The contribution of coral-reef-derived dimethyl sulfide to aerosol burden over the Great Barrier Reef: a modelling study
文献类型：期刊论文
| 作者 | Fiddes, Sonya L.1,2,3,14; Woodhouse, Matthew T.3; Utembe, Steve4; Schofield, Robyn5; Alexander, Simon P.6; Alroe, Joel7; Chambers, Scott D.8; Chen, Zhenyi9 ; Cravigan, Luke7; Dunne, Erin3
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| 刊名 | ATMOSPHERIC CHEMISTRY AND PHYSICS
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| 出版日期 | 2022-02-22 |
| 卷号 | 22 |
| ISSN号 | 1680-7316 |
| DOI | 10.5194/acp-22-2419-2022 |
| 通讯作者 | Fiddes, Sonya L.(sonya.fiddes@utas.edu.au) |
| 英文摘要 | Coral reefs have been found to produce the sulfur compound dimethyl sulfide (DMS), a climatically relevant aerosol precursor predominantly associated with phytoplankton. Until recently, the role of coral-reef-derived DMS within the climate system had not been quantified. A study preceding the present work found that DMS produced by corals had negligible long-term climatic forcing at the global-regional scale. However, at sub-daily timescales more typically associated with aerosol and cloud formation, the influence of coral-reef-derived DMS on local aerosol radiative effects remains unquantified. The Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) has been used in this work to study the role of coral-reef-derived DMS at sub-daily timescales for the first time. WRF-Chem was run to coincide with an October 2016 field campaign over the Great Barrier Reef, Queensland, Australia, against which the model was evaluated. After updating and scaling the DMS surface water climatology, the model reproduced DMS and sulfur concentrations well. The inclusion of coral-reef-derived DMS resulted in no significant change in sulfate aerosol mass or total aerosol number. Subsequently, no direct or indirect aerosol effects were detected. The results suggest that the co-location of the Great Barrier Reef with significant anthropogenic aerosol sources along the Queensland coast prevents coral-reef-derived aerosol from having a modulating influence on local aerosol burdens in the current climate. |
| WOS关键词 | MASS-SPECTROMETER ; BOUNDARY-LAYER ; AIR-QUALITY ; ATMOSPHERIC DIMETHYLSULFIDE ; MARINE STRATOCUMULUS ; CLOUD MICROPHYSICS ; PARTICLE FORMATION ; SOUTHEAST PACIFIC ; GLOBAL-MODEL ; VOCALS-REX |
| 资助项目 | Australian Research Council[DP150101649] ; Australian Research Council[CE170100023] ; Australian Research Council[CE110001028] ; Australian Research Council[15H01732] ; Australian Research Council[17KK0016] ; Ministry of Education, Culture, Sports, Science and Technology, Japan |
| WOS研究方向 | Environmental Sciences & Ecology ; Meteorology & Atmospheric Sciences |
| 语种 | 英语 |
| 出版者 | COPERNICUS GESELLSCHAFT MBH |
| WOS记录号 | WOS:000760857500001 |
| 资助机构 | Australian Research Council ; Ministry of Education, Culture, Sports, Science and Technology, Japan |
| 源URL | [http://ir.hfcas.ac.cn:8080/handle/334002/127921]  |
| 专题 | 中国科学院合肥物质科学研究院 |
| 通讯作者 | Fiddes, Sonya L. |
| 作者单位 | 1.Univ Melbourne, ARC Ctr Excellence Climate Syst Sci, Melbourne, Vic, Australia 2.Univ Melbourne, Australian German Climate & Energy Coll, Melbourne, Vic, Australia 3.CSIRO, Climate Sci Ctr, Oceans & Atmosphere, Aspendale, Vic, Australia 4.Environm Protect Author Victoria, Macleod, Australia 5.Univ Melbourne, ARC Ctr Excellence Climate Extremes, Melbourne, Vic, Australia 6.Australian Antarctic Div, Hobart, Tas, Australia 7.Queensland Univ Technol, Sch Earth & Atmospher Sci, Int Lab Air Qual & Hlth, Brisbane, Qld, Australia 8.Australian Nucl Sci & Technol Org, Lucas Heights, NSW, Australia 9.Chinese Acad Sci, Anhui Inst Opt & Fine Mech, Key Lab Environm Opt & Technol, Hefei 230031, Peoples R China 10.Univ Tsukuba, Fac Life & Environm Sci, Tsukuba, Ibaraki, Japan |
| 推荐引用方式 GB/T 7714 | Fiddes, Sonya L.,Woodhouse, Matthew T.,Utembe, Steve,et al. The contribution of coral-reef-derived dimethyl sulfide to aerosol burden over the Great Barrier Reef: a modelling study[J]. ATMOSPHERIC CHEMISTRY AND PHYSICS,2022,22. |
| APA | Fiddes, Sonya L..,Woodhouse, Matthew T..,Utembe, Steve.,Schofield, Robyn.,Alexander, Simon P..,...&Williams, Alastair G..(2022).The contribution of coral-reef-derived dimethyl sulfide to aerosol burden over the Great Barrier Reef: a modelling study.ATMOSPHERIC CHEMISTRY AND PHYSICS,22. |
| MLA | Fiddes, Sonya L.,et al."The contribution of coral-reef-derived dimethyl sulfide to aerosol burden over the Great Barrier Reef: a modelling study".ATMOSPHERIC CHEMISTRY AND PHYSICS 22(2022). |
入库方式： OAI收割
来源：合肥物质科学研究院
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