Poly(ionic liquid)-Armored MXene Membrane: Interlayer Engineering for Facilitated Water Transport
文献类型：期刊论文
| 作者 | Yi, Ming1,2,3; Wang, Mi4; Wang, Yan1,2; Wang, Yanlei4; Chang, Jian3; Kheirabad, Atefeh Khorsand3; He, Hongyan4; Yuan, Jiayin3; Zhang, Miao3 |
| 刊名 | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
 |
| 出版日期 | 2022-05-03 |
| 页码 | 8 |
| 关键词 | Anion Exchange Assembly MXene Nanochannel Hydrophilicity Poly(Ionic Liquid) |
| ISSN号 | 1433-7851 |
| DOI | 10.1002/anie.202202515 |
| 英文摘要 | Two-dimensional (2D) MXene-based lamellar membranes bearing interlayers of tunable hydrophilicity are promising for high-performance water purification. The current challenge lies in how to engineer the pore wall's surface properties in the subnano-confinement environment while ensuring its high selectivity. Herein, poly(ionic liquid)s, equipped with readily exchangeable counter anions, succeeded as a hydrophilicity modifier in addressing this issue. Lamellar membranes bearing nanochannels of tailorable hydrophilicity are constructed via assembly of poly(ionic liquid)-armored MXene nanosheets. By shifting the interlayer galleries from being hydrophilic to more hydrophobic via simple anion exchange, the MXene membrane performs drastically better for both the permeance (by two-fold improvement) and rejection (approximate to 99 %). This facile method opens up a new avenue for building 2D material-based membranes of enhancing molecular transport and sieving effect. |
| WOS关键词 | ULTRATHIN ; LIQUID)S ; CHANNELS |
| 资助项目 | National Key Research and Development Program of China[2020YFB1709301] ; Wallenberg Academy Fellow program of the Knut & Alice Wallenberg Foundation in Sweden[KAW 2017.0166] ; Swedish Research Council in Sweden[202105839] ; National Natural Science Foundation of China[21922813] ; Youth Innovation Promotion Association of CAS[2021046] ; Youth Innovation Promotion Association of CAS[Y2021022] ; China Scholarship Council[202006160136] |
| WOS研究方向 | Chemistry |
| 语种 | 英语 |
| WOS记录号 | WOS:000789999700001 |
| 出版者 | WILEY-V C H VERLAG GMBH |
| 资助机构 | National Key Research and Development Program of China ; Wallenberg Academy Fellow program of the Knut & Alice Wallenberg Foundation in Sweden ; Swedish Research Council in Sweden ; National Natural Science Foundation of China ; Youth Innovation Promotion Association of CAS ; China Scholarship Council |
| 源URL | [http://ir.ipe.ac.cn/handle/122111/53072]  |
| 专题 | 中国科学院过程工程研究所 |
| 通讯作者 | Wang, Yan; Wang, Yanlei; Yuan, Jiayin; Zhang, Miao |
| 作者单位 | 1.Huazhong Univ Sci & Technol, Key Lab Mat Chem Energy Convers & Storage, Wuhan 430074, Peoples R China 2.Huazhong Univ Sci & Technol, Hubei Key Lab Mat Chem & Serv Failure, Sch Chem & Chem Engn, Wuhan 430074, Peoples R China 3.Stockholm Univ, Dept Mat & Environm Chem, S-10691 Stockholm, Sweden 4.Chinese Acad Sci, Beijing Key Lab Ion Liquids Clean Proc, Inst Proc Engn, State Key Lab Multiphase Complex Syst, Beijing 100190, Peoples R China |
| 推荐引用方式 GB/T 7714 | Yi, Ming,Wang, Mi,Wang, Yan,et al. Poly(ionic liquid)-Armored MXene Membrane: Interlayer Engineering for Facilitated Water Transport[J]. ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,2022:8. |
| APA | Yi, Ming.,Wang, Mi.,Wang, Yan.,Wang, Yanlei.,Chang, Jian.,...&Zhang, Miao.(2022).Poly(ionic liquid)-Armored MXene Membrane: Interlayer Engineering for Facilitated Water Transport.ANGEWANDTE CHEMIE-INTERNATIONAL EDITION,8. |
| MLA | Yi, Ming,et al."Poly(ionic liquid)-Armored MXene Membrane: Interlayer Engineering for Facilitated Water Transport".ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022):8. |
入库方式： OAI收割
来源：过程工程研究所
浏览0
下载0
收藏0
其他版本
除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。