中国科学院机构知识库网格
Chinese Academy of Sciences Institutional Repositories Grid
首页 机构 成果 学者
  
  1. CAS IR Grid
  2. 地质与地球物理研究所
  3. 中国科学院地质与地球物理研究所
  4. 兰州油气中心
Inversion Characteristics of Hydrocarbon Gases Carbon Isotopes Varying With Temperature and Implications for Shale Exploration

文献类型：期刊论文

作者Wu, Yingqin2; Liu, Yanhong2; Wang, Tong1; Wang, Zhiyu2,3; Yuan, Longmiao2,3; Xia, Yanqin2
刊名FRONTIERS IN EARTH SCIENCE
出版日期2021-09-17
卷号9页码:8
关键词pyrolysis hydrocarbon source rocks organic matter types gas carbon isotope isotope inversion
DOI10.3389/feart.2021.620161
英文摘要In order to understand the influence of source rock types and maturity on hydrocarbon gases carbon isotope change more objectively, a closed-system pyrolysis experiment was carried out on six samples from 250 to 550 degrees C. The values of delta C-13(1), delta C-13(2), and delta C-13(3) were ranged from -73.3 to -29.8%, from -36.3 to -9.5%, and from -38.5 to -12.4%, respectively. The range of delta C-13(1) was the largest, reaching a top value of 43.5%. The results showed that the temperature has an effect on the carbon isotope value of pyrolysis gas. With the increase of the degree of thermal evolution, the carbon isotope value of methane in all samples, except for huangxian gangue, had a change trend from heavy to light firstly, then got heavier. In addition, the carbon isotope values of methane, ethane and propane had the features of delta C-13(1) < delta C-13(2) < delta C-13(3) when the temperatures were under 550 degrees C, which were made up of a series of positive carbon isotopes. However, when the temperature increased above 550 degrees C, there was an inversion of the simulated gas carbon isotope values in Huangxian coal gangue, Minqin oil shale and Huaan carbonaceous shale, i.e., delta C-13(2) > delta C-13(3) and delta C-13(2) > delta(1)3C(1). It indicates that the secondary cracking has occurred at high maturity or over maturity stage.
WOS关键词FORT-WORTH BASIN ; NATURAL-GAS ; BARNETT SHALE ; OIL CRACKING ; ORDOS BASIN ; GENERATION ; PYROLYSIS ; FRACTIONATION ; EVOLUTION ; REVERSAL
资助项目National Science Foundation[42072180] ; National Science Foundation[41772147] ; National Science Foundation[41272147] ; National Science Foundation[41831176] ; National Key R&D Program of China[2017YFA0604803] ; Chinese Academy of Sciences Instrument Equipment Function Development Technology Innovation Project[E0280101]
WOS研究方向Geology
语种英语
出版者FRONTIERS MEDIA SA
WOS记录号WOS:000728822500001
资助机构National Science Foundation ; National Science Foundation ; National Key R&D Program of China ; National Key R&D Program of China ; Chinese Academy of Sciences Instrument Equipment Function Development Technology Innovation Project ; Chinese Academy of Sciences Instrument Equipment Function Development Technology Innovation Project ; National Science Foundation ; National Science Foundation ; National Key R&D Program of China ; National Key R&D Program of China ; Chinese Academy of Sciences Instrument Equipment Function Development Technology Innovation Project ; Chinese Academy of Sciences Instrument Equipment Function Development Technology Innovation Project ; National Science Foundation ; National Science Foundation ; National Key R&D Program of China ; National Key R&D Program of China ; Chinese Academy of Sciences Instrument Equipment Function Development Technology Innovation Project ; Chinese Academy of Sciences Instrument Equipment Function Development Technology Innovation Project ; National Science Foundation ; National Science Foundation ; National Key R&D Program of China ; National Key R&D Program of China ; Chinese Academy of Sciences Instrument Equipment Function Development Technology Innovation Project ; Chinese Academy of Sciences Instrument Equipment Function Development Technology Innovation Project
源URL[http://ir.iggcas.ac.cn/handle/132A11/103907]  
专题地质与地球物理研究所_兰州油气中心
通讯作者Wu, Yingqin
作者单位1.Newcastle Univ, Sch Engn, Newcastle, England
2.Chinese Acad Sci, Gansu Prov Northwest Inst Ecoenvironm & Resources, Key Lab Petr Resources, Lanzhou, Peoples R China
3.Univ Chinese Acad Sci, Beijing, Peoples R China
推荐引用方式
GB/T 7714		 Wu, Yingqin,Liu, Yanhong,Wang, Tong,et al. Inversion Characteristics of Hydrocarbon Gases Carbon Isotopes Varying With Temperature and Implications for Shale Exploration[J]. FRONTIERS IN EARTH SCIENCE,2021,9:8.
APA Wu, Yingqin,Liu, Yanhong,Wang, Tong,Wang, Zhiyu,Yuan, Longmiao,&Xia, Yanqin.(2021).Inversion Characteristics of Hydrocarbon Gases Carbon Isotopes Varying With Temperature and Implications for Shale Exploration.FRONTIERS IN EARTH SCIENCE,9,8.
MLA Wu, Yingqin,et al."Inversion Characteristics of Hydrocarbon Gases Carbon Isotopes Varying With Temperature and Implications for Shale Exploration".FRONTIERS IN EARTH SCIENCE 9(2021):8.

入库方式： OAI收割

来源：地质与地球物理研究所

浏览0
下载0
收藏0
其他版本

除非特别说明，本系统中所有内容都受版权保护，并保留所有权利。