中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Critical Behavior in the Fe-Based Antiperovskite Compound AlC1.1Fe3

文献类型:期刊论文

作者Qian, Licai2; Liu, Xiansong2; Dai, Zhenxiang2; Feng, Shuangjiu2; Lv, Qingrong2; Lin, Shuai1; Kan, Xucai2
刊名JOURNAL OF SUPERCONDUCTIVITY AND NOVEL MAGNETISM
出版日期2022-04-21
关键词Antiperovskite Critical exponent Critical behavior Long-range ferromagnetic coupling Exchange interaction
ISSN号1557-1939
DOI10.1007/s10948-022-06205-9
通讯作者Lin, Shuai(linshuai17@issp.ac.cn) ; Kan, Xucai(kanxucai@ahu.edu.cn)
英文摘要In this study, the critical behavior of the Fe-based carbide antiperovskite compound AlC1.1Fe3 has been presented. There is a second-order phase transition and the magnetic state will change from ferromagnetic state to paramagnetic state near Curie temperature. Critical exponents (beta, gamma, delta) representing different significance of magnetism are obtained by separate classical methods, which are exceedingly agreeable with the mean-field model theory, indicating that magnetic behavior of AlC1.1Fe3 is dominated by long-range ferromagnetic coupling. According to the scaling equation m = f +/- (h), the experimental data obtained by the two experimental methods roughly overlap on the two curves, which demonstrates the reliability of these fitting parameters, and the convergence of the parameters also conforms to the mean-field model. Besides, the mutual exchange distance J(r) decreases as r(-4.695) due to the competitive Fe-Fe metal bond and Fe-C covalent bond. We suggest that the competition between the localized metal bond magnetic interaction and itinerant covalent bond hybridization should be responsible for the critical behavior of AlC1.1Fe3.
WOS关键词TRANSPORT-PROPERTIES ; PEROVSKITE ; NICKEL ; STATE ; 1ST
资助项目National Natural Science Foundation of China[51872004] ; Open fund for Discipline Construction, Institutes of Physical Science and Information Technology, Education Department of Anhui Province[KJ2019ZD03] ; Key Program of the Science and Technology Department of Anhui Province[201904a05020038]
WOS研究方向Physics
语种英语
WOS记录号WOS:000784628800001
出版者SPRINGER
资助机构National Natural Science Foundation of China ; Open fund for Discipline Construction, Institutes of Physical Science and Information Technology, Education Department of Anhui Province ; Key Program of the Science and Technology Department of Anhui Province
源URL[http://ir.hfcas.ac.cn:8080/handle/334002/128533]  
专题中国科学院合肥物质科学研究院
通讯作者Lin, Shuai; Kan, Xucai
作者单位1.Inst Solid State Phys, Key Lab Mat Phys, Hefei 230031, Peoples R China
2.Anhui Univ, Engn Technol Res Ctr Magnet Mat, Sch Mat Sci & Engn, Hefei 230601, Peoples R China
推荐引用方式
GB/T 7714
Qian, Licai,Liu, Xiansong,Dai, Zhenxiang,et al. Critical Behavior in the Fe-Based Antiperovskite Compound AlC1.1Fe3[J]. JOURNAL OF SUPERCONDUCTIVITY AND NOVEL MAGNETISM,2022.
APA Qian, Licai.,Liu, Xiansong.,Dai, Zhenxiang.,Feng, Shuangjiu.,Lv, Qingrong.,...&Kan, Xucai.(2022).Critical Behavior in the Fe-Based Antiperovskite Compound AlC1.1Fe3.JOURNAL OF SUPERCONDUCTIVITY AND NOVEL MAGNETISM.
MLA Qian, Licai,et al."Critical Behavior in the Fe-Based Antiperovskite Compound AlC1.1Fe3".JOURNAL OF SUPERCONDUCTIVITY AND NOVEL MAGNETISM (2022).

入库方式: OAI收割

来源:合肥物质科学研究院

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