中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
首页 机构 成果 学者
  
  1. CAS IR Grid
  2. 过程工程研究所
  3. 中国科学院过程工程研究所
Facile synthesis of magnetic recyclable Fe3O4@PDA@MoS2 nanocomposites for effectively hydrocracking of residue

文献类型：期刊论文

作者Zhu, Xiangyang1,2; Wang, Wenjie3; Xing, Huifang1,2,4; Bi, Qinling5; Wang, Li1; Rong, Meng1,2; Ni, Shan1,2; Yuan, Menglei1,2; Yang, Liangrong1,2,4; Liu, Huizhou1,2,4
刊名JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING
出版日期2021-12-01
卷号9期号:6页码:10
关键词Core-shell-shell Magnetic MoS2 Catalyst Hydrocracking
DOI10.1016/j.jece.2021.106839
英文摘要Magnetic nanocomposites provide manifold perspectives for sustainable development. However, the cumbersome operation process and energy consumption after treatment limit its application in the practical industry. Herein, we present a simple and universal strategy to synthesize Fe3O4@PDA@shell nanoparticles via in-situ homogeneous hydrolysis reaction growth different nanomaterials on the PDA modified Fe3O4 nanospheres, which can avoid multistep repetitive washing, redispersing, and drying. As an example, we introduced the synthesis process of Fe3O4@PDA@MoS2 catalyst used for heavy oil hydrocracking in detail. The synthesis processes were significantly simplified and the dispersity and stability of the nanosized MoS2 were improved due to the copious functional groups and strong adhesion properties of polydopamine. The as-prepared Fe3O4@P-DA@MoS2 nanoparticle catalysts showed high activity and excellent stability. The viscosity of residue was decreased by 99.8% and the recovery of the catalyst reached 90% under harsh conditions (405 degrees C at 13 MPa H-2). We also demonstrate the versatility of this strategy for other shell materials, such as WS2, VS2, Pd, and Rh components, which is promising for designing multifunctional core-shell-shell materials for various applications.
WOS关键词HALF-SHELLS ; NANOPARTICLES ; MOS2 ; REMOVAL ; NANOSTRUCTURES ; NANOCATALYSTS ; CONVERSION ; ADSORBENT ; CATALYSTS ; HYDROGEN
资助项目National Natural Science Foundation of China[21922814] ; National Natural Science Foundation of China[21961160745] ; National Natural Science Foundation of China[21921005] ; National Natural Science Foundation of China[22078333] ; National Natural Science Foundation of China[31961133019] ; Excellent Member in Youth Innovation Promotion Association, Chinese Academy of Sciences[Y202014] ; Shandong Energy Insititute[SEI I202133] ; China Petroleum Enterprise Cooperation Project[PRIKY17094] ; China Postdoctoral Science Foundation[2021M703239]
WOS研究方向Engineering
语种英语
WOS记录号WOS:000725681300008
出版者ELSEVIER SCI LTD
资助机构National Natural Science Foundation of China ; Excellent Member in Youth Innovation Promotion Association, Chinese Academy of Sciences ; Shandong Energy Insititute ; China Petroleum Enterprise Cooperation Project ; China Postdoctoral Science Foundation
源URL[http://ir.ipe.ac.cn/handle/122111/51290]  
专题中国科学院过程工程研究所
通讯作者Yang, Liangrong
作者单位1.Chinese Acad Sci, Inst Proc Engn, CAS Key Lab Green Proc & Engn, State Key Lab Biochem Engn, Beijing 100190, Peoples R China
2.Univ Chinese Acad Sci, Sch Chem Engn, Beijing 100049, Peoples R China
3.China Univ Petr, Beijing 102249, Peoples R China
4.Chinese Acad Sci, Qingdao Inst Bioenergy & Bioproc Technol, Qingdao 266061, Peoples R China
5.Petrochina, Petrochem Res Inst, Beijing 102206, Peoples R China
推荐引用方式
GB/T 7714		 Zhu, Xiangyang,Wang, Wenjie,Xing, Huifang,et al. Facile synthesis of magnetic recyclable Fe3O4@PDA@MoS2 nanocomposites for effectively hydrocracking of residue[J]. JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING,2021,9(6):10.
APA Zhu, Xiangyang.,Wang, Wenjie.,Xing, Huifang.,Bi, Qinling.,Wang, Li.,...&Liu, Huizhou.(2021).Facile synthesis of magnetic recyclable Fe3O4@PDA@MoS2 nanocomposites for effectively hydrocracking of residue.JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING,9(6),10.
MLA Zhu, Xiangyang,et al."Facile synthesis of magnetic recyclable Fe3O4@PDA@MoS2 nanocomposites for effectively hydrocracking of residue".JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING 9.6(2021):10.

入库方式： OAI收割

来源：过程工程研究所

浏览0
下载0
收藏0
其他版本

除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。