Recovery and reuse of floc sludge for high-performance capacitors
文献类型：期刊论文
| 作者 | Zhang, Di1,2; Hou, Rong1; Wang, Wenbo1,2; Zhao, He1 |
| 刊名 | FRONTIERS OF ENVIRONMENTAL SCIENCE & ENGINEERING
 |
| 出版日期 | 2022-06-01 |
| 卷号 | 16期号:6页码:12 |
| 关键词 | Floc sludge Porous carbon electrode Energy storage performance Supercapacitors |
| ISSN号 | 2095-2201 |
| DOI | 10.1007/s11783-021-1512-5 |
| 英文摘要 | In this paper, floc sludge was transformed into porous carbon matrix composites by acidification and KOH activation at high temperature and used as an electrode material for application in capacitors. The effects of different treatment processes on the electrochemical properties of sludge materials were compared. The results of electrochemical tests showed that the sludge electrode exhibited excellent energy storage performance after HNO3 acidification and KOH activation with a mass ratio of 3:1 (KOH/C). The specific capacitance of the sludge electrode reached 287 F/g at a current density of 1 A/g. In addition, the sludge electrode material showed excellent cycle stability (specific capacity retained at 93.4% after 5000 cycles at 5 A/g). Based on XRD, FTIR, SEM, TEM, and BET surface analysis, the morphology of sludge electrode materials can be effectively regulated by chemical pretreatment. The best-performing material showed a 3D porous morphology with a large specific surface area (2588 m(2)/g) and optimal pore size distribution, improving ion channels and charge conductivity. According to the life cycle assessment of floc sludge utilization, it reduced the resource consumption and toxicity risk by more than 90% compared with ordinary sludge disposal processes. This work provided a cost-effective and eco-friendly sludge reuse method and demonstrated the application potential of sludge-based materials in high-performance supercapacitors. (c) Higher Education Press 2021 |
| WOS关键词 | HIERARCHICAL POROUS CARBON ; SEWAGE-SLUDGE ; WASTE ; ACTIVATION ; REMOVAL |
| 资助项目 | National Natural Science Foundation of China[51978643] ; Youth Innovation Promotion Association, CAS[2014037] |
| WOS研究方向 | Engineering ; Environmental Sciences & Ecology |
| 语种 | 英语 |
| WOS记录号 | WOS:000708874900002 |
| 出版者 | HIGHER EDUCATION PRESS |
| 资助机构 | National Natural Science Foundation of China ; Youth Innovation Promotion Association, CAS |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/50597]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Zhao, He |
| 作者单位 | 1.Chinese Acad Sci, Beijing Engn Res Ctr Proc Pollut Control, Inst Proc Engn, CAS Key Lab Green Proc & Engn, Beijing 100190, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhang, Di,Hou, Rong,Wang, Wenbo,et al. Recovery and reuse of floc sludge for high-performance capacitors[J]. FRONTIERS OF ENVIRONMENTAL SCIENCE & ENGINEERING,2022,16(6):12. |
| APA | Zhang, Di,Hou, Rong,Wang, Wenbo,&Zhao, He.(2022).Recovery and reuse of floc sludge for high-performance capacitors.FRONTIERS OF ENVIRONMENTAL SCIENCE & ENGINEERING,16(6),12. |
| MLA | Zhang, Di,et al."Recovery and reuse of floc sludge for high-performance capacitors".FRONTIERS OF ENVIRONMENTAL SCIENCE & ENGINEERING 16.6(2022):12. |
入库方式： OAI收割
来源：过程工程研究所
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