Supramolecular Hydrogel with Orthogonally Responsive R/G/B Fluorophores Enables Multi-Color Switchable Biomimetic Soft Skins
文献类型：期刊论文
| 作者 | Liu, Hao2,3; Wei, Shuxin2,3; Qiu, Huiyu2; Si, Muqing2,3; Lin, Guoqing2; Lei, Zhenkuang2,3; Lu, Wei2,3; Zhou, Lei1; Chen, Tao2,3 |
| 刊名 | ADVANCED FUNCTIONAL MATERIALS
 |
| 出版日期 | 2021-11-18 |
| 页码 | 9 |
| 关键词 | aggregation-induced emission biomimetic skins dynamic polymer networks lanthanide coordination supramolecular fluorescent hydrogels |
| ISSN号 | 1616-301X |
| DOI | 10.1002/adfm.202108830 |
| 英文摘要 | Many living creatures have evolved to show diverse appearance color changes in response to multiple environmental stimuli for attraction, warning, or disguise in their environments. However, it is challenging to construct artificial soft polymer hydrogels with similar multi-responsive multicolor tunable behaviors, but such materials can serve as soft biomimetic skins to dramatically enhance the function of certain machines. Herein, a specially designed material structure to present an innovative class of supramolecular fluorescent polymeric hydrogels with the integrated properties of wide multi-color tunability, multi-responsiveness, self-healing, and remolding capacities is proposed. A key feature of this rational hydrogel design is that multiple fluorophores (blue (B) aggregation-induced emissive and red/green (R/G) lanthanide coordinated ones) are organized separately into different polymer chains of one single supramolecular polymer network. Consequently, the B and R/G fluorophores are engineered to be orthogonally responsive, and the fluorescence intensity of each fluorophore can be controlled independently by different external stimuli, which contribute to multi-responsive multicolor fluorescence response. Besides, the hydrogels also have satisfying self-healing and remolding capacities. All of these promising advantages together further enabled the construction of soft biomimetic color-changing skins that can help the existing robots achieve the desirable camouflaging function. |
| WOS关键词 | SHAPE-MEMORY HYDROGELS ; CONSTRUCTION ; EMISSION ; SURFACES |
| 资助项目 | National Natural Science Foundation of China[21774138] ; National Natural Science Foundation of China[52073297] ; National Natural Science Foundation of China[51773215] ; Key Research Program of Frontier Sciences, Chinese Academy of Sciences[QYZDB-SSW-SLH036] ; National Key Research and Development Program of China[2019YFC1606603] ; Youth Innovation Promotion Association of Chinese Academy of Sciences[2019297] ; K. C. Wong Education Foundation[GJTD-2019-13] |
| WOS研究方向 | Chemistry ; Science & Technology - Other Topics ; Materials Science ; Physics |
| 语种 | 英语 |
| WOS记录号 | WOS:000720316100001 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| 资助机构 | National Natural Science Foundation of China ; Key Research Program of Frontier Sciences, Chinese Academy of Sciences ; National Key Research and Development Program of China ; Youth Innovation Promotion Association of Chinese Academy of Sciences ; K. C. Wong Education Foundation |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/51044]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Lu, Wei; Zhou, Lei; Chen, Tao |
| 作者单位 | 1.Chinese Acad Sci, Inst Proc Engn, Natl Key Lab Biochem Engn, PLA Key Lab Biopharmaceut Prod & Formulat Engn, Beijing 100190, Peoples R China 2.Chinese Acad Sci, Key Lab Marine Mat & Related Technol, Zhejiang Key Lab Marine Mat & Protect Technol, Ningbo Inst Mat Technol & Engn, Ningbo 315201, Peoples R China 3.Univ Chinese Acad Sci, Sch Chem Sci, 19A Yuquan Rd, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Liu, Hao,Wei, Shuxin,Qiu, Huiyu,et al. Supramolecular Hydrogel with Orthogonally Responsive R/G/B Fluorophores Enables Multi-Color Switchable Biomimetic Soft Skins[J]. ADVANCED FUNCTIONAL MATERIALS,2021:9. |
| APA | Liu, Hao.,Wei, Shuxin.,Qiu, Huiyu.,Si, Muqing.,Lin, Guoqing.,...&Chen, Tao.(2021).Supramolecular Hydrogel with Orthogonally Responsive R/G/B Fluorophores Enables Multi-Color Switchable Biomimetic Soft Skins.ADVANCED FUNCTIONAL MATERIALS,9. |
| MLA | Liu, Hao,et al."Supramolecular Hydrogel with Orthogonally Responsive R/G/B Fluorophores Enables Multi-Color Switchable Biomimetic Soft Skins".ADVANCED FUNCTIONAL MATERIALS (2021):9. |
入库方式： OAI收割
来源：过程工程研究所
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