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Process simulation and evaluation for NH3/CO2 separation from melamine tail gas with protic ionic liquids

文献类型：期刊论文

作者Duan, Yuanmeng1,2; Zhan, Guoxiong2,3; Chang, Fei2; Shi, Sensen2; Zeng, Shaojuan2; Dong, Haifeng2; Abildskov, Jens1; Huusom, Jakob Kjobsted1; Zhang, Xiangping2,3
刊名SEPARATION AND PURIFICATION TECHNOLOGY
出版日期2022-05-01
卷号288页码:11
关键词Ionic liquid Melamine tail gas Process simulation Process evaluation
ISSN号1383-5866
DOI10.1016/j.seppur.2022.120680
英文摘要Melamine production is known to produce a tail gas with a significant amount of NH3 and CO2. The most common separation methods applied to melamine tail gas are water scrubbing and urea co-production technology. With good stability, non-volatility and tailored properties, ionic liquids (ILs) are regarded as vital potential solvents for gas separation. Therefore, two new process technologies, one is the ionic liquid-based process (IL-0), and the other is the enhanced ionic liquid process (IL-En) was employed and evaluated for energy and cost efficiency. The IL-En employs stripping on the treatment of melamine tail gas. The protic ionic liquid named 1-butyl imidazolium bis (trifluoromethylsulfonyl) imide ([Bim][NTf2]) was selected for the evaluation of the melamine tail gas cleaning process. Thermodynamic data were fitted to the NRTL equations. Three full process flowsheets were simulated in Aspen Plus V11 (TM). A basic and an enhanced ionic liquid process (IL-0 and IL-En), a conventional water scrubbing (WS) technology as a comparison, process sensitivity analysis and energy/economic evaluation were carried out. The results showed that the total separation cost of the IL-En can be reduced by 61% compared to that of the WS process. Moreover, the IL-based flowsheet is simpler than WS and avoids wastewater discharge.
WOS关键词HIGHLY EFFICIENT ; COSMO ; ABSORPTION ; CAPTURE ; SOLVENTS
资助项目National Natural Science Foundation of China[22122814] ; National Natural Science Foundation of China[21890764] ; National Natural Science Foundation of China[21921005] ; Major Scientific and Technological Innovation Project of Shandong Province of China[2019JZZY010518] ; Major Scientific and Technological Project of Shanxi Province of China[20201102005] ; Youth Innovation Promotion Association of the Chinese Academy of Sciences of China[2018064]
WOS研究方向Engineering
语种英语
WOS记录号WOS:000780427000002
出版者ELSEVIER
资助机构National Natural Science Foundation of China ; Major Scientific and Technological Innovation Project of Shandong Province of China ; Major Scientific and Technological Project of Shanxi Province of China ; Youth Innovation Promotion Association of the Chinese Academy of Sciences of China
源URL[http://ir.ipe.ac.cn/handle/122111/52764]  
专题中国科学院过程工程研究所
通讯作者Huusom, Jakob Kjobsted; Zhang, Xiangping
作者单位1.Tech Univ Denmark, Dept Chem & Biochem Engn, DK-2800 Lyngby, Denmark
2.Chinese Acad Sci, State Key Lab Multiphase Complex Syst, Beijing Key Lab Ion Liquids Clean Proc, CAS Key Lab Green Proc & Engn,Inst Proc Engn, 1 North 2nd St Zhongguancun, Beijing 100190, Peoples R China
3.Univ Chinese Acad Sci, Coll Chem & Engn, 19 A Yuquan Rd, Beijing 100049, Peoples R China
推荐引用方式
GB/T 7714		 Duan, Yuanmeng,Zhan, Guoxiong,Chang, Fei,et al. Process simulation and evaluation for NH3/CO2 separation from melamine tail gas with protic ionic liquids[J]. SEPARATION AND PURIFICATION TECHNOLOGY,2022,288:11.
APA Duan, Yuanmeng.,Zhan, Guoxiong.,Chang, Fei.,Shi, Sensen.,Zeng, Shaojuan.,...&Zhang, Xiangping.(2022).Process simulation and evaluation for NH3/CO2 separation from melamine tail gas with protic ionic liquids.SEPARATION AND PURIFICATION TECHNOLOGY,288,11.
MLA Duan, Yuanmeng,et al."Process simulation and evaluation for NH3/CO2 separation from melamine tail gas with protic ionic liquids".SEPARATION AND PURIFICATION TECHNOLOGY 288(2022):11.

入库方式： OAI收割

来源：过程工程研究所

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