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A Review on the Design and Performance of Enzyme-Aided Catalysis of Carbon Dioxide in Membrane, Electrochemical Cell and Photocatalytic Reactors

文献类型：期刊论文

作者Ahmad Rizal Lim, Fatin Nasreen1; Marpani, Fauziah1,2; Anak Dilol, Victoria Eliz1; Mohamad Pauzi, Syazana1; Othman, Nur Hidayati1; Alias, Nur Hashimah1,2; Nik Him, Nik Raikhan1,2; Luo, Jianquan3; Abd Rahman, Norazah1
刊名MEMBRANES
出版日期2022
卷号12期号:1页码:28
关键词enzyme membrane reactor enzyme immobilization carbon dioxide reduction photocatalytic electrochemical
DOI10.3390/membranes12010028
英文摘要Multi-enzyme cascade catalysis involved three types of dehydrogenase enzymes, namely, formate dehydrogenase (FDH), formaldehyde dehydrogenase (FaldDH), alcohol dehydrogenase (ADH), and an equimolar electron donor, nicotinamide adenine dinucleotide (NADH), assisting the reaction is an interesting pathway to reduce thermodynamically stable molecules of CO2 from the atmosphere. The biocatalytic sequence is interesting because it operates under mild reaction conditions (low temperature and pressure) and all the enzymes are highly selective, which allows the reaction to produce three basic chemicals (formic acid, formaldehyde, and methanol) in just one pot. There are various challenges, however, in applying the enzymatic conversion of CO2, namely, to obtain high productivity, increase reusability of the enzymes and cofactors, and to design a simple, facile, and efficient reactor setup that will sustain the multi-enzymatic cascade catalysis. This review reports on enzyme-aided reactor systems that support the reduction of CO2 to methanol. Such systems include enzyme membrane reactors, electrochemical cells, and photocatalytic reactor systems. Existing reactor setups are described, product yields and biocatalytic productivities are evaluated, and effective enzyme immobilization methods are discussed.
WOS关键词FORMATE DEHYDROGENASE ; CO2 REDUCTION ; RECENT PROGRESS ; EFFICIENT CONVERSION ; METHANOL ; IMMOBILIZATION ; GRAPHENE ; REGENERATION ; FORMALDEHYDE ; SYSTEM
资助项目Ministry of Higher Education, Malaysia under the Fundamental Research Grant Scheme[FRGS/1/2019/TK02/UITM/03/5]
WOS研究方向Biochemistry & Molecular Biology ; Chemistry ; Engineering ; Materials Science ; Polymer Science
语种英语
WOS记录号WOS:000750551100001
出版者MDPI
资助机构Ministry of Higher Education, Malaysia under the Fundamental Research Grant Scheme
源URL[http://ir.ipe.ac.cn/handle/122111/51911]  
专题中国科学院过程工程研究所
通讯作者Marpani, Fauziah
作者单位1.Univ Teknol MARA, Coll Engn, Sch Chem Engn, Shah Alam 40450, Malaysia
2.Univ Teknol MARA, Coll Engn, Sch Chem Engn, Catalysis Sustainable Water & Energy Nexus Res Gr, Shah Alam 40450, Malaysia
3.Chinese Acad Sci, Inst Proc Engn, State Key Lab Biochem Engn, Beijing 100190, Peoples R China
推荐引用方式
GB/T 7714		 Ahmad Rizal Lim, Fatin Nasreen,Marpani, Fauziah,Anak Dilol, Victoria Eliz,et al. A Review on the Design and Performance of Enzyme-Aided Catalysis of Carbon Dioxide in Membrane, Electrochemical Cell and Photocatalytic Reactors[J]. MEMBRANES,2022,12(1):28.
APA Ahmad Rizal Lim, Fatin Nasreen.,Marpani, Fauziah.,Anak Dilol, Victoria Eliz.,Mohamad Pauzi, Syazana.,Othman, Nur Hidayati.,...&Abd Rahman, Norazah.(2022).A Review on the Design and Performance of Enzyme-Aided Catalysis of Carbon Dioxide in Membrane, Electrochemical Cell and Photocatalytic Reactors.MEMBRANES,12(1),28.
MLA Ahmad Rizal Lim, Fatin Nasreen,et al."A Review on the Design and Performance of Enzyme-Aided Catalysis of Carbon Dioxide in Membrane, Electrochemical Cell and Photocatalytic Reactors".MEMBRANES 12.1(2022):28.

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来源：过程工程研究所

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