Structural architectures of polymer proton exchange membranes suitable for high-temperature fuel cell applications
文献类型：期刊论文
| 作者 | Dai, Junming2,3; Zhang, Yu2,3; Wang, Gang1; Zhuang, Yongbing2,3 |
| 刊名 | SCIENCE CHINA-MATERIALS
 |
| 出版日期 | 2021-12-24 |
| 页码 | 25 |
| 关键词 | proton exchange membranes high-temperature fuel cells structure-performance relationship proton conductivity |
| ISSN号 | 2095-8226 |
| DOI | 10.1007/s40843-021-1889-8 |
| 英文摘要 | High-temperature proton exchange membrane (HT-PEM) fuel cells offer more advantages than low-temperature PEM fuel cells. The ideal characteristics of HT-PEMs are high conductivities, low-humidity operation conditions, adequate mechanical properties, and competitive costs. Various molecular moieties, such as benzimidazole, benzo-thiazole, imide, and ether ether ketone, have been introduced to polymer chain backbones to satisfy the application requirements for HT-PEMs. The most common sulfonated polymers based on the main chain backbones have been employed to improve the rties. Side group/chain engineering, includ crosslinking, has been widely applied to HT-PEMs to further improve their proton conductivity, thermal stability, and mechanical properties. Currently, phosphoric acid-doped polybenzimidazole is the most successful polymer material for application in HT-PEMs. The compositing/blending modification methods of polymers are effective in obtaining high PA-doping levels and superior mechanical properties. In this review, the current progress of various membrane materials used for HT-PEMs is summarized. The synthesis and performance characteristics of polymers containing specific moieties in the chain backbones applied to HT-PEMs are discussed systemically. Various modification approaches and their deficiencies associated with HT-PEMs are analyzed and clarified. Prospects and future challenges are also presented. |
| WOS关键词 | ACID-DOPED POLYBENZIMIDAZOLE ; POLY(ARYLENE ETHER KETONE) ; SOLUBLE SULFONATED POLYBENZOTHIAZOLES ; CROSS-LINKED POLYBENZIMIDAZOLE ; ELECTROLYTE MEMBRANES ; COMPOSITE MEMBRANES ; PHOSPHORIC-ACID ; LOW-HUMIDITY ; POLYIMIDE COPOLYMERS ; POROUS MEMBRANES |
| 资助项目 | National Key Research and Development Program of China[2019YFC1906602] ; National Natural Science Foundation of China[U1904171] ; Foundation for "Talent Program" ; Open Fund of the State Key Laboratory of Biochemical Engineering, Institute of Process Engineering (IPE), Chinese Academy of Sciences (CAS) ; Project Fund of Jiangsu Bingcheng Hydrogen Energy Technology Co., Ltd. ; Young Backbone Teachers Training Program Foundation of Henan University of Technology |
| WOS研究方向 | Materials Science |
| 语种 | 英语 |
| WOS记录号 | WOS:000735344300002 |
| 出版者 | SCIENCE PRESS |
| 资助机构 | National Key Research and Development Program of China ; National Natural Science Foundation of China ; Foundation for "Talent Program" ; Open Fund of the State Key Laboratory of Biochemical Engineering, Institute of Process Engineering (IPE), Chinese Academy of Sciences (CAS) ; Project Fund of Jiangsu Bingcheng Hydrogen Energy Technology Co., Ltd. ; Young Backbone Teachers Training Program Foundation of Henan University of Technology |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/51565]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Wang, Gang; Zhuang, Yongbing |
| 作者单位 | 1.Henan Univ Technol, Sch Chem & Chem Engn, Zhengzhou 450001, Peoples R China 2.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, Beijing 100190, Peoples R China 3.Univ Chinese Acad Sci, Sch Chem Engn, Beijing 100049, Peoples R China |
| 推荐引用方式 GB/T 7714 | Dai, Junming,Zhang, Yu,Wang, Gang,et al. Structural architectures of polymer proton exchange membranes suitable for high-temperature fuel cell applications[J]. SCIENCE CHINA-MATERIALS,2021:25. |
| APA | Dai, Junming,Zhang, Yu,Wang, Gang,&Zhuang, Yongbing.(2021).Structural architectures of polymer proton exchange membranes suitable for high-temperature fuel cell applications.SCIENCE CHINA-MATERIALS,25. |
| MLA | Dai, Junming,et al."Structural architectures of polymer proton exchange membranes suitable for high-temperature fuel cell applications".SCIENCE CHINA-MATERIALS (2021):25. |
入库方式： OAI收割
来源：过程工程研究所
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