Nitrogen-doped hydrochars from shrimp waste as visible-light photocatalysts: Roles of nitrogen species
文献类型：期刊论文
| 作者 | Chen, Zeliang1,2; Jia, Hongxia3; Guo, Yanchuan4; Li, Yi5; Liu, Zhengang1,2 |
| 刊名 | ENVIRONMENTAL RESEARCH
 |
| 出版日期 | 2022-05-15 |
| 卷号 | 208页码:8 |
| ISSN号 | 0013-9351 |
| 关键词 | Waste biomass Hydrothermal carbonization Nitrogen doping Metal-free photocatalyst Photocatalysis Hydroxyl radicals |
| DOI | 10.1016/j.envres.2022.112695 |
| 英文摘要 | The increasing shrimp waste production has caused severe environmental problems. In this study, nitrogen doped hydrochars (NDHCs) were facilely synthesized from shrimp waste and glucose by one-pot hydrothermal carbonization (HTC). The characterizations showed that NDHCs had large surface areas of up to 30.5 m(2) g(-1) with numerous functional groups on their porous surfaces. The nitrogen content (1.3-2.8%) and species distribution in NDHCs were associated with the amount of added glucose. These NDHCs were applied as visible-light-induced photocatalysts, and their photocatalytic performances were evaluated by methylene blue (MB) degradation. The removal rate of MB reached 88.9% after 1 h of visible light radiation by NDHC-1, which was 2.3 times higher than that of glucose-derived hydrochar (GHC). The mechanism study showed that the improved photoactivity of NDHCs was attributed to the increased adsorption capacity by porous surface and the promoted formation of hydroxyl radicals by synergistic effects of quaternary N and pyrrolic N during photocatalysis. This study offered a green approach to preparing tunable, efficient, and low-cost photocatalyst from waste biomass and insight into the photocatalytic mechanism of hydrochar materials. |
| WOS关键词 | HYDROTHERMAL CARBONIZATION ; GRAPHENE ; CARBONS |
| 资助项目 | Key Research Program of Chinese Academy of Sciences, China[ZDRW-ZS-2018-1-3] ; Science andTechnology Service Network (STS) Program of Chinese Academy of Sciences,China[KFJ-STS-QYZX-101] ; Shandong Province Key Research and Development Program, China[2021CXGC010803] |
| WOS研究方向 | Environmental Sciences & Ecology ; Public, Environmental & Occupational Health |
| 语种 | 英语 |
| 出版者 | ACADEMIC PRESS INC ELSEVIER SCIENCE |
| WOS记录号 | WOS:000760190000002 |
| 资助机构 | Key Research Program of Chinese Academy of Sciences, China ; Science andTechnology Service Network (STS) Program of Chinese Academy of Sciences,China ; Shandong Province Key Research and Development Program, China |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/52252]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Liu, Zhengang |
| 作者单位 | 1.Chinese Acad Sci, Res Ctr Ecoenvironm Sci, 18 Shuangqing Rd, Beijing 100085, Peoples R China 2.Univ Chinese Acad Sci, Beijing 100049, Peoples R China 3.Informat Ctr Minist Ecol & Environm, 1 Yuhui South Rd, Beijing 100029, Peoples R China 4.Chinese Acad Sci, Tech Inst Phys & Chem, Key Lab Photochem Convers & Optoelect Mat, 29 Zhongguancun East Rd, Beijing 100190, Peoples R China 5.Chinese Acad Sci, Inst Proc Engn IPE, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Chen, Zeliang,Jia, Hongxia,Guo, Yanchuan,et al. Nitrogen-doped hydrochars from shrimp waste as visible-light photocatalysts: Roles of nitrogen species[J]. ENVIRONMENTAL RESEARCH,2022,208:8. |
| APA | Chen, Zeliang,Jia, Hongxia,Guo, Yanchuan,Li, Yi,&Liu, Zhengang.(2022).Nitrogen-doped hydrochars from shrimp waste as visible-light photocatalysts: Roles of nitrogen species.ENVIRONMENTAL RESEARCH,208,8. |
| MLA | Chen, Zeliang,et al."Nitrogen-doped hydrochars from shrimp waste as visible-light photocatalysts: Roles of nitrogen species".ENVIRONMENTAL RESEARCH 208(2022):8. |
入库方式： OAI收割
来源：过程工程研究所
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