High flux Fe/activated carbon membranes for efficient degradation of organic pollutants in water by activating sodium persulfate
文献类型：期刊论文
| 作者 | Chen, Long1; Ren, Xiaomin1; Li, Yanxiang2; Hu, Dan1; Feng, Xudong1; Liu, Ye1; Zhao, Juanjuan3 |
| 刊名 | SEPARATION AND PURIFICATION TECHNOLOGY
 |
| 出版日期 | 2022-03-15 |
| 卷号 | 285页码:13 |
| 关键词 | Persulfate Activated carbon Membrane Humic acid Synchronized treatment |
| ISSN号 | 1383-5866 |
| DOI | 10.1016/j.seppur.2021.120411 |
| 英文摘要 | Efficient removal of organic pollutants in water is an important task and difficult problem in environmental treatment. In this paper, activated carbon supported Fe ions catalyst (Fe/AC) was prepared by a modulated hydrothermal approach for catalytic activating sodium persulfate (PS) to remove trace of humic acid (HA) in water. The effect of the dosage of Fe/AC and PS, the initial content of HA, pH, temperature, inorganic salt on the degradation of HA were analyzed. At the optimum condition, the advanced oxidation system achieved removal efficiencies of HA, TOC and chromaticity of 99.92%, 70.50% and 96.43%, respectively by adding 1.0 g/L Fe/AC and 0.30 g/L PS into 30 mg/L HA solution for 2 h. With increasing temperature and ionic concentration, the degradation rate was promoted. The regeneration efficiency of the catalyst was 66.70% as the reduction of active sites in AC. Electron paramagnetic resonance (EPR) and quenching tests were used to investigate the mechanism and both sulfate radicals (center dot & nbsp;SO4-) and hydroxyl radicals (center dot & nbsp;OH) were verified as dominant force responsible for HA degradation. Furthermore, a constant HA solution with PS was cross-flow filtrated by Fe/AC membrane within 20 h with excellent rejection of HA (93.33%) and high flux (298.8 L.m(-2).h(-1)) under 0.1 MPa. The loaded Fe/AC effectively reduced the membrane fouling by HA and the coupled technology improved activation capacity of the Fe/AC. Other pollutions including amoxicillin, rhodamine B and methyl orange were employed to investigate the performance of the catalytic membrane. The combined technology exhibits an excellent performance of removing organic pollutants from water and provides a new idea for water environmental management. |
| WOS关键词 | WASTE-WATER ; HUMIC ACIDS ; OXIDATION ; DYE ; REMOVAL ; MICROWAVE ; SULFATE ; PEROXYMONOSULFATE ; ULTRAFILTRATION ; RADICALS |
| 资助项目 | Scientific Technological Innovation Service Ability Construction-Basic Scientific Research Funding[PXM2020_014213_000017] ; Open Research Fund Program of Key Laboratory of Cleaner Production and Integrated Resource Utilization of China National Light Industry[CP-2020YB4] ; Research Foundation for Youth Scholars of Beijing Technology and Business University[QNJJ2020-18] ; Postgraduate Research Ability Enhancement Project in 2020 and 2021[19008020144] ; Postgraduate Research Ability Enhancement Project in 2020 and 2021[19008021082] |
| WOS研究方向 | Engineering |
| 语种 | 英语 |
| WOS记录号 | WOS:000780444500003 |
| 出版者 | ELSEVIER |
| 资助机构 | Scientific Technological Innovation Service Ability Construction-Basic Scientific Research Funding ; Open Research Fund Program of Key Laboratory of Cleaner Production and Integrated Resource Utilization of China National Light Industry ; Research Foundation for Youth Scholars of Beijing Technology and Business University ; Postgraduate Research Ability Enhancement Project in 2020 and 2021 |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/52757]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Hu, Dan; Feng, Xudong |
| 作者单位 | 1.Beijing Technol & Business Univ, Sch Light Ind, Key Lab Cleaner Prod & Integrated Resource Utiliz, Beijing 100048, Peoples R China 2.Chinese Acad Sci, CAS Key Lab Green Proc & Engn, Inst Proc Engn, Beijing 100190, Peoples R China 3.Beijing Normal Univ, Coll Water Sci, Beijing 100875, Peoples R China |
| 推荐引用方式 GB/T 7714 | Chen, Long,Ren, Xiaomin,Li, Yanxiang,et al. High flux Fe/activated carbon membranes for efficient degradation of organic pollutants in water by activating sodium persulfate[J]. SEPARATION AND PURIFICATION TECHNOLOGY,2022,285:13. |
| APA | Chen, Long.,Ren, Xiaomin.,Li, Yanxiang.,Hu, Dan.,Feng, Xudong.,...&Zhao, Juanjuan.(2022).High flux Fe/activated carbon membranes for efficient degradation of organic pollutants in water by activating sodium persulfate.SEPARATION AND PURIFICATION TECHNOLOGY,285,13. |
| MLA | Chen, Long,et al."High flux Fe/activated carbon membranes for efficient degradation of organic pollutants in water by activating sodium persulfate".SEPARATION AND PURIFICATION TECHNOLOGY 285(2022):13. |
入库方式： OAI收割
来源：过程工程研究所
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