Zinc-based deep eutectic solvent - An efficient carbonic anhydrase mimic for CO2 hydration and conversion
文献类型：期刊论文
| 作者 | Zhang, Zhibo2; Li, Fangfang2; Nie, Yi1,3; Zhang, Xiangping3; Zhang, Suojiang3; Ji, Xiaoyan2 |
| 刊名 | SEPARATION AND PURIFICATION TECHNOLOGY
 |
| 出版日期 | 2021-12-01 |
| 卷号 | 276页码:7 |
| 关键词 | Enzyme mimic Carbon anhydrase DES Carbon dioxide Hydration |
| ISSN号 | 1383-5866 |
| DOI | 10.1016/j.seppur.2021.119446 |
| 英文摘要 | Carbonic anhydrase (CA) has demonstrated great potential to mitigate CO2 emissions by enzymatic conversion of CO2, while its commercial implementation is limited by the inherent shortcomings of CA, such as thermal and chemical instability, high sensitivity to the environment, and high cost. To overcome the drawbacks of CA and develop advanced technologies for mitigating CO2 emission, for the first time, mimetic CA (ZnHisGly) with the characteristics of natural CA was designed and synthesized, i.e., zinc-based deep eutectic solvent (DES), to boost CO2 hydration and conversion. The mimetic CA exhibited facile synthesis, high stability, and low cost as the characteristics of DES, and showed better catalytic performance compared to the currently reported mimetic CA. Particularly, its catalytic performance increased greatly with increasing pH and temperatures, which provides promising prospects in the industrial applications of DES-based CA mimics. |
| WOS关键词 | IMMOBILIZATION ; SEQUESTRATION ; PURIFICATION ; CATALYSTS ; DIOXIDE |
| 资助项目 | Kempe foundation in Sweden ; Swedish Energy Agency[P47500-1] |
| WOS研究方向 | Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:000706301300044 |
| 出版者 | ELSEVIER |
| 资助机构 | Kempe foundation in Sweden ; Swedish Energy Agency |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/50634]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Zhang, Zhibo; Ji, Xiaoyan |
| 作者单位 | 1.Zhengzhou Inst Emerging Ind Technol, Zhengzhou 450000, Henan, Peoples R China 2.Lulea Univ Technol, Div Energy Sci, Energy Engn, S-97187 Lulea, Sweden 3.Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, Inst Proc Engn, State Key Lab Multiphase Complex Syst,CAS Key Lab, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Zhang, Zhibo,Li, Fangfang,Nie, Yi,et al. Zinc-based deep eutectic solvent - An efficient carbonic anhydrase mimic for CO2 hydration and conversion[J]. SEPARATION AND PURIFICATION TECHNOLOGY,2021,276:7. |
| APA | Zhang, Zhibo,Li, Fangfang,Nie, Yi,Zhang, Xiangping,Zhang, Suojiang,&Ji, Xiaoyan.(2021).Zinc-based deep eutectic solvent - An efficient carbonic anhydrase mimic for CO2 hydration and conversion.SEPARATION AND PURIFICATION TECHNOLOGY,276,7. |
| MLA | Zhang, Zhibo,et al."Zinc-based deep eutectic solvent - An efficient carbonic anhydrase mimic for CO2 hydration and conversion".SEPARATION AND PURIFICATION TECHNOLOGY 276(2021):7. |
入库方式： OAI收割
来源：过程工程研究所
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