中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
Study on the Pore Structure and Fractal Characteristics of Different Lithofacies of Wufeng-Longmaxi Formation Shale in Southern Sichuan Basin, China

文献类型:期刊论文

作者Qian, Chao4,5; Li, Xizhe5; Shen, Weijun1,4; Zhang, Qing3; Guo, Wei5; Hu, Yong5; Cui, Yue2; Jia, Yuze2; Shen WJ(沈伟军)
刊名ACS OMEGA
出版日期2022-03-15
卷号7期号:10页码:8724-8738
ISSN号2470-1343
DOI10.1021/acsomega.1c06913
通讯作者Li, Xizhe(lixz69@petrochina.com.cn) ; Shen, Weijun(wishen763@imech.ac.cn)
英文摘要Gas content and flow characteristics are closely related to shale lithofacies, and significant differences exist in the pore structure and fractal characteristics among lithofacies. In this study, X-ray diffractometer (XRD), field-emission scanning electron microscopy (FE-SEM), gas adsorption (N-2 and CO2), and fractal theory were employed to systematically characterize the pore attributes of the marine Wufeng-Longmaxi formation shales. The information of various pores and microfractures among lithofacies was extracted and quantified via high-resolution FE-SEM image stitching technology. Shales were classified into four types based on mineral compositions, and siliceous shales possess the largest SEM-based surface porosity (2.84%) and the largest pore volume (PV) (average 0.0243 cm(3)/g) as well as specific surface area (SSA) (average 28.06 m(2)/g). The effect of lithofacies variation on the PV of shale is minor. In contrast, the lithofacies variation has a significant impact on the SSA, and the SSA of siliceous shale is 39.11% higher than that of argillaceous shale. PV and SSA show strong positive correlation with the total organic carbon (TOC) content but negative correlation with clay minerals. Siliceous shales have the greatest fractal dimension D1 (pore surface roughness) (average 2.6821), which is contributed by abundant organic matter pores with more complicated boundaries. The largest fractal dimension D2 (pore structure complexity) (average 2.8263) is found in mixed shales, which is attributed to well-developed intraparticle (intraP) pores associated with carbonate mineral dissolution. This indicates that siliceous shales have the highest methane adsorption capacity and that shale gas desorption, diffusion, and seepage are more difficult in mixed shales.
WOS关键词GAS-ADSORPTION ; FE-SEM ; JIAOSHIBA AREA ; N-2 ADSORPTION ; MARINE SHALE ; SCALE PORES ; BARNETT ; STORAGE ; CLASSIFICATION ; RESERVOIRS
资助项目National Natural Science Foundation of China[11802312] ; National Natural Science Foundation of China[U1762216] ; National Natural Science Foundation of China[11802313]
WOS研究方向Chemistry
语种英语
WOS记录号WOS:000783601100049
资助机构National Natural Science Foundation of China
源URL[http://dspace.imech.ac.cn/handle/311007/89033]  
专题力学研究所_流固耦合系统力学重点实验室(2012-)
通讯作者Li, Xizhe; Shen, Weijun
作者单位1.Univ Chinese Acad Sci, Sch Engn Sci, Beijing 100049, Peoples R China
2.Chinese Acad Sci, Inst Porous Flow & Fluid Mech, Langfang 065007, Hebei, Peoples R China
3.CNPC Chuanqing Drilling Engn Co Ltd, Shale Gas Explorat & Dev Dept, Chengdu 610051, Sichuan, Peoples R China
4.Chinese Acad Sci, Inst Mech, Key Lab Mech Fluid Solid Coupling Syst, Beijing 100190, Peoples R China
5.PetroChina, Res Inst Petr Explorat & Dev, Beijing 100083, Peoples R China
推荐引用方式
GB/T 7714
Qian, Chao,Li, Xizhe,Shen, Weijun,et al. Study on the Pore Structure and Fractal Characteristics of Different Lithofacies of Wufeng-Longmaxi Formation Shale in Southern Sichuan Basin, China[J]. ACS OMEGA,2022,7(10):8724-8738.
APA Qian, Chao.,Li, Xizhe.,Shen, Weijun.,Zhang, Qing.,Guo, Wei.,...&沈伟军.(2022).Study on the Pore Structure and Fractal Characteristics of Different Lithofacies of Wufeng-Longmaxi Formation Shale in Southern Sichuan Basin, China.ACS OMEGA,7(10),8724-8738.
MLA Qian, Chao,et al."Study on the Pore Structure and Fractal Characteristics of Different Lithofacies of Wufeng-Longmaxi Formation Shale in Southern Sichuan Basin, China".ACS OMEGA 7.10(2022):8724-8738.

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来源:力学研究所

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