Ce-Modified Mo/gamma-Al2O3 Catalysts for Production of Elemental Sulfur through Reducing SO2
文献类型：期刊论文
| 作者 | Yang, Yiqian1,3; Peng, Zhijian1; Zhao, Hui3; Wang, Emiang2; Li, Chunshan3 |
| 刊名 | INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH
 |
| 出版日期 | 2021-11-10 |
| 卷号 | 60期号:44页码:15942-15950 |
| ISSN号 | 0888-5885 |
| DOI | 10.1021/acs.iecr.1c01976 |
| 英文摘要 | A series of metal-modified Mo/gamma-Al2O3 catalysts were fabricated using the impregnation method. The influence of Ce content on the catalytic performance was systematically studied in a fixed-bed reactor. The catalysts were characterized by X-ray photoelectron spectroscopy, X-ray diffraction, scanning electron microscopy, and the Brunauer-Emmett-Teller technique. The reduction ability of the catalysts was recorded via H-2 temperature-programmed reduction. The valence state of Mo was raised to 6+ by the addition of Ce. What is more, the effect of temperature and GHSV were considered, and the evaluation of the optimized catalyst life catalyst was tested. A sulfur yield of 88.27% was achieved at 350 degrees C with SO2/H-2 = 1:3. |
| WOS关键词 | CARBON-MONOXIDE ; REDUCTION ; DIOXIDE ; RECOVERY ; GAS ; CO ; HYDROGEN ; MIXTURE ; METHANE ; CERIA |
| WOS研究方向 | Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:000718276400007 |
| 出版者 | AMER CHEMICAL SOC |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/51034]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Peng, Zhijian; Wang, Emiang |
| 作者单位 | 1.China Univ Geosci, Sch Engn & Technol, Beijing 100083, Peoples R China 2.Univ Chinese Acad Sci, Sch Chem Engn, Beijing 100049, Peoples R China 3.Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, Inst Proc Engn, CAS Key Lab Green Proc & Engn,State Key Lab Multi, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Yang, Yiqian,Peng, Zhijian,Zhao, Hui,et al. Ce-Modified Mo/gamma-Al2O3 Catalysts for Production of Elemental Sulfur through Reducing SO2[J]. INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,2021,60(44):15942-15950. |
| APA | Yang, Yiqian,Peng, Zhijian,Zhao, Hui,Wang, Emiang,&Li, Chunshan.(2021).Ce-Modified Mo/gamma-Al2O3 Catalysts for Production of Elemental Sulfur through Reducing SO2.INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH,60(44),15942-15950. |
| MLA | Yang, Yiqian,et al."Ce-Modified Mo/gamma-Al2O3 Catalysts for Production of Elemental Sulfur through Reducing SO2".INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH 60.44(2021):15942-15950. |
入库方式： OAI收割
来源：过程工程研究所
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