Enzyme-photo-coupled catalytic systems
文献类型：期刊论文
| 作者 | Zhang, Shaohua3,6; Liu, Shusong2; Sun, Yiying3; Li, Shihao3; Shi, Jiafu1,2,5; Jiang, Zhongyi3,4,5 |
| 刊名 | CHEMICAL SOCIETY REVIEWS
 |
| 出版日期 | 2021-11-04 |
| 页码 | 18 |
| ISSN号 | 0306-0012 |
| DOI | 10.1039/d1cs00392e |
| 英文摘要 | Efficient chemical transformation in a green, low-carbon way is crucial for the sustainable development of modern society. Enzyme-photo-coupled catalytic systems (EPCS) that integrate the exceptional selectivity of enzyme catalysis and the unique reactivity of photocatalysis hold great promise in solar-driven 'molecular editing'. However, the involvement of multiple components and catalytic processes challenged the design of efficient and stable EPCS. To show a clear picture of the complex catalytic system, in this review, we analyze EPCS from the perspective of system engineering. First, we disintegrate the complex system into four elementary components, and reorganize these components into biocatalytic and photocatalytic ensembles (BE and PE). By resolving current accessible systems, we identify that connectivity and compatibility between BE and PE are two crucial factors that govern the performance of EPCS. Then, we discuss the origin of undesirable connectivity and low compatibility, and deduce the possible solutions. Based on these understandings, we propose the designing principles of EPCS. Lastly, we provide a future perspective of EPCS. |
| WOS关键词 | CARBON-DIOXIDE ; REDUCTION ; OXIDATION ; CO2 |
| 资助项目 | National Key Research and Development Program of China[2020YFA0907902] ; National Natural Science Funds of China[21776213] ; National Natural Science Funds of China[21621004] ; Natural Science Fund of Tianjin[19JCYBJC19700] ; Open Funding Project of the State Key Laboratory of Biochemical Engineering[2020KF-06] ; Tianjin Synthetic Biotechnology Innovation Capacity Improvement Project[TSBICIP-KJGG-003] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| 出版者 | ROYAL SOC CHEMISTRY |
| WOS记录号 | WOS:000714412200001 |
| 资助机构 | National Key Research and Development Program of China ; National Natural Science Funds of China ; Natural Science Fund of Tianjin ; Open Funding Project of the State Key Laboratory of Biochemical Engineering ; Tianjin Synthetic Biotechnology Innovation Capacity Improvement Project |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/50887]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Shi, Jiafu; Jiang, Zhongyi |
| 作者单位 | 1.Chinese Acad Sci, State Key Lab Biochem Engn, Inst Proc Engn, Beijing 10090, Peoples R China 2.Tianjin Univ, Sch Environm Sci & Engn, Tianjin 300072, Peoples R China 3.Tianjin Univ, Sch Chem Engn & Technol, Key Lab Green Chem Technol, Minist Educ, Tianjin 300072, Peoples R China 4.Collaborat Innovat Ctr Chem Sci & Engn Tianjin, Tianjin 300072, Peoples R China 5.Tianjin Univ, Joint Sch Natl Univ Singapore & Tianjin Univ, Int Campus, Fuzhou 350207, Peoples R China 6.Radboud Univ Nijmegen, Inst Mol & Mat, Nijmegen, Netherlands |
| 推荐引用方式 GB/T 7714 | Zhang, Shaohua,Liu, Shusong,Sun, Yiying,et al. Enzyme-photo-coupled catalytic systems[J]. CHEMICAL SOCIETY REVIEWS,2021:18. |
| APA | Zhang, Shaohua,Liu, Shusong,Sun, Yiying,Li, Shihao,Shi, Jiafu,&Jiang, Zhongyi.(2021).Enzyme-photo-coupled catalytic systems.CHEMICAL SOCIETY REVIEWS,18. |
| MLA | Zhang, Shaohua,et al."Enzyme-photo-coupled catalytic systems".CHEMICAL SOCIETY REVIEWS (2021):18. |
入库方式： OAI收割
来源：过程工程研究所
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