Mesoporous silica nanosheets with well-dispersed small Ag nanoparticles for the construction of robust transparent antibacterial nanocoatings
文献类型：期刊论文
| 作者 | Wang, Xuan1; Wang, Yulu1; Li, Xiaoyu2; Du, Xin1 |
| 刊名 | MICROPOROUS AND MESOPOROUS MATERIALS
 |
| 出版日期 | 2021-12-01 |
| 卷号 | 328页码:10 |
| ISSN号 | 1387-1811 |
| 关键词 | Mesoporous silica nanosheets Ag nanoparticles Antibacterial activity Mechanical robustness High transparence |
| DOI | 10.1016/j.micromeso.2021.111476 |
| 英文摘要 | The fabrication of robust transparent antibacterial nanocoatings on the surface of device and equipment has significant implication for protecting human from bacterial infections in daily life. However, it still faces some challenges such as low antibacterial efficiency and poor mechanical stability, which hinder their wide applications. Therefore, it is urgent to explore the design and fabrication of superior antibacterial nanocoatings with high-robustness. In this work, robust transparent antibacterial nanocoatings were successfully fabricated by employing two-dimensional mesoporous nanosheets as a novel building block. Aminopropyl-modified mesoporous silica nanosheets (MSNSs-NH2) with uniform pore sizes of ca. 5-8 nm were first fabricated by one-pot liquid-liquid interface growth method, and were employed as a carrier to achieve well-dispersed loading of many small Ag nanoparticles (NPs) of ca. 2-4 nm to form MSNSs-NH2@Ag as antibacterial agent. Next, robust transparent antibacterial nanocoatings were prepared by simple dip-coating method without any postprocessing. It is worth noting that the use of two-dimensional MSNSs-NH2 with large spreading area not only facilitates the uniform loading of small Ag NPs for high antibacterial capacity of nanocoatings, but also is beneficial to enhance the mechanical robustness of nanocoatings due to the firm spreadability of single layer mesoporous nanosheets on the flat substrates. The optimal coated glass slide exhibits the enhanced transmittance (94.2% at 535 nm), high-mechanical robustness (pencil hardness test: >3H, tape adhesion test: >4B) and excellent antibacterial activity (at least killing 80% bacteria) toward Gram-negative Escherichia coli. This work may provide an exploration strategy to construct multifunctional nanocoatings by using the novel mesoporous nanosheets as a building block. |
| WOS关键词 | CORE-SHELL NANOPARTICLES ; SILVER NANOPARTICLES ; SURFACES ; COATINGS ; PARTICLES ; FILMS ; ION |
| WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science |
| 语种 | 英语 |
| 出版者 | ELSEVIER |
| WOS记录号 | WOS:000709958600001 |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/50734]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Li, Xiaoyu; Du, Xin |
| 作者单位 | 1.Univ Sci & Technol Beijing, Dept Chem & Biol Engn, Beijing Key Lab Bioengn & Sensing Technol, Beijing 100083, Peoples R China 2.Chinese Acad Sci, Inst Proc Engn, Natl Engn Lab Hydromet Cleaner Prod Technol, Key Lab Green Proc & Engn, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Wang, Xuan,Wang, Yulu,Li, Xiaoyu,et al. Mesoporous silica nanosheets with well-dispersed small Ag nanoparticles for the construction of robust transparent antibacterial nanocoatings[J]. MICROPOROUS AND MESOPOROUS MATERIALS,2021,328:10. |
| APA | Wang, Xuan,Wang, Yulu,Li, Xiaoyu,&Du, Xin.(2021).Mesoporous silica nanosheets with well-dispersed small Ag nanoparticles for the construction of robust transparent antibacterial nanocoatings.MICROPOROUS AND MESOPOROUS MATERIALS,328,10. |
| MLA | Wang, Xuan,et al."Mesoporous silica nanosheets with well-dispersed small Ag nanoparticles for the construction of robust transparent antibacterial nanocoatings".MICROPOROUS AND MESOPOROUS MATERIALS 328(2021):10. |
入库方式： OAI收割
来源：过程工程研究所
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