL NUCLEAR-WASTE ; PHASE EVOLUTION ; SOLID-SOLUTION ; COORDINATION CHEMISTRY ; SILICATE-GLASSES ; METAL-OXIDES ; K-EDGE ; FE |
| 资助项目 | National Natural Science Foundations of China[41701560] ; National Natural Science Foundations of China[11775102] ; National Natural Science Foundations of China[11805088] ; Guangzhou Science and Technology Foundation of China[201804010197] ; Guangzhou Science and Technology Foundation of China[201704020200] ; Research Grants Council of Hong Kong ; Fundamental Research Funds for the Central Universities |
| WOS研究方向 | Materials Science |
| 语种 | 英语 |
| WOS记录号 | WOS:000490398400001 |
| 出版者 | WILEY |
| 资助机构 | National Natural Science Foundations of China ; Guangzhou Science and Technology Foundation of China ; Research Grants Council of Hong Kong ; Fundamental Research Funds for the Central Universities |
| 源URL | [http://119.78.100.186/handle/113462/141749]  |
| 专题 | 中国科学院近代物理研究所 |
| 通讯作者 | Liao, Changzhong; Li, Yuhong |
| 作者单位 | 1.Lanzhou Univ, Sch Nucl Sci & Technol, Lanzhou 730000, Gansu, Peoples R China 2.Chinese Acad Sci, Inst Modern Phys, Lanzhou, Gansu, Peoples R China 3.Univ Chinese Acad Sci, Sch Nucl Sci & Technol, Beijing, Peoples R China 4.Guangzhou Univ, Sch Environm Sci & Engn, Guangdong Prov Key Lab Radionuclides Pollut Contr, Guangzhou, Guangdong, Peoples R China 5.Univ Hong Kong, Dept Civil Engn, Hong Kong, Peoples R China 6.Guangdong Inst Ecoenvironm Sci & Technol, Guangdong Key Lab Integrated Agroenvironm Pollut, Guangzhou, Guangdong, Peoples R China 7.Natl Synchrotron Radiat Res Ctr, Hsinchu Sci Pk, Hsinchu, Taiwan |
| 推荐引用方式 GB/T 7714 | Ji, Shiyin,Su, Minhua,Liao, Changzhong,et al. Synchrotron x-ray spectroscopy investigation of the Ca(1-x)Ln(x)ZrTi(2-x)(Al, Fe)(x)O-7 zirconolite ceramics (Ln = La, Nd, Gd, Ho, Yb)[J]. JOURNAL OF THE AMERICAN CERAMIC SOCIETY,2019:13. |
| APA | Ji, Shiyin.,Su, Minhua.,Liao, Changzhong.,Ma, Shengshou.,Wang, Zhiguang.,...&Li, Yuhong.(2019).Synchrotron x-ray spectroscopy investigation of the Ca(1-x)Ln(x)ZrTi(2-x)(Al, Fe)(x)O-7 zirconolite ceramics (Ln = La, Nd, Gd, Ho, Yb).JOURNAL OF THE AMERICAN CERAMIC SOCIETY,13. |
| MLA | Ji, Shiyin,et al."Synchrotron x-ray spectroscopy investigation of the Ca(1-x)Ln(x)ZrTi(2-x)(Al, Fe)(x)O-7 zirconolite ceramics (Ln = La, Nd, Gd, Ho, Yb)".JOURNAL OF THE AMERICAN CERAMIC SOCIETY (2019):13. |
入库方式： OAI收割
来源：近代物理研究所
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