Co-pyrolysis of corn stover with industrial coal ash for in situ efficient remediation of heavy metals in multi-polluted soil
文献类型：期刊论文
| 作者 | Xia, Yu1,2,3; Li, Yi4; Sun, Yuting5; Miao, Wei3; Liu, Zhengang1,2 |
| 刊名 | ENVIRONMENTAL POLLUTION
 |
| 出版日期 | 2021-11-15 |
| 卷号 | 289页码:8 |
| 关键词 | Coal ash Waste biomass Polluted soil Soil remediation Paddy rice |
| ISSN号 | 0269-7491 |
| DOI | 10.1016/j.envpol.2021.117840 |
| 英文摘要 | Coal ash incorporated biochar (CA/BC) composite was prepared by co-pyrolysis of agricultural residue and in-dustrial coal ash and applied for remediation of soils polluted by lead (Pb) and cadmium (Cd). The results showed that immobilization efficiency of CA/BC for heavy metals (HMs) was significantly enhanced by 77.1 % (Pb) and 42.7 % (Cd) compared to pristine biochar (BC), and this was mainly due to the increased pH value, surface functionality and surface negative charge. By the introduction of 5 % CA/BC, the polluted soils showed the highest reduction of leaching toxicity by 67.9 % (Pb) and 49.7 % (Cd), respectively. The chemical speciation of Pb and Cd in soils was changed remarkably and the reduced bioavailable Pb and Cd were mainly transformed from acid-soluble fraction into the most stable form of residual fraction. The mechanism study showed that surface precipitation, complexation, cation exchange and cation-pi interaction of CA/BC mainly contributed to heavy metals (HMs) immobilization. The pot experiments further confirmed that incorporation of 5 % CA/BC effectively reduced plant Pb and Cd accumulation by 81 % and 62.5 % respectively, and significantly promoted the plant growth of paddy rice by 3.1, 2.2 and 2.0 times in terms of root, stem length and dry mass parameters. The present study offered a cost-effective and green method to prepare soil amendment with great potential for remediation of soils polluted by HMs and realized the value-added utilization of waste agricultural residue and industrial coal ash. |
| WOS关键词 | FLY-ASH ; CONTAMINATED SOILS ; RELATIVE DISTRIBUTION ; SORPTION MECHANISMS ; AQUEOUS-SOLUTION ; BIOCHAR ; CADMIUM ; BIOAVAILABILITY ; REMOVAL ; IMMOBILIZATION |
| 资助项目 | Key Research Program of Chinese Academy of Science[ZDRW-ZS-2018-1-3] |
| WOS研究方向 | Environmental Sciences & Ecology |
| 语种 | 英语 |
| WOS记录号 | WOS:000696803700002 |
| 出版者 | ELSEVIER SCI LTD |
| 资助机构 | Key Research Program of Chinese Academy of Science |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/50184]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Liu, Zhengang |
| 作者单位 | 1.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, Dept Solid Waste Treatment & Recycling, Beijing 100085, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.China Urban Construct Design & Res Inst Co Ltd, Beijing 100120, Peoples R China 4.Chinese Acad Sci, Inst Proc Engn IPE, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China 5.Beijing Univ Chem Technol, Coll Life Sci & Technol, Beijing 100029, Peoples R China |
| 推荐引用方式 GB/T 7714 | Xia, Yu,Li, Yi,Sun, Yuting,et al. Co-pyrolysis of corn stover with industrial coal ash for in situ efficient remediation of heavy metals in multi-polluted soil[J]. ENVIRONMENTAL POLLUTION,2021,289:8. |
| APA | Xia, Yu,Li, Yi,Sun, Yuting,Miao, Wei,&Liu, Zhengang.(2021).Co-pyrolysis of corn stover with industrial coal ash for in situ efficient remediation of heavy metals in multi-polluted soil.ENVIRONMENTAL POLLUTION,289,8. |
| MLA | Xia, Yu,et al."Co-pyrolysis of corn stover with industrial coal ash for in situ efficient remediation of heavy metals in multi-polluted soil".ENVIRONMENTAL POLLUTION 289(2021):8. |
入库方式： OAI收割
来源：过程工程研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。